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Electrochemical energy systems rely on particulate porous electrodes to store or convert energies. While the three-dimensional porous structures were introduced to maximize the interfacial area for better overall performance of the system,…

Applied Physics · Physics 2021-02-16 Shubham Agrawal , Peng Bai

Understanding the dynamics of electric-double-layer (EDL) charging in porous media is essential for advancements in next-generation energy storage devices. Due to the high computational demands of direct numerical simulations and a lack of…

Chemical Physics · Physics 2023-09-04 Filipe Henrique , Pawel J. Zuk , Ankur Gupta

We generalize the compact group approach to conducting systems to give a self-consistent analytical solution to the problem of the effective quasistatic electrical conductivity of macroscopically homogeneous and isotropic dispersions of…

Statistical Mechanics · Physics 2019-11-05 M. Ya. Sushko , A. K. Semenov

Colloidal spheres with a partial platinum surface coating perform auto-phoretic motion when suspended in hydrogen peroxide solution. We present a theoretical analysis of the self-propulsion velocity of these particles using a continuum…

Soft Condensed Matter · Physics 2015-02-12 Joost de Graaf , Georg Rempfer , Christian Holm

The electrostatic screening of charge in one-dimensional confinement leads to long-range breakdown in electroneutrality within a nanopore. Through a series of continuum simulations, we demonstrate the principles of electroneutrality…

Soft Condensed Matter · Physics 2021-11-10 J. Pedro de Souza , Amir Levy , Martin Z. Bazant

Porous electrode theory, pioneered by John Newman and collaborators, provides a useful macroscopic description of battery cycling behavior, rooted in microscopic physical models rather than empirical circuit approximations. The theory…

Chemical Physics · Physics 2017-02-28 Raymond B. Smith , Martin Z. Bazant

Five parameters of a model of a polymer electrolyte membrane fuel cell cathode (the porosity of the gas diffusion layer, the porosity of the catalyst layer, the exchange current density of the oxygen reduction reaction, the effective ionic…

Materials Science · Physics 2013-08-22 Qingzhi Guo , Vijay A. Sethuraman , Ralph E. White

The results of the investigation of changes of parameters of dynamic bipolar charge-voltage and bipolar and unipolar dynamic current-voltage characteristics and transient currents connected with the pulse change of humidity for the samples…

Materials Science · Physics 2007-05-23 S. Bravina , N. Morozovsky , R. Boukroub

Electrowetting is a commonly used tool to manipulate sessile drops on hydrophobic surfaces. By applying an external voltage over a liquid and a dielectric-coated surface, one achieves a reduction of the macroscopic contact angles for…

Soft Condensed Matter · Physics 2019-07-05 Ranabir Dey , Mathijs van Gorcum , Frieder Mugele , Jacco H. Snoeijer

Under externally applied electric fields, lipid membranes tend to permeate and change their electrical resistance by the combined processes of pore creation and pore evolution (expansion or contraction). This study is focused on the pore…

Biological Physics · Physics 2008-12-03 Zlatko Vasilkoski

Battery electrode surfaces are generally coated with electronically insulating solid films of thickness 1-50 nm. Both electrons and Li+ can move at the electrode-surface film interface in response to the voltage, which adds complexity to…

Materials Science · Physics 2015-07-10 Kevin Leung , Andrew Leenheer

We study here the curious particle dynamics resulting from electro-osmotic flow around a microchannel junction corner whose dielectric walls are weakly polarizable. The hydrodynamic velocity field is obtained via superposition of a linear…

Fluid Dynamics · Physics 2015-06-19 Matan Zehavi , Gilad Yossifon

We calculate the thermophoretic drift of a charged single colloidal particle with hydrodynamically slipping surface immersed in an electrolyte solution in response to a small temperature gradient. Here, we rely on a linearized hydrodynamic…

Soft Condensed Matter · Physics 2023-04-26 Daniel B. Mayer , Dieter Braun , Thomas Franosch

Electrophoretic (EP) mobility reversal is commonly observed for strongly charged macromolecules in multivalent salt solutions. This curious effect takes place, e.g., when a charged polymer, such as DNA, adsorbs excess counterions so that…

Soft Condensed Matter · Physics 2023-03-28 Xiang Yang , Sahin Buyukdagli , Alberto Scacchi , Maria Sammalkorpi , Tapio Ala-Nissila

Due to evergrowing importance of understanding flow of bio-fluids in Lab-on-CD based systems, we investigate the flow behaviour of power-law fluids in the rotating electroosmotic flow through a polyelectrolyte grafted (soft) narrow channel.…

Fluid Dynamics · Physics 2019-12-20 Maneesh Patel , S S Harish Kruthiventi , P Kaushik

When an electric field is applied to an electrolyte-saturated polymer gel embedded with charged colloidal particles, the force that must be exerted by the hydrogel on each particle reflects a delicate balance of electrical, hydrodynamic and…

Soft Condensed Matter · Physics 2009-11-13 Reghan J. Hill , Martin Ostoja-Starzewski

Acid-induced release of stored ions from polyacrylic acid hydrogels (with a free surface fully permeable to the ion and acid flux) was observed to increase the gel osmotic pressure that leads to rapid, temporary swelling faster than the…

Soft Condensed Matter · Physics 2024-01-24 Chinmay Katke , Peter A. Korevaar , C. Nadir Kaplan

In the article we study a hyperbolic-elliptic system of PDE. The system can describe two different physical phenomena: 1st one is the motion of magnetic vortices in the II-type superconductor and 2nd one \ is the collective motion of cells.…

Analysis of PDEs · Mathematics 2024-09-26 N. V. Chemetov

We study conformational and electrophoretic properties of polyelectrolytes (PEs) in tetravalent salt solutions under the action of electric fields by means of molecular dynamics simulations. Chain conformations are found to have a sensitive…

Soft Condensed Matter · Physics 2011-08-26 Kun-Mao Wu , Yu-Fu Wei , Pai-Yi Hsiao

This paper extends the Lorentz-Abraham model of an electron (i.e. the equations of motion for a small spherical shell of charge, which is rigid in its proper frame) to treat a small spherically symmetric charge distribution, allowing for…

Classical Physics · Physics 2016-04-27 P. D. Flammer