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We present a computer simulation study on the crystal nucleation process in suspensions of hard spheres, fully taking into account the solvent hydrodynamics. If the dynamics of collodial crystallization were purely diffusive, the crystal…

Soft Condensed Matter · Physics 2015-06-12 Marc Radu , Tanja Schilling

Polyethylene (PE) chains, with CH2 groups replaced by CBr2 at regular intervals ("precision PE"), have been observed to exhibit competing polymorphs driven by a preference for quantized fold lengths by Tasaki et al. Motivated by this recent…

Soft Condensed Matter · Physics 2024-08-01 Kutlwano Gabana , Gillian A. Gehring , Hendrik Meyer , Goran Ungar , Xiangbing Zeng , William S. Fall

We study a system of active particles with soft repulsive interactions that lead to an active cluster-crystal phase in two dimensions. We use two different modelizations of the active force - Active Brownian particles (ABP) and…

Active matter studies are increasingly geared towards the high-density or glassy limit. This is mainly inspired by the remarkable resemblance between active glassy materials and conventional passive glassy matter. Interestingly, within this…

Soft Condensed Matter · Physics 2022-11-28 Vincent E. Debets , Liesbeth M. C. Janssen

We computationally study suspensions of slow and fast active Brownian particles that have undergone motility induced phase separation and are at steady state. Such mixtures, of varying non-zero activity, remain largely unexplored even…

Soft Condensed Matter · Physics 2024-07-11 Nicholas J Lauersdorf , Ehssan Nazockdast , Daphne Klotsa

Based on Brownian Dynamics (BD) simulations, we study the dynamical self-assembly of active Brownian particles with dipole-dipole interactions, stemming from a permanent point dipole at the particle center. The propulsion direction of each…

Soft Condensed Matter · Physics 2021-06-09 Guo-Jun Liao , Carol K. Hall , Sabine H. L. Klapp

A collection of rings made of active Brownian particles (ABPs) for different packing fractions and activities is investigated using computer simulations. We show that active rings display an emergent dynamic clustering instead of the…

Soft Condensed Matter · Physics 2024-02-27 Ligesh Theeyancheri , Subhasish Chaki , Tapomoy Bhattacharjee , Rajarshi Chakrabarti

We consider homogeneous crystallisation rates in confocal microscopy experiments on colloidal nearly hard spheres at the single particle level. These we compare with Brownian dynamics simuations by carefully modelling the softness in the…

Soft Condensed Matter · Physics 2017-12-27 Jade Taffs , Stephen R. Williams , Hajime Tanaka , C. Patrick Royall

We study how varying the P \'eclet number (Pe) affects the steady state sedimentation of colloidal particles that interact through short-ranged attractions. By employing a hybrid molecular dynamics simulation method we demonstrate that the…

Statistical Mechanics · Physics 2015-06-03 A. Moncho-Jorda' , A. A. Louis , J. T. Padding

We study the conditions under which and how an imposed cluster of fixed colloidal particles at prescribed positions triggers crystal nucleation from a metastable colloidal fluid. Dynamical density functional theory of freezing and Brownian…

Soft Condensed Matter · Physics 2009-11-13 Sven van Teeffelen , Christos N. Likos , Hartmut Löwen

We determined bulk crystal nucleation rates in aqueous suspensions of charged spheres at low metastability. Experiments were performed in dependence on electrolyte concen-tration and for two different particle number densities. The…

Soft Condensed Matter · Physics 2021-11-04 Jürgen Schwarz , Paul Leiderer , Thomas Palberg

The steady state and phase ordering kinetics in a pure active Borwnian particle system are studied in recent years. In binary mixture of active and passive Brownian particles passive particles are used as probe to understand the properties…

Soft Condensed Matter · Physics 2021-08-23 Shambhavi Dikshit , Shradha Mishra

The active phase-field-crystal (active PFC) model provides a simple microscopic mean field description of crystallization in active systems. It combines the PFC model (or conserved Swift-Hohenberg equation) of colloidal crystallization and…

Soft Condensed Matter · Physics 2021-03-10 Lukas Ophaus , Edgar Knobloch , Svetlana V. Gurevich , Uwe Thiele

We study the freezing kinetics of colloidal polycrystals made of micelles of Pluronic F108, a thermosensitive copolymer, to which a small amount of silica nanoparticles of size comparable to that of the micelles are added. We use rheology…

Soft Condensed Matter · Physics 2013-03-18 A. Louhichi , E. Tamborini , N. Ghofraniha , F. Caton , D. Roux , J. Oberdisse , L. Cipelletti , L. Ramos

Nucleation is an activated process in which the system has to overcome a free energy barrier in order for a first-order phase transition between the metastable and the stable phases to take place. In the liquid-to-solid transition the…

Soft Condensed Matter · Physics 2016-11-28 John Russo , Hajime Tanaka

Chiral active matter is a variant of active matter systems in which the motion of the constituent particles violates mirror symmetry. In this letter, we simulate two-dimensional chiral Active Brownian Particles, the simplest chiral model in…

Soft Condensed Matter · Physics 2025-12-03 Kangeun Jeong , Yuta Kuroda , Yuki Asatani , Takeshi Kawasaki , Kunimasa Miyazaki

We investigate the structural and dynamic properties of active Brownian particles (APs) confined within a soft annulus-shaped channel. Depending on the strength of the confinement and the P\'eclet number, we observe a novel re-entrant…

Soft Condensed Matter · Physics 2025-05-15 Timo Knippenberg , Ashreya Jayaram , Thomas Speck , Clemens Bechinger

We investigate conformations and dynamics of a polymer considering its monomers to be active Brownian particles. This active polymer shows very intriguing physical behavior which is absent in an active Rouse chain. The chain initially…

Soft Condensed Matter · Physics 2020-04-13 Shalabh K. Anand , Sunil P. Singh

Particle systems interacting with a soft repulsion, at thermal equilibrium and under some circumstances, are known to form cluster crystals, i.e. periodic arrangements of particle aggregates. We study here how these states are modified by…

Statistical Mechanics · Physics 2018-11-28 Lorenzo Caprini , Emilio Hernandez-Garcia , Cristobal Lopez

Chemically active Brownian particles with surface catalytic reactions may repel each other due to diffusiophoretic interactions in the reaction and product concentration fields. The system behavior can be described by a `chemical' coupling…

Soft Condensed Matter · Physics 2017-12-04 Wen Yan , John F. Brady