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Silver fulminate (AgCNO) is a primary explosive, which exists in two polymorphic phases namely orthorhombic (\emph{Cmcm}) and trigonal (\emph{R$\bar{3}$}) forms at ambient conditions. In the present study, we have investigated the effect of…

Materials Science · Physics 2015-06-22 N. Yedukondalu , G. Vaitheeswaran

Only several compounds bearing Ag(II) cation and other transition metal cation have been known. Herein, we predict stability and crystal structures of hypothetical ternary silver(II) fluorides with copper, nickel and cobalt in 1:1…

Materials Science · Physics 2021-07-29 Mateusz A. Domański , Mariana Derzsi , Wojciech Grochala

We present theoretical study of relative stability as well as of the magnetic and electronic properties of AgF2 and CuF2, in two related structural forms: orthorhombic (ambient pressure form of AgF2) and monoclinic (ambient pressure form of…

Materials Science · Physics 2024-03-28 Daniel Jezierski , Wojciech Grochala

Metal oxyfluorides constitute a broad group of chemical compounds with rich spectrum of crystal structures and properties. Here we predict, based on evolutionary algorithm approach, the crystal structure and selected properties of…

Materials Science · Physics 2021-05-28 Mateusz Domański , Wojciech Grochala

Silver chromate ($\mathrm{Ag_{2}CrO_{4}}$) has attracted considerable attention in recent years due to its promising photocatalytic performance, which strongly depends on the crystallographic orientation of its exposed surfaces. A detailed…

Materials Science · Physics 2026-05-20 Augusto Facundes , Thiago T. Dorini , Theodora W. von Zuben , Miguel A. San-Miguel

The silver-fluorine phase diagram has been scrutinized as a function of external pressure using theoretical methods. Our results indicate that two novel stoichiometries containing Ag+ and Ag2+ cations (Ag3F4 and Ag2F3) are thermodynamically…

Materials Science · Physics 2021-01-22 Dominik Kurzydłowski , Mariana Derzsi , Eva Zurek , Wojciech Grochala

Binary transition metal chalcogenides have attracted increasing attention for their unique structural and electronic properties. High pressure is powerful tool for tuning their crystal structure and electronic structure away from their…

Materials Science · Physics 2016-07-11 Zhao Zhao , Hua Wei , Wendy L. Mao

We investigate the high-pressure behaviour of beryllium, magnesium and calcium difluorides using ab initio random structure searching and density functional theory (DFT) calculations, over the pressure range 0-70 GPa. Beryllium fluoride…

Materials Science · Physics 2017-03-01 J. R. Nelson , R. J. Needs , C. J. Pickard

Sodium chloride (NaCl), or rocksalt, is well characterized at ambient pressure. Due to the large electronegativity difference between Na and Cl atoms, it has highly ionic chemical bonding, with stoichiometry 1:1 dictated by charge balance,…

Crystal and electronic structure, lattice dynamics and thermodynamic stability of little known mixed valent diamagnetic AgIAgIIIF4 beta form of AgF2 is thoroughly examined for the first time and compared with well known antiferromagnetic…

Materials Science · Physics 2021-01-06 Kamil Tokar , Mariana Derzsi , Wojciech Grochala

We use density functional theory (DFT) to study the thermodynamic stability and migration of copper ions and small clusters embedded in amorphous silicon dioxide. We perform the calculations over an ensemble of statistically independent…

Materials Science · Physics 2015-06-11 David M. Guzman , Nicolas Onofrio , Alejandro Strachan

The effects of pressure on the crystal structure of the three known polymorphs of magnesium sulfate have been theoretically study by means of DFT calculations up to 45 GPa. We determined that at ambient conditions gamma MgSO4 is an unstable…

Materials Science · Physics 2017-05-31 A. Benmakhlouf , D. Errandonea , M. Bouchenafa , S. Maabed , A. Bouhemadou , A. Bentabet

Studying the effect of high pressure (exceeding 10 kbar) on the structure of solids allows to gain deeper insight in the mechanism governing crystal structure stability. Here we report a study on the high-pressure behaviour of zinc…

Materials Science · Physics 2020-04-08 Dominik Kurzydłowski , Anna Oleksiak , Sharad Babu Pillai , Prafulla K. Jha

Solid hydrogen sulfide is well known as a typical molecular crystal but its stability under pressure is still under debate. Particularly, Eremets et al. found the high pressure superconductivity with $T_{c}\approx$ 190 K in a H$_{2}$S…

Superconductivity · Physics 2015-05-20 Defang Duan , Xiaoli Huang , Fubo Tian , Da Li , Hongyu , Yu , Yunxian Liu , Yanbin Ma , Bingbing Liu , Tian Cui

Group I/II materials exhibit unexpected structural phase transitions at high pressures, providing potential insight into the origins of elemental superconductivity. We present here a computational study of elemental barium and binary…

Materials Science · Physics 2012-07-16 Joshua A. Taillon , William W. Tipton , Richard G. Hennig

Based on theoretical calculations, we introduce a new AgIIAgIIIF5 monoclinic polymorph with a rare high spin AgIII. Our analysis of the experimental xray diffraction data available in the literature reveals that this polymorph was likely…

Materials Science · Physics 2025-10-16 Daniel Jezierski , Wojciech Grochala

Using the ab initio approaches, the comparative stability, structural, elastic, and electronic properties of three polymorphs of the superconducting disilicide YIr2Si2, which differ in the atomic configurations of [Ir2Si2] (or [Si2Ir2])…

Superconductivity · Physics 2015-05-28 Igor R. Shein

Silver iodide (AgI) is a prototypical superionic conductor, undergoing a first-order phase transition at 147 Celsius that enables rapid ionic transport through its lattice, making it attractive for solid-state ionic devices. However, due to…

Structures of calcium peroxide (CaO2) are investigated in the pressure range 0-200 GPa using the ab initio random structure searching (AIRSS) method and density functional theory (DFT) calculations. At 0 GPa, there are several CaO2…

Materials Science · Physics 2017-03-01 Joseph R. Nelson , Richard J. Needs , Chris J. Pickard

Compounds harboring active valence electrons, such as unconventional stoichiometric compounds of main group elements including sodium, chlorine, and carbon, have conventionally been perceived as unstable under ambient conditions, requiring…

Chemical Physics · Physics 2024-08-09 Liuhua Mu , Xuchang Su , Haiping Fang , Lei Zhang
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