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Ion transport in porous media is present in a wealth of technologies, e.g., energy storage devices such as batteries and supercapacitors, and environmental technologies such as electrochemical carbon capture and capacitive deionization.…

Soft Condensed Matter · Physics 2022-06-17 Filipe Henrique , Pawel J. Zuk , Ankur Gupta

We numerically simulate the transport of elliptic Janus particles along narrow two-dimensional channels with reflecting walls. The self-propulsion velocity of the particle is oriented along either their major (prolate) or minor axis…

Biological Physics · Physics 2014-06-24 Pulak K. Ghosh , Peter Hanggi , Fabio Marchesoni , Franco Nori

Membranes are ubiquitous in nature with primary functions that include adaptive filtering and selective transport of chemical and molecular species. Being critical to cellular functions, they are also fundamental in many areas of science…

In living cells, molecular motors create activity that enhances the diffusion of particles throughout the cytoplasm, and not just ones attached to the motors. We demonstrate initial steps toward creating artificial cells that mimic this…

Soft Condensed Matter · Physics 2019-05-01 Viva R. Horowitz , Zachary C. Chambers , İrep Gözen , Thomas G. Dimiduk , Vinothan N. Manoharan

The alteration of the dielectric membrane properties by membrane engineering techniques such as carbon nanotube (CNT) coating opens the way to novel molecular transport strategies for biosensing purposes. In this article, we predict a…

Soft Condensed Matter · Physics 2022-01-12 Sahin Buyukdagli

Microfluidic channels with embedded ion permselective medium under the application of electric current are commonly used for electrokinetic processes as on-chip ion concentration polarization (ICP) and bioparticle preconcentration to…

Fluid Dynamics · Physics 2022-11-22 Barak Sabbagh , Sinwook Park , Gilad Yossifon

We review recent advances in rectification control of artificial microswimmers, also known as Janus particles, diffusing along narrow, periodically corrugated channels. The swimmer self-propulsion mechanism is modeled so as to incorporate a…

Soft Condensed Matter · Physics 2014-12-19 Xue Ao , Pulak Kumar Ghosh , Yunyun Li , Gerhard Schmid , Peter Hänggi , Fabio Marchesoni

Transport of ions and small molecules across the cell membrane against electrochemical gradients is catalyzed by integral membrane proteins that use a source of free energy to drive the energetically uphill flux of the transported…

Biomolecules · Quantitative Biology 2022-03-25 Oliver Beckstein , Fiona Naughton

We develop a correlation-corrected transport theory in order to predict ionic and polymer transport properties of membrane nanopores in physical conditions where mean-field electrostatics breaks down. The experimentally observed low KCl…

Soft Condensed Matter · Physics 2014-11-06 Sahin Buyukdagli , Tapio Ala-Nissila

To overcome the traditional paradigm of filtration, where separation is essentially performed upon steric sieving principles, we explore the concept of dynamic osmosis through active membranes. A partially permeable membrane presents a…

Soft Condensed Matter · Physics 2020-02-10 Sophie Marbach , Nikita Kavokine , Lyderic Bocquet

The optimal functioning of nanopore-based biosensing tools necessitates rapid polymer capture from the ion reservoir. We identify an ionic correlation-induced transport mechanism that provides this condition without the chemical…

Soft Condensed Matter · Physics 2018-05-10 Sahin Buyukdagli

The past decade has witnessed the rapid progress in synthesizing nanoporous organic networks or polymer frameworks for various potential applications. Generally speaking, functionalization of porous networks to add extra properties and…

Materials Science · Physics 2016-10-11 Jian-Ke Sun , Markus Antonietti , Jiayin Yuan

We investigate the mobility of nanometer-size solutes in water in a uniform external electric field. General arguments are presented to show that a closed surface cutting a volume from a polar liquid will carry an effective non-zero surface…

Soft Condensed Matter · Physics 2016-08-24 Mohammadhasan Dinpajooh , Dmitry V. Matyushov

The shift in water security demands improvements in alternative solutions such as saltwater desalination. One of the most efficient technologies in this scope is the reverse osmosis systems, a technology based on a membrane separation…

Soft Condensed Matter · Physics 2024-06-19 João P. K. Abal , Marcia C. Barbosa

Nanopores are both a tool to study single-molecule biophysics and nanoscale ion transport, but also a promising material for desalination or osmotic power generation. Understanding the physics underlying ion transport through nano-sized…

Soft Condensed Matter · Physics 2021-04-02 Sanjin Marion , Michal Macha , Sebastian J. Davis , Andrey Chernev , Aleksandra Radenovic

Using computer simulations, we study a membrane of parallel narrow pores filled with one-dimensional wires of hydrogen-bonded water molecules. We show that such a membrane is equivalent to a system of effective charges located at opposite…

Computational Physics · Physics 2018-05-24 Georg Menzl , Jürgen Köfinger , Christoph Dellago

We present a numerical study of nonlinear electrokinetic transport in porous media, focusing on the role of heterogeneity in a porous microstructure on ion concentration polarization and over-limiting current. For simplicity, the porous…

Fluid Dynamics · Physics 2019-01-10 Shima Alizadeh , Martin Z. Bazant , Ali Mani

Effective Poisson-Nernst-Planck (PNP) equations are derived for macroscopic ion transport in charged porous media under periodic fluid flow by an asymptotic multi-scale expansion with drift. The microscopic setting is a two-component…

Mathematical Physics · Physics 2014-07-16 Markus Schmuck , Martin Z. Bazant

Ion channels orchestrate the communication between cells and their environment. These are special proteins capable of changing their shape to allow ions to pass through membranes in response to stimuli like membrane tension. As the letters…

Biological Physics · Physics 2024-09-17 Uğur Çetiner

Optical forces - studied since the earliest days of laser physics - continue to reveal rich dynamics and enable powerful tools for manipulation of objects on micro- and nanoscales, and even individual atoms. Lateral optical forces, which…