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Controlling nanostructure from molecular, crystal lattice to the electrode level remains as arts in practice, where nucleation and growth of the crystals still require more fundamental understanding and precise control to shape the…

The role of Li-based batteries in the electrification of society cannot be understated, however their operational lifetime is often limited by the formation of dendrites, i.e. the localised deposition of Li that can cause shorts between the…

Conventional electrical circuits are generally rigid in their components and working styles which are not flexible and stretchable. From an alternative, liquid metal based soft electronics is offering important opportunities for innovating…

Applied Physics · Physics 2018-03-29 Yi Ren , Jing Liu

Liquid metal electrodes are one of the key components of different electrical energy storage technologies. The understanding of transport phenomena in liquid electrodes is mandatory in order to ensure efficient operation. In the present…

Fluid Dynamics · Physics 2021-04-02 Paolo Personnettaz , Steffen Landgraf , Michael Nimtz , Norbert Weber , Tom Weier

It is well known that the dielectric constant of two-dimensional (2D) electron system goes negative at low electron densities. A consequence of the negative dielectric constant could be the formation of the droplet state. The droplet state…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Junren Shi , Song He , X. C. Xie

Passivating lithium ion battery electrode surfaces to prevent electrolyte decomposition is critical for battery operations. Recent work on conformal atomic layer deposition (ALD) coating of anodes and cathodes has shown significant…

The properties of rechargeable lithium-ion batteries are determined by the electrochemical and kinetic properties of their constituent materials as well as by their underlying microstructure. Microstructural design can be leveraged to…

Materials Science · Physics 2022-03-11 Giovanna Bucci , Tushar Swamy , W. Craig Carter , Morad Behandish

Lithium (Li) metal anodes are essential for developing next-generation high-energy-density batteries. However, Li dendrite/whisker formation caused short-circuiting issue and short cycle life have prevented lithium metal from being viably…

Materials Science · Physics 2022-05-02 Bingyu Lu , Wurigumula Bao , Weiliang Yao , Jean-Marie Doux , Chengcheng Fang , Ying Shirley Meng

Nematic drops suspended in the isotropic phase of the same substance were subjected to alternating electrical fields of varying frequency. The system was carefully kept in the isotropic-nematic coexistance region, which was broadened due to…

Soft Condensed Matter · Physics 2009-03-27 Günter K. Auernhammer , Jinyu Zhao , Beate Ullrich , Doris Vollmer

The behavior of a microdrop of dielectric liquid suspended in a magnetic fluid and exposed to the action of electric and magnetic fields is studied experimentally. With increasing electric field, the deformation of droplets into oblate…

Soft Condensed Matter · Physics 2012-03-27 Arthur Zakinyan , Elena Tkacheva , Yury Dikansky

We perform phase-field simulations of the electrodeposition process that forms dendrites within metal-anode batteries including anisotropic representation. We describe the evolution of a phase field, the lithium-ion concentration, and an…

Describing Li-ion battery positive electrodes in terms of distinct transition metal or oxygen redox regimes can lead to confusion in understanding metal-ligand hybridisation, oxygen dimerisation, and degradation. There is a pressing need to…

Dendrite free electrodeposition of lithium metal is necessary for the adoption of high energy density rechargeable lithium metal batteries. Here, we demonstrate a new mechanism of using a liquid crystalline electrolyte to suppress dendrite…

Applied Physics · Physics 2020-10-29 Zeeshan Ahmad , Zijian Hong , Venkatasubramanian Viswanathan

The design and performance of liquid metal batteries, a new technology for grid-scale energy storage, depend on fluid mechanics because the battery electrodes and electrolytes are entirely liquid. Here we review prior and current research…

Fluid Dynamics · Physics 2017-10-10 Douglas H. Kelley , Tom Weier

We argue that there is a new liquid phase in the two-dimensional electron system in Si MOSFETs at low enough electron densities. The recently observed metal-insulator transition results as a crossover from the percolation transition of the…

Strongly Correlated Electrons · Physics 2009-10-30 Song He , X. C. Xie

Most next-generation Li-ion battery chemistries require a functioning lithium metal (Li) anode. However, its application in secondary batteries has been inhibited because of uncontrollable dendrite growth during cycling. Mechanical…

Materials Science · Physics 2017-01-11 Chen Xu , Zeeshan Ahmad , Asghar Aryanfar , Venkatasubramanian Viswanathan , Julia R. Greer

We study the formation and decay of electron-hole droplets in diamonds at both low and high temperatures under different excitations by master equations. The calculation reveals that at low temperature the kinetics of the system behaves as…

Materials Science · Physics 2007-05-23 J. H. Jiang , M. W. Wu , M. Nagai , M. Kuwata-Gonokami

A common, yet unmodelled experimental phenomenon is explained first through the experimental data and then through modelling efforts. The phenomenon is a large, temporary loss in voltage during constant current discharge. This effect can be…

Chemical Physics · Physics 2024-08-31 Michael Cornish , Monica Marinescu , Dharshannan Sugunan

The present study looks into the pinch-off dynamics of a compound droplet, which is suspended in another fluid in a parallel plate microchannel. The droplet is subjected to a transverse electric field in the presence of an imposed pressure…

Fluid Dynamics · Physics 2019-06-26 Somnath Santra , Sayan Das , Suman Chakraborty

All-solid-state batteries hold great promise for electric vehicle applications due to their enhanced safety and higher energy density. However, further performance optimization requires a deeper understanding of their degradation…

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