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We report a joint experimental and theoretical study of a three-sideband (3-SB) modification of the "reconstruction of attosecond beating by interference of two-photon transitions" (RABBIT) setup. The 3-SB RABBIT scheme makes it possible to…

Atomic Physics · Physics 2023-01-24 D Bharti , H Srinivas , F Shobeiry , K R Hamilton , R Moshammer , T Pfeifer , K Bartschat , A Harth

Measured photoionization time delays may exhibit large variations as a function of the emission angles, even for spherically symmetric targets, as shown in recent RABBITT (reconstruction of attosecond beating by interference of two-photon…

Atomic Physics · Physics 2022-12-29 D. I. R. Boll , L. Martini , A. Palacios , O. A. Fojón

Based on the frequency-domain theory, we investigate the above-threshold ionization (ATI) process of an atom in a two-color laser field with infrared (IR) and extreme ultraviolet (XUV) frequencies, where the photon energy of the XUV laser…

Atomic Physics · Physics 2015-06-16 Kui Zhang , Jing Chen , Panming Fu , Zong-Chao Yan , Bingbing Wang

Using the frequency-domain theory, the high-order above threshold ionization (HATI) of a molecule is treated as a two-step transition: an above threshold ionization (ATI) followed by a laser-assisted collision (LAC). It is found that the…

Atomic Physics · Physics 2009-05-28 Bingbing Wang , Yingchun Guo , Zong-Chao Yan , Panming Fu

We report new techniques for driving high-fidelity stimulated Raman transitions in trapped ion qubits. An electro-optic modulator induces sidebands on an optical source, and interference between the sidebands allows coherent Rabi…

In this work, we study the resonant tunneling (RT) of electrons and H atoms in double-barrier (DB) systems. Our numerical calculations directly verify the correspondence between the resonant tunneling energies and the energy levels of…

Mesoscale and Nanoscale Physics · Physics 2024-11-14 Wei Li , Yong Yang

The two basic approaches underlying the metrology of attosecond pulse trains are compared, i.e. the 2nd order Intensity Volume Autocorrelation and the Resolution of Attosecond Beating by Interference of Two photon Transitions (RABITT). They…

We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…

Atomic Physics · Physics 2022-05-03 Jakub Benda , Zdeněk Mašín , Jimena D. Gorfinkiel

The performance of direct-drive inertial confinement fusion implosions relies critically on the coupling of laser energy to the target plasma. Cross-beam energy transfer (CBET), the resonant exchange of energy between intersecting laser…

We study theoretically the reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) in strongly polar molecules. The time-dependent energy of a polar molecule in the infrared (IR) field gives rise to an…

Atomic Physics · Physics 2024-01-30 Jakub Benda , Zdeněk Mašín

Above-threshold ionization (ATI) results from strong field laser-matter interaction and it is one of the fundamental processes that may be used to extract electron structural and dynamical information about the atomic or molecular target.…

Atomic Physics · Physics 2016-01-06 Noslen Suárez , Alexis Chacón , Marcelo Ciappina , Jens Biegert , Maciej Lewenstein

We investigate laser-driven vibronic transitions of a single two-level atomic ion in harmonic and hard wall traps. In the Lamb-Dicke regime, for tuned or detuned lasers with respect to the internal frequency of the ion, and weak or strong…

Quantum Physics · Physics 2009-11-13 I. Lizuain , J. G. Muga

We theoretically explore a variant of RABBITT spectroscopy in which the attosecond-pulse train comprises isolated pairs of consecutive harmonics of the fundamental infrared probe frequency. In this scheme, one-photon and two-photon…

Atomic Physics · Physics 2019-05-15 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

Parity mixing in photoionization, i.e. when emitted electrons have different parities but the same energy, causes interference observable only in angle-resolved measurements. The interference typically manifests as a symmetry violation in…

Atomic Physics · Physics 2026-04-20 Maria M. Popova , Sergei N. Yudin , Alexei N. Grum-Grzhimailo , Elena V. Gryzlova

Photoexcitation of trapped ions by Hermite-Gaussian (HG) modes from guided beam structures is proposed and investigated theoretically. In particular, simple analytical expressions for the Rabi frequencies of induced atomic transitions are…

We present results of high-resolution experiments on single ionization of He, Ne and Ar by ultra-short (25 fs, 6 fs) 795 nm laser pulses at intensities 0.15-2.0x10^15 W/cm^2. We show that the ATI-like pattern can survive deep in the…

Atomic Physics · Physics 2009-11-10 A. Rudenko , K. Zrost , C. D. Schröter , V. L. B. de Jesus , B. Feuerstein , R. Moshammer , J. Ullrich

Resonant Raman excitation by ultrafast vacuum ultraviolet laser pulses is a powerful means to study electron dynamics in molecules, but experiments must contend with linear background ionization: frequencies high enough to reach resonant…

Chemical Physics · Physics 2015-06-23 S. Miyabe , P. Bucksbaum

We study the absorption and dispersion properties of a weak tunable probe field in a four-level Y-type atomic system driven by two strong laser (coupling) fields within the framework of density matrix formalism. It is found that the probe…

Atomic Physics · Physics 2014-03-12 L. Safari , D. Iablonskyi , F. Fratini

Attosecond measurements reveal new physical insights in photo ionization dynamics from atoms, molecules and condensed matter. However, on such time scales even small timing jitter can significantly reduce the time resolution in pump-probe…

Optics · Physics 2020-05-20 Constantin Krüger , Jaco Fuchs , Laura Cattaneo , Ursula Keller