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We present a systematic investigation of the low-frequency charge carrier dynamics in different charge states of the organic conductors $\theta$-(BEDT-TTF)$_2$$M$Zn(SCN)$_4$ with $M$=Rb,Tl, which result from quenching or relaxing the charge…

Strongly Correlated Electrons · Physics 2022-05-25 Tatjana Thomas , Tim Thyzel , Hungwei Sun , Kenichiro Hashimoto , Takahiko Sasaki , Hiroshi M. Yamamoto , Jens Müller

We have studied the low-frequency dynamics of the charge carriers in different organic charge-transfer salts $\kappa$-(BEDT-TTF)$_2$X with polymeric anions X by using resistance noise spectroscopy. Our aim is to investigate the structural,…

Strongly Correlated Electrons · Physics 2015-09-30 J. Müller , B. Hartmann , R. Rommel , J. Brandenburg , S. M. Winter , J. A. Schlueter

We present results of the coefficient of thermal expansion for the frustrated quasi-two-dimensional molecular conductor $\theta$-(BEDT-TTF)$_2$RbZn(SCN)$_4$ for temperatures 1.5 K $\leq T \leq$ 290 K. A pronounced first-order phase…

Strongly Correlated Electrons · Physics 2024-05-08 Yohei Saito , Owen Ganter , Chao Shang , Kenichiro Hashimoto , Takahiko Sasaki , Stephen M. Winter , Jens Müller , Michael Lang

The critical cooling rate $R_{\rm c}$ above which charge ordering is kinetically avoided upon cooling, which results in charge-glass formation, was investigated for the geometrically frustrated system $\theta$-(BEDT-TTF)$_2X$. X-ray…

Strongly Correlated Electrons · Physics 2014-08-14 T. Sato , F. Kagawa , K. Kobayashi , A. Ueda , H. Mori , K. Miyagawa , K. Kanoda , R. Kumai , Y. Murakami , Y. Tokura

Geometrically frustrated spin systems often do not exhibit long-range ordering, resulting in either quantum-mechanically disordered states, such as quantum spin liquids, or classically disordered states, such as spin ices or spin glasses.…

Strongly Correlated Electrons · Physics 2013-11-07 F. Kagawa , T. Sato , K. Miyagawa , K. Kanoda , Y. Tokura , K. Kobayashi , R. Kumai , Y. Murakami

We utilize a glass-like structural transition in order to induce a Mott metal-insulator transition in the quasi-two-dimensional organic charge-transfer salt $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br. In this material, the terminal ethylene…

Strongly Correlated Electrons · Physics 2014-12-19 B. Hartmann , J. Müller , T. Sasaki

Non-equilibrium charge dynamics, such as cooling-rate-dependent charge vitrification and physical aging, have been demonstrated for a charge-cluster glass in $\theta$-(BEDT-TTF)$_2$CsZn(SCN)$_4$ using electron transport measurements. The…

Strongly Correlated Electrons · Physics 2014-03-17 T. Sato , F. Kagawa , K. Kobayashi , K. Miyagawa , K. Kanoda , R. Kumai , Y. Murakami , Y. Tokura

We present a scenario for the peculiar coexistence of charge fluctuations observed in quasi-2D 1/4-filled organic conductors $\theta$-(BEDT-TTF)$_2X$ in the quantum critical regime where the charge ordering is suppressed down to zero…

Strongly Correlated Electrons · Physics 2009-11-13 Masafumi Udagawa , Yukitoshi Motome

We present high-resolution measurements of the relative length change as a function of temperature of the organic charge-transfer salt $\kappa$-(BEDT-TTF)$_2$Hg(SCN)$_2$Cl. We identify anomalous features at $T_g \approx\,63$ K which can be…

Strongly Correlated Electrons · Physics 2018-02-14 Elena Gati , Stephen M. Winter , John A. Schlueter , Harald Schubert , Jens Müller , Michael Lang

We describe our perspective on the Structural Glass Transition (SGT) problem built on the premise that a viable theory must provide a consistent picture of the dynamics and statics, which are manifested by large increase in shear viscosity…

Soft Condensed Matter · Physics 2009-12-15 T. R. Kirkpatrick , D. Thirumalai

Understanding the physics of glass formation remains one of the major unsolved challenges of condensed matter science. As a material solidifies into a glass, it exhibits a spectacular slowdown of the dynamics upon cooling or compression,…

Statistical Mechanics · Physics 2018-10-03 Liesbeth M. C. Janssen

Complementary Neutron Spin Echo and X-ray experiments and Molecular Dynamics simulations have been performed on difluorotetrachloroethane (CFCl2-CFCl2) glassy crystal. Static, single-molecule reorientational dynamics and collective dynamics…

Soft Condensed Matter · Physics 2009-11-11 F. Affouard , E. Cochin , F. Danède , R. Decressain , M. Descamps , W. Haeussler

We investigate the characteristic length scales associated with the glass transition phenomenon. By studying an atomic glass-forming liquid in negatively curved space, for which the local order is well identified and the amount of…

Statistical Mechanics · Physics 2010-02-10 François Sausset , Gilles Tarjus

We introduce a new quantity to probe the glass transition. This quantity is a linear generalized compressibility which depends solely on the positions of the particles. We have performed a molecular dynamics simulation on a glass forming…

Disordered Systems and Neural Networks · Physics 2009-11-07 Herve M. Carruzzo , Clare C. Yu

The structural arrest of a polymeric suspension might be driven by an increase of the cross--linker concentration, that drives the gel transition, as well as by an increase of the polymer density, that induces a glass transition. These…

Statistical Mechanics · Physics 2014-06-20 Nagi Khalil , Antonio Coniglio , Antonio de Candia , Annalisa Fierro , Massimo Pica Ciamarra

We show that introducing long-range Coulomb interactions immediately lifts the massive ground state degeneracy induced by geometric frustration for electrons on quarter-filled triangular lattices in the classical limit. Important…

Strongly Correlated Electrons · Physics 2015-07-22 Samiyeh Mahmoudian , Louk Rademaker , Arnaud Ralko , Simone Fratini , Vladimir Dobrosavljević

Studies of low-frequency resistance noise demonstrate that glassy freezing occurs in a two-dimensional electron system in silicon in the vicinity of the metal-insulator transition (MIT). The width of the metallic glass phase, which…

Strongly Correlated Electrons · Physics 2009-11-10 D. Popovic , S. Bogdanovich , J. Jaroszynski , T. M. Klapwijk

The dynamical arrest of gels is the consequence of a well defined structural phase transition, leading to the formation of a spanning cluster of bonded particles. The dynamical glass transition, instead, is not accompanied by any clear…

Soft Condensed Matter · Physics 2016-07-21 Raffaele Pastore , Antonio de Candia , Anallisa Fierro , Massimo Pica Ciamarra , Antonio Coniglio

We consider the stationary state of a fluid comprised of inelastic hard spheres or disks under the influence of a random, momentum-conserving external force. Starting from the microscopic description of the dynamics, we derive a nonlinear…

Statistical Mechanics · Physics 2013-02-25 W. T. Kranz , M. Sperl , A. Zippelius

We present a detailed structural investigation of the organic superconductor $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br at temperatures $T$ from 9 to 300 K. Anomalies in the $T$ dependence of the lattice parameters are associated with a…

Materials Science · Physics 2016-08-16 A. U. B. Wolter , R. Feyerherm , E. Dudzik , S. Süllow , Ch. Strack , M. Lang , D. Schweitzer
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