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This paper presents a physics-based constitutive equation to predict the thermo-chemical aging in elastomers. High-temperature oxidation in elastomers is a complex phenomenon. The macromolecular network of elastomers' microstructures…

Materials Science · Physics 2021-04-20 Maryam Shakiba , Aimane Najmeddine

We propose a physics and chemistry-based constitutive framework to predict the stress responses of thermo-chemically aged elastomers and capture their brittle failure using the phase-field approach. High-temperature aging in the presence of…

Materials Science · Physics 2024-01-25 Aimane Najmeddine , Maryam Shakiba

A multiphasic constitutive model of the skin that implicitly accounts for the process of intrinsic (i.e.\ chronological) ageing via variation of the constitutive parameters is proposed. The structurally-motivated constitutive formulation…

Biological Physics · Physics 2018-01-18 D Pond , A McBride , L Davids , B D Reddy , G Limbert

We present a multiscale model bridging length and time scales from molecular to continuum levels with the objective of predicting the yield behavior of amorphous glassy polyethylene (PE). Constitutive parameters are obtained from molecular…

Computational Physics · Physics 2019-02-06 N. Vu-Bac , P. Areias , T. Rabczuk

This paper presents a micro-mechanical approach to describe the effects of thermo-oxidation on the constitutive behavior of aged elastomers at the long-range timescales. In particular, this model focuses on the effects of thermo-oxidative…

Soft Condensed Matter · Physics 2018-11-01 Hamid Mohammadi , Roozbeh Dargazany

A constitutive model is developed to predict the viscoelastic response of polyimide resins that are used in high temperature applications. This model is based on a thermodynamic framework that uses the notion that the `natural…

Numerical Analysis · Computer Science 2010-10-25 Satish Karra , K. R. Rajagopal

Ductile metals undergo a considerable amount of plastic deformation before failure. Void nucleation, growth and coalescence is the mechanism of failure in such metals. {\alpha}/{\beta} titanium alloys are ductile in nature and are widely…

Materials Science · Physics 2020-02-12 Umair Bin Asim , M Amir Siddiq , Robert M McMeeking , Mehmet E Kartal

Constitutive models play a crucial role in materials science as they describe the behavior of the materials in mathematical forms. Over the last few decades, the rapid development of manufacturing technologies have led to the discovery of…

Materials Science · Physics 2024-10-17 Xinxin Wu , Yin Zhang , Sheng Mao

It is known that the permittivity of the ferroelectric films is affected by several phenomena, which deteriorate the material quality (e.g. the redistribution of the crystal lattice defects, appearance of the electrode-adjacent…

Materials Science · Physics 2008-12-12 Pavel Mokry

Industrial polymeric materials often rely on antioxidants to achieve long-term reliability. Previous studies have frequently discussed the stabilization effect in the presence of macroscopic additive migration. However, the micro- to…

Soft Condensed Matter · Physics 2026-02-17 Takato Ishida , Emmanuel Richaud

In order to reveal the coupling effect among the chemical activity and the hydraulic seepage as well as the mechanical properties, a constitutive theoretical framework considering the chemical activity for saturated porous media is derived…

Soft Condensed Matter · Physics 2023-03-21 Ya-yuan Hu , Shu-hang Yuan

Multi-material 3D printing, particularly through polymer jetting, enables the fabrication of digital materials by mixing distinct photopolymers at the micron scale within a single build to create a composite with tunable mechanical…

Constitutive equations are developed for a polymer fluid, which is treated as a permanent network of strands bridged by junctions. The junctions are assumed to slide with respect to their reference positions under loading. Governing…

Materials Science · Physics 2007-05-23 A. D. Drozdov , R. K. Gupta

Solvent-based techniques usually involve preparing dilute blends of electron-donor and electron-acceptor materials dissolved in a volatile solvent. After some form of coating onto a substrate, the solvent evaporates. An initially…

Mesoscale and Nanoscale Physics · Physics 2012-03-01 Olga Wodo , Baskar Ganapathysubramanian

Predicting the process of porosity-based ductile damage in polycrystalline metallic materials is an essential practical topic. Ductile damage and its precursors are represented by extreme values in stress and material state quantities, the…

Materials Science · Physics 2023-08-09 Yinling Zhang , Nan Chen , Curt A. Bronkhorst , Hansohl Cho , Robert Argus

The recently developed evolutionary algorithm USPEX proved to be a tool that enables accurate and reliable prediction of structures for a given chemical composition. Here we extend this method to predict the crystal structure of polymers by…

Materials Science · Physics 2019-01-03 Qiang Zhu , Vinit Sharma , Artem R Oganov , Rampi Ramprasad

A thermodynamic framework has been developed for a class of amorphous polymers used in fused deposition modeling (FDM), in order to predict the residual stresses and the accompanying distortion of the geometry of the printed part (warping).…

Classical Physics · Physics 2021-02-09 P. Sreejith , K. Kannan , K. R. Rajagopal

We study the effect of physical aging on the mechanical properties of a model polymer glass using molecular dynamics simulations. The creep compliance is determined simultaneously with the structural relaxation under a constant uniaxial…

Soft Condensed Matter · Physics 2009-11-13 Mya Warren , Joerg Rottler

This article concludes a three-part series developing a self-consistent theoretical framework of the electromechanics of lipid membranes at the continuum scale. Owing to their small thickness, lipid membranes are commonly modeled as…

Soft Condensed Matter · Physics 2025-02-26 Yannick A. D. Omar , Zachary G. Lipel , Kranthi K. Mandadapu

We derive from particle-level dynamics a constitutive model describing the rheology of two-dimensional dense soft suspensions below the jamming transition, in a regime where hydrodynamic interactions between particles are screened. Based on…

Soft Condensed Matter · Physics 2026-01-08 N. Cuny , E. Bertin , R. Mari
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