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Strong resonant dipole-dipole interactions in flexible Rydberg aggregates enable the formation of exciton pulses, the interplay of atomic motion and electronic excitation transfer which feature high fidelity entanglement transport. Here, we…

Quantum Physics · Physics 2016-12-26 Karsten Leonhardt

The optoelectronic and transport properties of two-dimensional transition metal dichalcogenide semiconductors (2D TMDs) are highly susceptible to external perturbation, enabling precise tailoring of material function through post-synthetic…

Mesoscale and Nanoscale Physics · Physics 2022-03-18 Haowen Su , Ding Xu , Shan-Wen Cheng , Baichang Li , Song Liu , Kenji Watanabe , Takashi Taniguchi , Timothy C. Berkelbach , James Hone , Milan Delor

In a recent publication Larson \textit{et al.} reported remarkably clear $d$-$d$ excitations for NiO and CoO measured with x-ray energies well below the transition metal $K$ edge. In this letter we demonstrate that we can obtain an accurate…

Strongly Correlated Electrons · Physics 2008-01-09 M. W. Haverkort , A. Tanaka , L. H. Tjeng , G. A. Sawatzky

The spin structure and spin dynamics of excitons in an ensemble of (In,Al)As/AlAs quantum dots (QDs) with type-I band alignment, containing both direct and indirect band gap dots, are studied. Time-resolved and spectral selective techniques…

Mesoscale and Nanoscale Physics · Physics 2019-05-15 J. Rautert , T. S. Shamirzaev , S. V. Nekrasov , D. R. Yakovlev , P. Klenovský , Yu. G. Kusrayev , M. Bayer

Time-dependent density-functional theory (TDDFT) is widely used to describe electronic excitations in complex finite systems with large numbers of atoms, such as biomolecules and nanocrystals. The first part of this paper will give a simple…

Materials Science · Physics 2008-08-15 C. A. Ullrich , V. Turkowski

Excitons drive the optoelectronic properties of organic semiconductors which underpin devices including solar cells and light-emitting diodes. Here we show that excitons can exhibit topologically non-trivial states protected by inversion…

Mesoscale and Nanoscale Physics · Physics 2025-05-21 Wojciech J. Jankowski , Joshua J. P. Thompson , Bartomeu Monserrat , Robert-Jan Slager

Two-dimensional transition metal dichalcogenides (TMD) offer a unique platform for creating van-der-Waals heterojunctions with fascinating physical properties and promising applications in optoelectronics and valleytronics. Because of their…

Materials Science · Physics 2023-05-09 J. E. Zimmermann , M. Axt , F. Mooshammer , P. Nagler , C. Schüller , T. Korn , U. Höfer , G. Mette

We study carrier interaction induced many-body effects on the excitonic optical properties of highly photoexcited one-dimensional semiconductor quantum wire systems by solving the dynamically screened Bethe-Salpeter equation using realistic…

Strongly Correlated Electrons · Physics 2009-11-07 D. W. Wang , S. Das Sarma

Time-dependent density functional theory (TDDFT) has been applied to the calculation of absorption spectra for two-dimensional atomic layer materials. We reveal that the character of the first bright exciton state of bi-layer hexagonal…

Materials Science · Physics 2020-01-08 Yasumitsu Suzuki , Kazuyuki Watanabe

Two-dimensional (2D) heterostructures (HS) formed by transition-metal dichalcogenide (TMDC) monolayers offer a unique platform for the study of intralayer and interlayer excitons as well as moir\'e-pattern-induced features. Particularly,…

Mesoscale and Nanoscale Physics · Physics 2021-11-15 Mohammed Adel Aly , Manan Shah , Lorenz Maximilian Schneider , Kyungnam Kang , Martin Koch , Eui-Hyeok Yang , Arash Rahimi-Iman

We show both experimentally and theoretically that the recently observed optically induced in-plane charge separation in quantum well (QW) structures and the exciton ring emission pattern at this charge separation boundary have an extremely…

Other Condensed Matter · Physics 2009-11-10 Gang Chen , Ronen Rapaport , Steven H. Simon , Loren Pfeiffer , Ken West

We demonstrate that exciton conductance in organic materials can be enhanced by several orders of magnitude when the molecules are strongly coupled to an electromagnetic mode. Using a 1D model system, we show how the formation of a…

Mesoscale and Nanoscale Physics · Physics 2015-05-26 Johannes Feist , Francisco J. Garcia-Vidal

A new microscopic approach to the optical transitions in quantum dots and quantum dot molecules, which accounts for both diagonal and non-diagonal exciton-phonon interaction, is developed. The cumulant expansion of the linear polarization…

Other Condensed Matter · Physics 2015-06-25 E. A. Muljarov , T. Takagahara , R. Zimmermann

Starting from the many-body Bethe-Salpeter equation we derive an exchange-correlation kernel $f_{xc}$ that reproduces excitonic effects in bulk materials within time-dependent density functional theory. The resulting $f_{xc}$ accounts for…

Condensed Matter · Physics 2010-07-01 Lucia Reining , Valerio Olevano , Angel Rubio , Giovanni Onida

We use atomistic tight-binding theory with a configuration interaction description of Coulomb and exchange effects to describe excitons in symmetric quantum dots in a vertical electric field. We show that field-induced manipulation of…

Mesoscale and Nanoscale Physics · Physics 2012-12-20 Garnett W. Bryant , Natalia Malkova , James Sims

In an organic blend the vibrational normal mode excited by exciton splitting is the same as the one coupled to charge hopping. Excess driving force for exciton splitting can therefore aid charge transfer, if vibrational relaxation is slow…

Mesoscale and Nanoscale Physics · Physics 2010-04-05 James Kirkpatrick

We investigate the transport of dipolar indirect excitons along the growth plane of polar (Al,Ga)N/GaN quantum well structures by means of spatially- and time-resolved photoluminescence spectroscopy. The transport in these strongly…

Higher-order electronic transitions of all inorganic lead halide perovskite quantum dots (QDs) (CsPbX$_3$: X = Cl, Br, I) are hardly detected by traditional spectroscopic techniques due to the condensed electronic level of QDs. This work…

Materials Science · Physics 2023-11-22 Prasenjit Mandal , Ranjani Viswanatha

The dipole-dipole interactions between excitons are of paramount importance in the nanoscale structures. When two excitons are placed together they can exchange the energy can manifest in the resonant Raman cross sections. We provide…

Mesoscale and Nanoscale Physics · Physics 2024-04-09 Anna Wroblewska , Niclas S. Mueller , Mariusz Zdrojek , Stephanie Reich , Georgy Gordeev

Transition metal dichalcogenides (TMDCs) have demonstrated significant potential as versatile quantum materials for light absorption and emission. Their unique properties are primarily governed by exciton-photon interactions, which can be…