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We experimentally demonstrate that a squeezed probe optical field can improve the sensitivity of the magnetic field measurements based on nonlinear magneto-optical rotation (NMOR) with an amplitude-modulated pump when compared to a coherent…

Quantum Physics · Physics 2023-07-19 Jiahui Li , Irina Novikova

Nuclear magnetic resonance (NMR) is a powerful method for determining the structure of molecules and proteins. While conventional NMR requires averaging over large ensembles, recent progress with single-spin quantum sensors has created the…

We present a new magnetometry method integrating an ensemble of nitrogen-vacancy (NV) centers in a single-crystal diamond with an extended dynamic range for monitoring the fast changing magnetic-field. The NV-center spin resonance frequency…

We develop an efficient package for the simulation of nuclear magnetic resonance spin echo experiments to study the effects of strong electronic spin correlations on the dynamics of the nuclear spin ensemble. A mean-field model is used to…

Strongly Correlated Electrons · Physics 2026-02-09 Charles Snider , Stephen Carr , D. E. Feldman , Chandrasekhar Ramanathan , V. F. Mitrović

In pulsed dynamic nuclear polarization (DNP), enhancement of the polarization of bulk nuclei requires the repeated application of a microwave pulse sequence. So far, analysis of a one-time transfer of electron spin polarization to a…

Chemical Physics · Physics 2025-07-24 Shebha Anandhi Jegadeesan , Yujie Zhao , Graham M. Smith , Ilya Kuprov , Guinevere Mathies

Precise control of the resonant frequency of a spin qubit is of fundamental importance to quantum sensing protocols. We demonstrate a control technique on a single nitrogen-vacancy (NV) centre in diamond where the applied magnetic field is…

We have developed a nuclear magnetic resonance spectrometer with a series tuned input circuit for measurements on samples at millikelvin temperatures based on an integrated two-stage superconducting quantum interference device current…

Superconductivity · Physics 2009-11-13 L. V. Levitin , R. G. Bennett , A. Casey , B. P. Cowan , C. P. Lusher , J. Saunders , D. Drung , Th. Schurig

Nuclear magnetic resonance (NMR) spectroscopy provides detailed information pertaining to dynamic processes through line-shape changes, which have been traditionally limited to equilibrium conditions. However, there is a wealth of…

Dynamic nuclear polarisation (DNP) refers to a class of techniques used to increase the signal in nuclear magnetic resonance measurements by transferring spin polarisation from ensembles of highly polarised electrons to target nuclear…

Quantum Physics · Physics 2020-12-24 L. T. Hall , D. A. Broadway , A. Stacey , D. A. Simpson , J-P. Tetienne , L. C. L. Hollenberg

Spin relaxometry with nitrogen-vacancy (NV) centers in diamond offers a spectrally selective, atomically localized, and calibrated measurement of microwave-frequency magnetic noise, presenting a versatile probe for condensed matter and…

Single-molecule nuclear magnetic resonance (NMR) is a crown-jewel challenge in the field of magnetic resonance spectroscopy and has important applications in chemical analysis and in quantum computing. Recently, it becomes possible to…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Fazhan Shi , Xi Kong , Pengfei Wang , Fei Kong , Nan Zhao , Ren-Bao Liu , Jiangfeng Du

Dynamic nuclear polarization (DNP) is a promising strategy for generating a significantly increased non-thermal spin polarization in nuclear magnetic resonance (NMR) applications thereby circumventing the need for strong magnetic fields.…

Quantum Physics · Physics 2015-07-15 Alexander Karabanov , Daniel Wisniewski , Igor Lesanovsky , Walter Köckenberger

While photoelectric detection of magnetic resonance (PDMR) can be applied to miniaturize nitrogen-vacancy (NV) center-based quantum sensors, real demonstration of PDMR-based magnetic field sensing remains as a distinctive challenge. To…

Quantum Physics · Physics 2026-02-13 Xuan-Ming Shen , Qilong Wu , Huihui Yu , Pei-Nan Ni , Qing Lou , Chao-Nan Lin , Xun Yang , Chong-Xin Shan , Yuan Zhang

We demonstrate a way to polarize and detect nuclear spin in a gate-defined quantum point contact operating at high Landau levels. Resistively-detected Nuclear Magnetic Resonance (RDNMR) can be achieved up to the $5$th Landau level and at a…

Mesoscale and Nanoscale Physics · Physics 2018-06-06 M. H. Fauzi , A. Noorhidayati , M. F. Sahdan , K. Sato , K. Nagase , Y. Hirayama

The active manipulation of nuclear spins with radio-frequency (RF) coils is at the heart of nuclear magnetic resonance (NMR) spectroscopy and spin-based quantum devices. Here, we present a microcoil transmitter system designed to generate…

Mesoscale and Nanoscale Physics · Physics 2021-03-10 K. Herb , J. Zopes , K. S. Cujia , C. L. Degen

We demonstrate time reversal of nuclear spin dynamics in highly magnetized dilute liquid 3He-4He mixtures through effective inversion of long-range dipolar interactions. These experiments, which involve using magic sandwich NMR pulse…

Other Condensed Matter · Physics 2007-10-10 Michael E. Hayden , Emmanuel Baudin , Geneviève Tastevin , Pierre-Jean Nacher

Nitrogen vacancy (NV) centers in diamond have been used as ultrasensitive magnetometers to perform nuclear magnetic resonance (NMR) spectroscopy of statistically polarized samples at 1 - 100 nm length scales. However, the spectral linewidth…

This paper proposes a high-precision time measurement method based on digital frequency-domain phase-fitting (DFPF) by using the digitized nuclear pulses. The averaging effect inherent in the frequency-domain cross-correlation and…

Instrumentation and Detectors · Physics 2025-04-17 Jianjun Wang , Zhaohui Bu , Zhao Wang , Jincheng Xu , Liguo Zhou , Qibin Zheng

Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…

The sensitivity of a practical quantum magnetometer is challenged by both inhomogeneous coupling between sensors and environment and errors in quantum control. Based on the physical criteria of modern quantum sensing, we present a robust…