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A strong electronic reconstruction resulting in a quenching of the Fe magnetic moments has recently been predicted to be at the origin of the giant magnetocaloric effect displayed by Fe2Pbased materials. To verify this scenario, X-ray…

Materials Science · Physics 2015-02-02 H. Yibole , F. Guillou , L. Caron , E. Jiménez , F. M. F. de Groot , P. Roy , R. de Groot , N. H. van Dijk , E. Brück

Using a combination of th local-density approximtion (LDA) and dynamicla mean-field theory (DMFT) calculations, we explore the correlated electronic structure of a member of the layered Iron oxychalcogenide Na_{2}Fe_{2}OSe_{2}. We find that…

Strongly Correlated Electrons · Physics 2013-07-08 Luis Craco , Mukul S. Laad , Stefano Leoni

Hard plane antiferromagnetic order where ordered moments lie perpendicular to the single-ion crystal electric field easy axis is rare in Ce-based Kondo lattices and is a subject of active interest. Here we show that Ce$_2$Rh$_3$Ge$_5$…

CaBaFe4O7 is a mixed-valent transition metal oxide having both Fe2+ and Fe3+ ions in tetrahedral coordination. Here we characterize its magnetic properties by magnetization measurements and investigate its local electronic structure using…

Strongly Correlated Electrons · Physics 2015-05-20 N. Hollmann , Z. Hu , Hua Wu , M. Valldor , N. Qureshi , T. Willers , Y. -Y. Chin , J. C. Cezar , A. Tanaka , N. B. Brookes , L. H. Tjeng

In the isostructural oxides Ca3CoMO6 (M = Co, Rh, Ir), the CoMO6 chains made up of face-sharing CoO6 trigonal prisms and MO6 octahedra are separated by Ca atoms. We analyzed the magnetic and electronic properties of these oxides on the…

Strongly Correlated Electrons · Physics 2011-01-05 Yuemei Zhang , Erjun Kan , Hongjun Xiang , Antoine Villesuzanne , Myung-Hwan Whangbo

SmCo5 is an important hard magnetic material, due to its large magnetic anisotropy energy (MAE). We have studied the magnetic properties of SmCo5 using density functional theory (DFT) calculations where the Sm f-bands, which are difficult…

Materials Science · Physics 2009-11-10 P. Larson , I. I. Mazin , D. A. Papaconstantopoulos

Electronic structure and magnetic properties for iron deficient TlFe$_{2-x}$Se$_2$ compounds are studied by first-principles calculations. We find that for the case of $x=0.5$ with a Fe-vacancy ordered orthorhombic superstructure, the…

Superconductivity · Physics 2011-05-23 Chao Cao , Jianhui Dai

The iron arsenide Sr2CrO3FeAs with the tetragonal Sr2GaO3CuS-type structure was synthesized and its crystal structure re-determined by neutron powder diffraction. In contrast to previous X-ray crystallographic studies, a mixed occupancy of…

Superconductivity · Physics 2010-02-24 Marcus Tegel , Franziska Hummel , Yixi Su , Tapan Chatterji , Michela Brunelli , Dirk Johrendt

We expand our study on cubic BiFeO$_3$ alloys presented in [K. Koumpouras and I. Galanakis, \textit{J. Magn. Magn. Mater} 323, 2328 (2011)] to include also the BiMnO$_3$ and Bi$_2$MnFeO$_6$ alloys. For the latter we considered three…

Materials Science · Physics 2012-04-23 K. Koumpouras , I. Galanakis

Iron, cobalt and nickel are archetypal ferromagnetic metals. In bulk, electronic conduction in these materials takes place mainly through the $s$ and $p$ electrons, whereas the magnetic moments are mostly in the narrow $d$-electron bands,…

Strongly Correlated Electrons · Physics 2009-06-18 M. R. Calvo , J. Fernández-Rossier , J. J. Palacios , D. Jacob , D. Natelson , C. Untiedt

A new mechanism of the Verway transition in magnetite (Fe3O4), which has been argued to be a charge ordering transition so far, is proposed. Based on the mean field calculations for the three band model of spinless fermions appropriate for…

Strongly Correlated Electrons · Physics 2007-05-23 Hitoshi Seo , Masao Ogata , Hidetoshi Fukuyama

Magnetism in transition metal compounds is usually considered starting from a description of isolated ions, as exact as possible, and treating their (exchange) interaction at a later stage. We show that this standard approach may break down…

Strongly Correlated Electrons · Physics 2016-10-24 S. V. Streltsov , D. I. Khomskii

Recently, the mixed transition metal oxides of the form Li(Ni1-y-zCoyMnz)O2, have become the center of attention as promising candidates for novel battery material. These materials have also revealed very interesting magnetic properties due…

Strongly Correlated Electrons · Physics 2013-07-30 J. Magnus Wikberg , Martin Mansson , Mohammed Dahbi , Kazuya Kamazawa , Jun Sugiyama

Among the numerous 2D system that can be prepared via exfoliation, iron phosphorus trisulfide (FePS3) attracts a lot of attention recently due to its broad-range photoresponse, its unusual Ising-type magnetic order and possible applications…

Materials Science · Physics 2023-01-16 Mohammad Amirabbasi , Peter Kratzer

In this paper we present an analysis of the magnetic toroidal moment and its relation to the various structural modes in R3c-distorted perovskites with magnetic cations on either the perovskite A or B site. We evaluate the toroidal moment…

Materials Science · Physics 2015-05-13 Claude Ederer

Room-temperature ferrimagnetism was discovered for the anti-site-disordered perovskite Ca2MnOsO6 with Tc = 305 K. Ca2MnOsO6 crystallizes into an orthorhombic structure with a space group of Pnma, in which Mn and Os share the…

Some Bravais lattices have a particular geometry that can slow down the motion of Bloch electrons by pre-localization due to the band-structure properties. Another known source of electronic localization in solids is the Coulomb repulsion…

Strongly Correlated Electrons · Physics 2017-07-13 A. Hausoel , M. Karolak , E. Sasioglu , A. Lichtenstein , K. Held , A. Katanin , A. Toschi , G. Sangiovanni

We present here an investigation of the magnetic ordering in the Mott insulating oxyselenide materials Ln2O2Fe2OSe2 (Ln = Ce, Nd). Neutron powder diffraction data are consistent with a non-collinear multi-k ordering on the iron sublattice…

Strongly Correlated Electrons · Physics 2014-10-21 Emma E. McCabe , Andrew S. Wills , Laurent Chapon , Pascal Manuel , John S. O. Evans

The recent discovery of superconductivity at high pressure in the two-leg ladder compounds BaFe$_2X_3$ ($X$=S, Se) started the novel field of quasi-one-dimensional iron-based superconductors. In this publication, we use Density Functional…

Strongly Correlated Electrons · Physics 2019-12-04 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Shuai Dong , Elbio Dagotto

High-pressure diamond anvil cells have been widely used to create novel states of matter. Nevertheless, the lack of universal in-situ magnetic measurement techniques at megabar pressures makes it difficult to understand the underlying…

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