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We report on optically induced, ultrafast magnetization dynamics in the Heusler alloy $\mathrm{Co_{2}FeAl}$, probed by time-resolved magneto-optical Kerr effect. Experimental results are compared to results from electronic structure theory…

Spin angular momentum transfer in magnetic bilayers offers the possibility of ultrafast and low-loss operation for next-generation spintronic devices. We report the field- and temperature- dependent measurements on the magnetization…

Materials Science · Physics 2023-01-03 X. Liu , P. Liu , H. C. Yuan , J. Y. Shi , H. L. Wang , S. H. Nie , F. Jin , Z. Zheng , X. Z. Yu , J. H. Zhao , H. B. Zhao , G. Lüpke

The measured magnetization dynamics of ferromagnetic iron--cobalt Fe$_{1-x}$Co$_x$ alloys show a strong dependence on the alloy composition, especially near $x=0.25$. Here, we calculate from first principles the electron-phonon coupling…

Materials Science · Physics 2024-10-21 Kevin Moseni , Richard B Wilson , Sinisa Coh

We report on time- and angle-resolved transverse magneto-optical Kerr effect spectroscopy in the soft x-ray range that, by analysis via polarization-dependent magnetic scattering simulations, allows us to determine the spatio-temporal and…

Understanding the rich physics of magnetization dynamics in perpendicular synthetic antiferromagnets (p-SAFs) is crucial for developing next-generation spintronic devices. In this work, we systematically investigate the magnetization…

Mesoscale and Nanoscale Physics · Physics 2023-07-06 Dingbin Huang , Delin Zhang , Yun Kim , Jian-Ping Wang , Xiaojia Wang

Recently magnetic storage and magnetic memory have shifted towards the use of magnetic thin films with perpendicular magnetic anisotropy (PMA). Understanding the magnetic damping in these materials is crucial, but normal Ferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2018-03-14 Dustin M. Lattery , Delin Zhang , Jie Zhu , Paul Crowell , Jian-Ping Wang , Xiaojia Wang

The ability to controllably manipulate the laser-induced ultrafast magnetic dynamics is a prerequisite for future high speed spintronic devices. The optimization of devices requires the controllability of the ultrafast demagnetization time,…

Mesoscale and Nanoscale Physics · Physics 2018-02-14 Wei Zhang , Wei He , Xiang-Qun Zhang , Zhao-Hua Cheng , Jiao Teng , Manfred Fähnle

The magneto-optical Kerr effect (MOKE) in the extreme ultraviolet (EUV) regime has helped to elucidate some of the key processes that lead to the manipulation of magnetism on ultrafast timescales. However, as we show in this paper, the…

Ultrafast magnetization dynamics in metallic heterostructures consists of a combination of local demagnetization in the ferromagnetic constituent and spin-dependent transport contributions within and in between the constituents. Separation…

Understanding spin dynamics on femto- and picosecond timescales offers new opportunities for faster and more efficient spintronic devices. Here, we experimentally investigate the coherent spin dynamics after ultrashort laser excitation by…

Mesoscale and Nanoscale Physics · Physics 2024-01-26 Anulekha De , Akira Lentfert , Laura Scheuer , Benjamin Stadtmüller , Georg von Freymann , Martin Aeschlimann , Philipp Pirro

Element-selective techniques are central for the understanding of ultrafast spin dynamics in multi-element materials like magnetic alloys. Recently, though, it turned out that the commonly used technique of transverse magneto-optical Kerr…

We investigate optically induced ultrafast magnetization dynamics in [Co(0.5 nm)/Pd(1 nm)]x5/NiFe(t) exchange-spring samples with tilted perpendicular magnetic anisotropy using a time-resolved magneto-optical Kerr effect magnetometer. The…

The magneto-optical response of Fe and Ni during ultrafast demagnetization is studied experimentally and theoretically. We have performed pump-probe experiments in the transverse magneto-optical Kerr effect (T-MOKE) geometry using photon…

The magnetization response of bulk ferromagnets after excitation by an ultrashort optical pulse is calculated using a dynamical model of the Elliott-Yafet type that includes the effects of the spin-orbit interaction in the ab-initio…

Materials Science · Physics 2015-06-03 Sven Essert , Hans Christian Schneider

We theoretically investigate spin-dependent carrier dynamics due to the electron-phonon interaction after ultrafast optical excitation in ferromagnetic metals. We calculate the electron-phonon matrix elements including the spin-orbit…

Materials Science · Physics 2015-05-30 Sven Essert , Hans Christian Schneider

The remagnetization process after ultrafast demagnetization can be described by relaxation mechanisms between the spin, electron, and lattice reservoirs. Thereby, collective spin excitations in form of spin waves and their angular momentum…

Despite intense experimental effort, theoretical proposals and modeling approaches, a lack of consensus exists about the intrinsic mechanisms driving ultrafast magnetization dynamics in 3$d$ ferromagnets. In this work, we find evidence of…

Materials Science · Physics 2023-03-29 Theodor Griepe , Unai Atxitia

We present a comprehensive experimental and numerical study of magnetization dynamics triggered in a thin metallic film by single-cycle terahertz pulses of $\sim20$ MV/m electric field amplitude and $\sim1$ ps duration. The experimental…

The Elliott-Yafet mechanism is arguably the most promising candidate to explain the ultrafast demagnetization dynamics in ferromagnetic transition metals on timescales on the order of 100 femtoseconds. So far, only electron-phonon…

We examined the photo-induced dynamics of ferromagnetic Co/Pt thin films demonstrating perpendicular magnetic anisotropy with element specificity using resonant polar magneto-optical Kerr effect measurements at Pt~N${}_{6,7}$ and…

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