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Related papers: Ultracold $^{88}\rm{Sr}_2$ molecules in the absolu…

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Using resonance-enhanced two-photon ionization, we detect ultracold, ground-state RbCs molecules formed via photoassociation in a laser-cooled mixture of 85Rb and 133Cs atoms. We obtain extensive bound-bound excitation spectra of these…

Atomic Physics · Physics 2009-11-10 Andrew J. Kerman , Jeremy M. Sage , Sunil Sainis , Thomas Bergeman , David DeMille

The study of the conversion of ultracold atoms into molecules has long remained a hot topic in atomic, molecular, and optical physics. However, most prior research has focused on diatomic molecules, with relatively scarce exploration of…

Quantum Gases · Physics 2026-01-21 Jia-Hui Zhang , Wen-Yuan Wang , Fu-Quan Dou

Ultracold LiCs molecules in the absolute ground state X$^1\Sigma^+$, v"=0, J"=0 are formed via a single photo-association step starting from laser-cooled atoms. The selective production of v"=0, J"=2 molecules with a 50-fold higher rate is…

Quantum Physics · Physics 2010-08-09 J. Deiglmayr , A. Grochola , M. Repp , K. Mörtlbauer , C. Glück , J. Lange , O. Dulieu , R. Wester , M. Weidemüller

In this work we model and realize stimulated Raman adiabatic passage (STIRAP) in the diatomic $\mathrm{^{23}Na^{40}K}$ molecule from weakly bound Feshbach molecules to the rovibronic ground state via the…

We report here on the production of an ultracold gas of tightly bound Rb2 molecules in the ro-vibrational triplet ground state, close to quantum degeneracy. This is achieved by optically transferring weakly bound Rb2 molecules to the…

Quantum Physics · Physics 2009-11-13 F. Lang , K. Winkler , C. Strauss , R. Grimm , J. Hecker Denschlag

One possibility for the creation of ultracold, high-phase-space-density quantum gases of molecules in the rovibrational ground state relies on first associating weakly-bound molecules from quantum-degenerate atomic gases on a Feshbach…

Using the technique of stimulated Raman adiabatic passage (STIRAP) we have coherently transferred ultracold 87Rb2 Feshbach molecules into a more deeply bound vibrational quantum level. Our measurements indicate a high transfer efficiency of…

Other Condensed Matter · Physics 2009-11-11 K. Winkler , F. Lang , G. Thalhammer , P. v. d. Straten , R. Grimm , J. Hecker Denschlag

We report the creation of a sample of over 1000 ultracold $^{87}$RbCs molecules in the lowest rovibrational ground state, from an atomic mixture of $^{87}$Rb and Cs, by magnetoassociation on an interspecies Feshbach resonance followed by…

We show that the interaction of polar alkali dimers in the quintet spin state leads to the formation of a deeply bound reaction complex. The reaction complex can decompose adiabatically into homonuclear alkali dimers (for all molecules…

Atomic Physics · Physics 2013-11-22 Michał Tomza , Kirk W. Madison , Robert Moszynski , Roman V. Krems

We report the comprehensive theoretical investigation of the Sr-SrOH system identifying it as a promising route to production of ultracold asymmetric top molecules. Combining high-level ab initio electronic structure calculations with…

Atomic Physics · Physics 2025-08-21 Maciej B. Kosicki , Mateusz Borkowski , Marcin Umiński , Piotr S. Żuchowski

We present spectra of ultracold $^7$Li$^{85}$Rb molecules in their electronic ground state formed by spontaneous decay of weakly bound photoassociated molecules. Beginning with atoms in a dual species magneto-optical trap (MOT), weakly…

Atomic Physics · Physics 2014-12-24 John Lorenz , Adeel Altaf , Sourav Dutta , Yong P. Chen , D. S. Elliott

We propose a method to suppress the chemical reactions between ultracold bosonic ground-state $^{23}$Na$^{87}$Rb molecules based on optical shielding. By applying a laser with a frequency blue-detuned from the transition between the lowest…

Quantum Gases · Physics 2020-10-14 T. Xie , M. Lepers , R. Vexiau , A. Orban , O. Dulieu , N. Bouloufa-Maafa

We produce an ultracold and dense sample of rovibronic ground state Cs_2 molecules close to the regime of quantum degeneracy, in a single hyperfine level, in the presence of an optical lattice. The molecules are individually trapped, in the…

We demonstrate single-shot imaging and narrow-line cooling of individual alkaline earth atoms in optical tweezers; specifically, strontium-88 atoms trapped in $515.2~\text{nm}$ light. We achieve high-fidelity single-atom-resolved imaging by…

The collision of molecules at ultracold temperatures is of great importance for understanding the chemical interactions at the quantum regime. While much theoretical work has been devoted to this, experimental data are only available…

Quantum Gases · Physics 2018-01-30 Xin Ye , Mingyang Guo , Maykel L. González-Martínez , Goulven Quéméner , Dajun Wang

Stimulated Raman Adiabatic Passage (STIRAP) and its variants, such as multi-state chainwise-STIRAP allow efficiently transferring the populations in multi-state system and have been widely used to prepare ultracold deeply-bound molecules.…

Quantum Physics · Physics 2024-07-30 Jiahui Zhang

We report the formation of ultracold $^{7}$Li$^{85}$Rb molecules in the $a^{3}\Sigma^{+}$ electronic state by photoassociation (PA) and their detection via resonantly enhanced multiphoton ionization (REMPI). With our dual-species Li and Rb…

Atomic Physics · Physics 2015-06-22 Adeel Altaf , Sourav Dutta , John Lorenz , Jesús Pérez-Ríos , Yong P. Chen , D. S. Elliott

The study of ultracold molecules tightly trapped in an optical lattice can expand the frontier of precision measurement and spectroscopy, and provide a deeper insight into molecular and fundamental physics. Here we create, probe, and image…

Atomic Physics · Physics 2015-12-22 B. H. McGuyer , M. McDonald , G. Z. Iwata , M. G. Tarallo , A. T. Grier , F. Apfelbeck , T. Zelevinsky

Neutral atoms trapped in the evanescent optical potentials of nanotapered optical fibers are a promising platform for developing quantum technologies and exploring fundamental science, such as quantum networks and quantum electrodynamics.…

We report on the direct conversion of laser-cooled 41K and 87Rb atoms into ultracold 41K87Rb molecules in the rovibrational ground state via photoassociation followed by stimulated Raman adiabatic passage. High-resolution spectroscopy based…

Atomic Physics · Physics 2015-05-19 K. Aikawa , D. Akamatsu , M. Hayashi , K. Oasa , J. Kobayashi , P. Naidon , T. Kishimoto , M. Ueda , S. Inouye