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Time-of-flight neutron spectroscopy has been used to determine the crystalline electric field (CEF) Hamiltonian, eigenvalues and eigenvectors appropriate to the $J$ = 7/2 Yb$^{3+}$ ion in the candidate quantum spin ice pyrochlore magnet…

Strongly Correlated Electrons · Physics 2016-03-09 J. Gaudet , D. D. Maharaj , G. Sala , E. Kermarrec , K. A. Ross , H. A. Dabkowska , A. I. Kolesnikov , G. E. Granroth , B. D. Gaulin

We introduce PyCrystalField, a Python software package for calculating single-ion crystal electric field (CEF) Hamiltonians. This software can calculate a CEF Hamiltonian \textit{ab initio} from a point charge model for any transition or…

Strongly Correlated Electrons · Physics 2021-01-19 Allen Scheie

The crystalline electric field (CEF) is investigated in Pr$_3$Pt$_{23}$Si$_{11}$ and Nd$_3$Pt$_{23}$Si$_{11}$ by neutron spectroscopy (NS). At low temperature, the number of observed CEF excitations is consistent with the orthorhombic…

Strongly Correlated Electrons · Physics 2016-12-13 R. M. Galéra , C. Opagiste , M. Amara , J. C. Toussaint , M. B. Lepetit , S. Rols

Low-resolution nuclear Hamiltonians, obtained from chiral effective field theory (EFT) and softened using renormalization group techniques, have been very successful in nuclear structure theory. The associated EFT truncation uncertainty for…

Nuclear Theory · Physics 2025-09-30 Tom Plies , Matthias Heinz , Achim Schwenk

On the basis of the point charge model, we formulate the crystalline electronic field (CEF) Hamiltonian $H_{\rm CEF}$ in the rare-earth based quasicrystal (QC) and approximant crystal (AC) with ligand ions located at pseudo 5-fold…

Strongly Correlated Electrons · Physics 2022-03-22 Shinji Watanabe , Mina Kawamoto

We study the correlated quantum magnet, YbCl$_3$, with neutron scattering, magnetic susceptibility, and heat capacity measurements. The crystal field Hamiltonian is determined through simultaneous refinements of the inelastic neutron…

We use neutron scattering and bulk property measurements to determine the single-ion crystal-field Hamiltonians of delafossites $\rm KErSe_2$ and $\rm CsErSe_2$. These two systems contains planar equilateral triangular Er lattices arranged…

Strongly Correlated Electrons · Physics 2020-04-29 A. Scheie , V. O. Garlea , L. D. Sanjeewa , J. Xing , A. S. Sefat

We report the synthesis of powder and single-crystal samples of the cerium pyrohafnate and their characterization using neutron diffraction, thermogravimetry and X-ray absorption spectroscopy. We evaluate the amount of non-magnetic…

The Crystalline Electric Field (CEF) influence is usually described by considering an ideally symmetrical rare-earth site. In the case of cage compounds, ample excursions of the rare-earth inside the cage require an adapted CEF description.…

Strongly Correlated Electrons · Physics 2019-05-15 Mehdi Amara

We investigate the crystal electric field (CEF) excitations of Yb$^{3+}$ ions in powder samples of the triangular-lattice rare-earth-based antiferromagnet YbZn$_2$GaO$_5$ using inelastic neutron scattering (INS). Three CEF excitations from…

Strongly Correlated Electrons · Physics 2025-07-18 Leshan Zhao , Tong Chen , Matthew B. Stone , Qiang Zhang , Colin L. Sarkis , S. M. Koohpayeh , Collin Broholm

Inelastic neutron scattering experiments were performed to investigate the crystalline electric field (CEF) excitations of Nd3+ (J = 9/2) in the iron pnictide NdFeAsO. The crystal field level structures for both the high-temperature…

Superconductivity · Physics 2014-01-08 Y. Xiao , M. Zbiri , R. A. Downie , J. -W. G. Bos , Th. Brueckel , T. Chatterji

Although uncertainty quantification has been making its way into nuclear theory, these methods have yet to be explored in the context of reaction theory. For example, it is well known that different parameterizations of the optical…

Nuclear Theory · Physics 2017-03-01 A. E. Lovell , F. M. Nunes , J. Sarich , S. M. Wild

The standard model coherent elastic neutrino-nucleus scattering (CE$\nu$NS) cross section is subject to nuclear form factor uncertainties, mainly driven by the root-mean-square radius of the neutron density distribution. Motivated by…

High Energy Physics - Phenomenology · Physics 2019-07-02 D. Aristizabal Sierra , Jiajun Liao , D. Marfatia

The pyrochlore magnet $\rm Yb_2Ti_2O_7$ has been proposed as a quantum spin ice candidate, a spin liquid state expected to display emergent quantum electrodynamics with gauge photons among its elementary excitations. However, $\rm…

Strongly Correlated Electrons · Physics 2018-06-20 Gabriele Sala , Dalini D. Maharaj , Matthew B. Stone , Hanna A. Dabkowska , Bruce D. Gaulin

We present bulk and neutron scattering measurements performed on the isotopically enriched $^{154}\mathrm{Sm_2Ti_2O_7}$ and $^{154}\mathrm{Sm_2Sn_2O_7}$ samples. Both compounds display sharp heat capacity anomalies, at 350 mK and 440 mK,…

I review some central physics opportunities at the 15 ... 30 GeV continuous beam electron accelerator ELFE, proposed to be built in conjunction with the DESY linear collider. Our present detailed knowledge of single parton distributions in…

High Energy Physics - Phenomenology · Physics 2008-11-26 Paul Hoyer

The delafossite family of compounds with a triangular lattice of rare earth ions has been recently proposed as a candidate host for quantum spin liquid (QSL) states. To realize QSLs, the crystal-electric-field (CEF) ground state of the rare…

Strongly Correlated Electrons · Physics 2020-07-20 Shang Gao , Fan Xiao , Kazuya Kamazawa , Kazuhiko Ikeuchi , Daniel Biner , Karl Krämer , Christian Rüegg , Taka-hisa Arima

Computational crystal-field models have provided consistent models of both electronic and Zeeman-hyperfine structure for several rare earth ions. These techniques have not yet been applied to the Zeeman-hyperfine structure of Eu$^{3+}$…

Materials Science · Physics 2022-04-13 Kieran M. Smith , Michael F. Reid , Matthew J. Sellars , Rose L. Ahlefeldt

Central quantities in spectroscopy and magnetism of transition ions in crystals are crystal field parameters (CFPs). Nature self-imposed limits on orthorhombic and lower symmetry CFPs, and existence of intrinsically incomparable CFP sets…

Materials Science · Physics 2009-06-03 C. Rudowicz , P. Gnutek

The application of effective field theory (EFT) methods to nuclear systems provides the opportunity to rigorously estimate the uncertainties originating in the nuclear Hamiltonian. Yet this is just one source of uncertainty in the…

Nuclear Theory · Physics 2016-05-13 R. J. Furnstahl , D. R. Phillips , S. Wesolowski
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