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Dynamic nuclear polarisation, which transfers the spin polarisation of electrons to nuclei, is routinely applied to enhance the sensitivity of nuclear magnetic resonance; it is also critical in spintronics, particularly when spin…

We investigate the coherence properties of individual nuclear spin quantum bits in diamond [Dutt et al., Science, 316, 1312 (2007)] when a proximal electronic spin associated with a nitrogen-vacancy (NV) center is being interrogated by…

A controlled qubit in a rotating frame opens new opportunities to probe fundamental quantum physics, such as geometric phases in physically rotating frames, and can potentially enhance detection of magnetic fields. Realising a single qubit…

The nitrogen-vacancy (NV) centre, as a promising candidate solid state system of quantum information processing, its electron spin coherence is influenced by the magnetic field fluctuations due to the local environment. In pure diamonds,…

Mesoscale and Nanoscale Physics · Physics 2011-04-08 Nan Zhao , Jian-Liang Hu , Sai-Wah Ho , Tsz-Kai Wen , R. B. Liu

Isolated nuclear spins offer a promising building block for quantum information processing systems, but their weak interactions often impede preparation, control, and detection. Hyperfine coupling to a proximal electronic spin can enhance…

Quantum Physics · Physics 2013-05-29 Benjamin Smeltzer , Jean McIntyre , Lilian Childress

Coherent control and optical readout of the electron spin of the $^{29}$SiV$^{-}$ center in diamond has been demonstrated in literature, with exciting prospects for implementations as memory nodes and spin qubits. Nuclear spins may be even…

Quantum Physics · Physics 2022-06-15 Hyma H. Vallabhapurapu , Chris Adambukulam , Andre Saraiva , Arne Laucht

Precise coherent control of the individual electronic spins associated with atom-like impurities in the solid state is essential for applications in quantum information processing and quantum metrology. We demonstrate all-optical…

Quantum Physics · Physics 2015-03-05 Yiwen Chu , Matthew Markham , Daniel J. Twitchen , Mikhail D. Lukin

We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify…

Mesoscale and Nanoscale Physics · Physics 2012-10-23 T. H. Taminiau , J. J. T. Wagenaar , T. van der Sar , F. Jelezko , V. V. Dobrovitski , R. Hanson

Spin degrees of freedom of charged nitrogen-vacancy (NV$^-$) centers in diamond have large decoherence times even at room temperature, can be initialized and read out using optical fields, and are therefore a promising candidate for solid…

Other Condensed Matter · Physics 2009-11-13 A. M. Zagoskin , J. R. Johansson , S. Ashhab , Franco Nori

Nitrogen-Vacancy (NV) centers in diamonds provide a room-temperature platform for various emerging quantum technologies, e.g. the long nuclear spin coherence times as potential quantum memory registers. We demonstrate a freezing protocol…

Quantum Physics · Physics 2023-08-14 Abhishek Kejriwal , Dasika Shishir , Sumiran Pujari , Kasturi Saha

We experimentally demonstrate high degree of polarization of 13C nuclear spins weakly interacting with nitrogen-vacancy (NV) centers in diamond. We combine coherent microwave excitation pulses with optical illumination to provide controlled…

Quantum Physics · Physics 2019-10-25 Jiwon Yun , Kiho Kim , Dohun Kim

Nuclear spins in solids exhibit long coherence times due to the small nuclear gyromagnetic ratio. This weak environmental coupling comes at the expense of slow quantum gate operations, which should be as fast as possible for many…

Quantum Physics · Physics 2022-11-11 R. M. Goldblatt , A. M. Martin , A. A. Wood

Coherent coupling between single quantum objects is at the heart of modern quantum physics. When coupling is strong enough to prevail over decoherence, it can be used for the engineering of correlated quantum states. Especially for…

Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…

Nitrogen vacancy (NV) centers, optically-active atomic defects in diamond, have attracted tremendous interest for quantum sensing, network, and computing applications due to their excellent quantum coherence and remarkable versatility in a…

Nuclear spins in the proximity of electronic spin defects in solids are promising platforms for quantum information processing due to their ability to preserve quantum states for a remarkably long time. Here we report a comprehensive study…

Quantum Physics · Physics 2023-10-03 Mykyta Onizhuk , Giulia Galli

An obstacle for spin-based quantum sensors is magnetic noise due to proximal spins. However, such a spin cluster surrounding the sensor can become an asset, if it can be controlled. Here, we polarize and readout a cluster of three nitrogen…

Quantum Physics · Physics 2016-09-07 Helena S. Knowles , Dhiren M. Kara , Mete Atatüre

Nuclear magnetic resonance (NMR) is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities -…

Coupled electron-nuclear spins represent a promising quantum system, where the optically induced electron spin polarization can be dynamically transferred to nuclear spins via the hyperfine interaction. Most experiments on dynamic nuclear…

Materials Science · Physics 2026-01-13 A. N. Anisimov , A. V. Poshakinskiy , G. V. Astakhov

A promising approach for multi-qubit quantum registers is to use optically addressable spins to control multiple dark electron-spin defects in the environment. While recent experiments have observed signatures of coherent interactions with…

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