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In this communication we study the transport properties of two-dimensional assemblies of [Fe(Htrz)2(trz)](BF4) spin-crossover nanoparticles (NPs) with two different morphologies. The NPs have been synthesized made in a similar manner than…

Recent years have shown steady progress in research towards molecular electronics [1,2], where molecules have been investigated as switches [3-5], diodes [6], and electronic mixers [7]. In much of the previous work a Scanning Tunnelling…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 R. H. M. Smit , Y. Noat , C. Untiedt , N. D. Lang , M. van Hemert , J. M. van Ruitenbeek

We investigate nonequilibrium phenomena in magnetic nano-junctions using a numerical approach that combines classical spin dynamics with the hierarchical equations of motion technique for quantum dynamics of conduction electrons. Our focus…

Mesoscale and Nanoscale Physics · Physics 2024-02-26 Rudolf Smorka , Michael Thoss , Martin Žonda

We investigate electron transport through a mixed-valence molecular complex in which an excess electron can tunnel between hetero-valent transition metal ions, each having a fixed localized spin. We show that in this class of molecules the…

Mesoscale and Nanoscale Physics · Physics 2009-03-11 F. Reckermann , M. Leijnse , M. R. Wegewijs

In spin crossover materials, an abrupt phase transition between a low spin state and a high spin state can be driven by temperature, pressure or by light irradiation. Of a special relevance are Fe(II) based coordination polymers where, in…

Formation of a magnetic hysteresis loop with respect to a bias voltage is investigated theoretically in a spin-valve device based on a single magnetic molecule. We consider a device consisting of two ferromagnetic electrodes bridged by a…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 Anna Płomińska , Maciej Misiorny , Ireneusz Weymann

We theoretically study the crossover between spin Hall effect and spin swapping, a recently predicted phenomenon that consists in the interchange between the current flow and its spin polarization directions [Lifshits and Dyakonov, Phys.…

Mesoscale and Nanoscale Physics · Physics 2015-05-15 Hamed Ben Mohamed Saidaoui , Y. Otani , A. Manchon

We investigate the spin of a multielectron GaAs quantum dot in a sequence of nine charge occupancies, by exchange coupling the multielectron dot to a neighboring two-electron double quantum dot. For all nine occupancies, we make use of a…

Molecular platforms are regarded as promising candidates in the generation of units of information for quantum computing. Herein, a strategy combining spin-crossover metal ions and radical ligands is proposed from a model Hamiltonian first…

Quantum Physics · Physics 2022-12-07 Roseiro Pablo , Petit Louis , Robert Vincent , Yalouz Saad

A model describing spin-polarized current via discrete energy levels of a metallic nanoparticle, which has strongly asymmetric tunnel contacts to two ferromagnetic leads, is presented. In absence of spin-relaxation, the model leads to a…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Y. G. Wei , C. E. Malec , D. Davidović

We present a protocol that detects molecular conformational changes with two nitroxide electron-spin labels and a nitrogen-vacancy (NV) center in diamond. More specifically, we demonstrate that the NV can detect energy shifts induced by the…

Quantum Physics · Physics 2022-12-21 C. Munuera-Javaloy , R. Puebla , B. D'Anjou , M. B. Plenio , J. Casanova

The ability to control and understand the phase transitions of individual nanoscale building blocks is key to advancing the next generation of low-power reconfigurable nanophotonic devices. To address this critical challenge, molecular…

We investigate gold-4,4'-bipyridine-gold single-molecule junctions with the mechanically controllable break junction technique at cryogenic temperature ($T=4.2\,\text{K}$). We observe bistable probabilistic conductance switching between the…

Mesoscale and Nanoscale Physics · Physics 2020-09-15 Gréta Mezei , Zoltán Balogh , András Magyarkuti , András Halbritter

Pulsed spin-torque switching has been studied using single-shot time-resolved electrical measurements in perpendicularly magnetized magnetic tunnel junctions as a function of pulse amplitude and junction size in 50 to 100 nm diameter…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Christian Hahn , Georg Wolf , Bartek Kardasz , Steve Watts , Mustafa Pinarbasi , Andrew D. Kent

We investigated the time dependence of two-electron spin states in a double quantum dot fabricated in an InAs nanowire. In this system, spin-orbit interaction has substantial influence on the spin states of confined electrons. Pumping…

Mesoscale and Nanoscale Physics · Physics 2009-04-30 A. Pfund , I. Shorubalko , K. Ensslin , R. Leturcq

Coherent spin resonance methods, such as nuclear magnetic resonance and electron spin resonance spectroscopy, have led to spectrally highly sensitive, non-invasive quantum imaging techniques. Here, we propose a pump-probe spin resonance…

Quantum Physics · Physics 2024-12-02 Philipp Haslinger , Stefan Nimmrichter , Dennis Rätzel

Long spin relaxation times are a prerequisite for the use of spins in data storage or nanospintronics technologies. An atomic-scale solid-state realization of such a system is the spin of a transition metal atom adsorbed on a suitable…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 Jan Hermenau , Markus Ternes , Manuel Steinbrecher , Roland Wiesendanger , Jens Wiebe

We determine the spin exchange coupling J between two electrons located in two vertically tunnel-coupled quantum dots, and its variation when magnetic (B) and electric (E) fields (both in-plane and perpendicular) are applied. We predict a…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 Guido Burkard , Georg Seelig , Daniel Loss

The $2d$ Hubbard model with nearest-neighbour hopping on the square lattice and an average of one electron per site is known to undergo an extended crossover from metallic to insulating behavior driven by proliferating antiferromagnetic…

Strongly Correlated Electrons · Physics 2020-03-19 Aaram J. Kim , Fedor Simkovic , Evgeny Kozik

We investigate the dependence of switching current density on the junction sizes in the spin transfer torque nanopillar structures by using micromagnetic simulations. While the macro spin model predicts weak dependence of switching current…

Materials Science · Physics 2015-06-12 Chun-Yeol You , Myung-Hwa Jung