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Very recently we revealed a large family of triangular lattice quantum spin liquid candidates named rare-earth chalcogenides, which features a high-symmetry structure without structural/charge disorders and spin impurities, and may serve as…

CeCd$_3$P$_3$ and CeCd$_3$As$_3$ compounds adopt the hexagonal ScAl$_3$C$_3$-type structure, where magnetic Ce ions on a triangular lattice order antiferromagnetically below $T_\text{N} \sim$0.42~K. Their crystalline electric field (CEF)…

Strongly Correlated Electrons · Physics 2023-02-24 Obinna P. Uzoh , Suyoung Kim , Eundeok Mun

We apply moderate-high-energy inelastic neutron scattering (INS) measurements to investigate Yb$^{3+}$ crystalline electric field (CEF) levels in the triangular spin-liquid candidate YbMgGaO$_4$. Three CEF excitations from the ground-state…

Magnetocaloric effect (MCE) was investigated in the single crystal of CsGd(MoO$_4$)$_2$ in the temperature range from 2 to 30 K and fields up to 5 T applied along the easy and hard magnetic axis. The analysis of specific heat and…

Other Condensed Matter · Physics 2017-09-05 V. Tkáč , A. Orendáčová , R. Tarasenko , M. Orendáč , A. Feher

The rare earth intermetallic system \textit{R}Al\textit{X} (\textit{R} = rare earth elements, \textit{X} = Si and Ge) is known to be a promising candidate of magnetic Weyl semimetal. Due to the complex interactions between the rare earth…

After the discovery of the ARECh2 (A=alkali or monovalent ions, RE=rare-earth, Ch= chalcogen) triangular lattice quantum spin liquid (QSL) family, a series of its oxide, sulfide, and selenide counterparts has been consistently reported and…

Strongly Correlated Electrons · Physics 2024-08-20 Weiwei Liu , Zheng Zhang , Dayu Yan , Jianshu Li , Zhitao Zhang , Jianting Ji , Feng Jin , Youguo Shi , Qingming Zhang

The lack of the theory of the crystalline electric field (CEF) in rare-earth based quasicrystal (QC) and approximant crystal (AC) has prevented us from understanding the electronic states. Recent success of the formulation of the CEF theory…

Strongly Correlated Electrons · Physics 2023-07-24 Shinji Watanabe , Tatsuya Iwasaki

We have measured the crystalline electric field (CEF) excitations of the CeMIn5 (M = Co, Rh, Ir) series of heavy fermion superconductors by means of inelastic neutron scattering. Fits to a CEF model reproduce the inelastic neutron…

We have performed X-ray powder diffraction, magnetization, electrical resistivity, heat capacity and inelastic neutron scattering (INS) to investigate the physical properties of the intermetallic series of compounds CeCuBi$_{2-x}$Sb$_{x}$.…

We use inelastic neutron scattering to study the crystalline electric field (CEF) excitations of Ce$^{3+}$ in CeFeAsO$_{1-x}$F$_{x}$($x=0,0.16$). For nonsuperconducting CeFeAsO, the Ce CEF levels have three magnetic doublets in the…

The crystalline electric field (CEF) is investigated in Pr$_3$Pt$_{23}$Si$_{11}$ and Nd$_3$Pt$_{23}$Si$_{11}$ by neutron spectroscopy (NS). At low temperature, the number of observed CEF excitations is consistent with the orthorhombic…

Strongly Correlated Electrons · Physics 2016-12-13 R. M. Galéra , C. Opagiste , M. Amara , J. C. Toussaint , M. B. Lepetit , S. Rols

An indispensable step toward understanding magnetic interactions in rare-earth magnets is to determine the spatially anisotropic single-ion properties set by crystal electric field (CEF) physics. The CEF Hamiltonian yields a discrete energy…

Recently reported van der Waals layered honeycomb rare-earth chalcohalides REChX (RE = rare earth, Ch = chalcogen, and X = halogen) are considered to be promising Kitaev spin liquid (KSL) candidates. The high-quality single crystals of…

Strongly Correlated Electrons · Physics 2024-10-28 Yanzhen Cai , Wei Ren , Xijing Dai , Jing Kang , Weizhen Zhuo , Mingtai Xie , Anmin Zhang , Jianting Ji , Feng Jin , Zheng Zhang , Qingming Zhang

Alkali metal rare-earth chalcogenide $ARECh2$ (A=alkali or monovalent metal, RE=rare earth, Ch=O, S, Se, Te), is a large family of quantum spin liquid (QSL) candidates we discovered recently. Unlike $YbMgGaO4$, most members in the family…

Strongly Correlated Electrons · Physics 2021-05-26 Zheng Zhang , Jianshu Li , Weiwei Liu , Zhitao Zhang , Jianting Ji , Feng Jin , Rui Chen , Junfeng Wang , Xiaoqun Wang , Jie Ma , Qingming Zhang

The interplay of magnetic correlations, crystal electric field interactions, and spin-orbit coupling in low-dimensional frustrated magnets fosters novel ground states with unusual excitations. Here, we report the magnetic properties and…

Materials Science · Physics 2024-09-02 S. Guchhait , A. Painganoor , S. S. Islam , J. Sichelschmidt , M. D. Le , N. B. Christensen , R. Nath

We investigate the magnetic and crystal electric field (CEF) states of the Kondo lattice system CeCuGa3 by muon spin relaxation (muSR), neutron diffraction, and inelastic neutron scattering (INS) measurements. A noncentrosymmetric…

The crystalline electric field (CEF) of Ce3+ in trigonal symmetry has recently become of some relevance, for instance, in the search of frustrated magnetic systems. Fortunately, it is one of the CEF case in which a manageable analytic…

Strongly Correlated Electrons · Physics 2018-11-21 Jacintha Banda , Binod K. Rai , Helge Rosner , Emilia Morosan , Christoph Geibel , Manuel Brando

Low temperature optical spectroscopy in applied magnetic fields provides clear evidence of magnetoelastic coupling in the spin ice material Ho$_2$Ti$_2$O$_7$. In far-IR reflectometry measurements, we observe field dependent features around…

The crystalline electric field (CEF) energy level scheme of the heavy fermion superconductor CeCoIn_5 has been determined by means of inelastic neutron scattering (INS). Peaks observed in the INS spectra at 8 meV and 27 meV with incident…

The magnetic properties and crystal electric field (CEF) scheme of BiErGeO$_5$ are investigated via magnetization, heat capacity, muon spin relaxation (muSR), and inelastic neutron scattering (INS) experiments on a polycrystalline sample.…

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