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The interaction of matter with a quantized electromagnetic mode is considered. Representing a strong exciting field, the mode is assumed to contain a large number of photons. As a result, the material response is highly nonlinear: the…

Quantum Physics · Physics 2020-01-17 Ákos Gombkötő , Sándor Varró , Péter Mati , Péter Földi

High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…

High-harmonic generation (HHG) normally requires a careful adjustment of the driving laser intensity (typically $10^{14} - 10^{15}$ W/cm$^2$) and gas medium parameters to enable good phase matching conditions. In contrast with conventional…

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

Atomic Physics · Physics 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

We present a study of photon statistics associated with high-order harmonic generation (HHG) involving one-mode and intermodal correlations of the high harmonic photons. The aim of the paper is to give insight into the nonclassical…

Quantum Physics · Physics 2021-09-15 Ákos Gombkötő , Péter Földi , Sándor Varró

We theoretically investigate high-order harmonic generation (HHG) in graphene under mid-infrared (MIR) and terahertz (THz) fields based on a quantum master equation. Numerical simulations show that MIR-induced HHG in graphene can be…

Materials Science · Physics 2023-07-03 Wenwen Mao , Angel Rubio , Shunsuke A. Sato

We report on theoretical study of second harmonic generation in graphene. Phenomenological analysis based on symmetry arguments is carried out. It is demontrated, that in ideal graphene samples second harmonic generation is possible only if…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 M. M. Glazov

We report calculations of the high harmonic generation spectra of the C\textsubscript{60} fullerene molecule, employing a diverse set of real-time time-dependent quantum chemical methods. All methodologies involve expanding the propagated…

Chemical Physics · Physics 2023-12-05 Aleksander P. Woźniak , Robert Moszyński

We investigate the high harmonic generation (HHG) from solids by simulating the dynamics of a single active electron in periodic potentials. The corresponding time-dependent Schr\"odinger equations (TDSE) are solved numerically by using…

Atomic Physics · Physics 2016-03-31 Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

We investigate high-order harmonic generation in inhomogeneous media for reduced dimensionality models. We perform a phase-space analysis, in which we identify specific features caused by the field inhomogeneity. We compute high-order…

Atomic Physics · Physics 2016-05-25 C. Zagoya , M. Bonner , H. Chomet , E. Slade , C. Figueira de Morisson Faria

Graphene placed in a magnetic field possesses an extremely high mid/far-infrared optical nonlinearity originating from its unusual band structure and selection rules for the optical transitions near the Dirac point. Here we study the linear…

Mesoscale and Nanoscale Physics · Physics 2016-11-26 Xianghan Yao , Alexey Belyanin

We present studies of high-order harmonic generation (HHG) at laser intensities well above saturation. We use driving laser pulses which present a particular electron dynamics in the turn-on stage. Our results predict an increasing on the…

Atomic Physics · Physics 2015-06-19 J. A. Pérez-Hernández , M. F. Ciappina , M. Lewenstein , A. Zaïr , L. Roso

Using Time-Dependent Density Functional Theory (TDDFT) nonlinear nonperturbative response of the molecular system is studied for photoisomerization reaction. The 1,3-cyclohexadiene photoisomerization is probed by the high-harmonic…

Chemical Physics · Physics 2024-08-06 Lauren Bauerle , Agnieszka Jaron

The nonlinear optical and optoelectronic properties of graphene with the emphasis on the processes of harmonic generation, frequency mixing, photon drag and photogalvanic effects as well as generation of photocurrents due to coherent…

Mesoscale and Nanoscale Physics · Physics 2014-02-04 M. M. Glazov , S. D. Ganichev

In the past two decades high-harmonic generation (HHG) has become a key process in ultra-fast science due to the extremely short time-structure of the underlying electron dynamics being imprinted in the emitted harmonic light bursts. After…

Atomic Physics · Physics 2012-01-25 Markus C. Kohler , Thomas Pfeifer , Karen Z. Hatsagortsyan , Christoph H. Keitel

We present a theoretical analysis of high-order harmonic generation from ion-atom collisions in the presence of linearly polarized intense laser pulses. Photons with frequencies significantly higher than in standard atomic high-harmonic…

Atomic Physics · Physics 2009-11-10 Manfred Lein , Jan M. Rost

High-harmonic generation (HHG) is a nonlinear process in which a material sample is irradiated by intense laser pulses, causing the emission of high harmonics of the incident light. HHG has historically been explained by theories employing…

In quantum sideband high harmonic generation (QSHHG), high harmonic generation is perturbed by a bright quantum field resulting in harmonic sidebands, with the intent to transfer non-classical properties from the quantum perturbation to the…

Quantum Physics · Physics 2025-05-29 Neda Boroumand , Adam Thorpe , Graeme Bart , Lu Wang , David N. Purschke , Giulio Vampa , Thomas Brabec

We perform a detailed analysis of high-order harmonic generation (HHG) in atoms within the strong field approximation (SFA) by considering spatially inhomogeneous monochromatic laser fields. We investigate how the individual pairs of…

Atomic Physics · Physics 2015-06-05 T. Shaaran , M. F. Ciappina , M. Lewenstein
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