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The reactivity of interstellar carbon atoms (C) on the water-dominated ices is one of the possible ways to form interstellar complex organic molecules (iCOMs). In this work, we report a quantum chemical study of the coupling reaction of C…

Astrophysics of Galaxies · Physics 2023-10-24 Stefano Ferrero , Cecilia Ceccarelli , Piero Ugliengo , Mariona Sodupe , Albert Rimola

Indene (C$_9$H$_8$) is the only polycyclic pure hydrocarbon identified in the interstellar medium to date, with an observed abundance orders of magnitude higher than predicted by astrochemical models. The dissociation and radiative…

Processing by interstellar photons affects the composition of the icy mantles on interstellar grains. The rate of photodissociation in solids differs from that of molecules in the gas phase. The aim of this work was to determine an average,…

Astrophysics of Galaxies · Physics 2018-05-16 Juris Kalvans

Ion Coulomb crystals (ICC), formed by atomic ions at low temperatures in radiofrequency and Penning ion traps, are structures that have remarkable properties and many applications. Images of Coulomb crystals are striking and reveal the…

Quantum Physics · Physics 2022-08-11 Richard C. Thompson

External flows of energy, entropy, and matter can cause sudden transitions in the stability of biological and industrial systems, fundamentally altering their dynamical function. How might we control and design these transitions in chemical…

Molecular Networks · Quantitative Biology 2023-06-19 Zachary G. Nicolaou , Schuyler B. Nicholson , Adilson E. Motter , Jason R. Green

The 29 reactions linking carbon monosulfide (CS) to methyl mercaptan (CH3SH) via ten intermediate radicals and molecules have been characterized with relevance to surface chemistry in cold interstellar ices. More intermediate species than…

Astrophysics of Galaxies · Physics 2018-06-11 T Lamberts

Titan is unique in the solar system as it hosts a dense atmosphere mainly made of N$_2$ and CH$_4$. Cassini-Huygens revealed the presence of an intense atmospheric photochemistry initiated by the photo-dissociation and ionization of N$_2$…

Earth and Planetary Astrophysics · Physics 2020-02-26 David Dubois , Nathalie Carrasco , Lora Jovanovic , Ludovic Vettier , Thomas Gautier , Joseph Westlake

Mixtures of bare atomic nuclei on a nearly uniform degenerate electron background are a realistic model of matter in the interior of white dwarfs. Despite tremendous progress in understanding their phase diagrams achieved mainly via…

Solar and Stellar Astrophysics · Physics 2025-04-17 D. A. Baiko

Isolating neutral and charged particles from the environment is essential in precision experiments. For decades, this has been achieved by trapping ions with radio-frequency (rf) fields and neutral particles with optical fields. Recently,…

Atomic Physics · Physics 2021-05-05 Tobias Schaetz

A detailed understanding of biochemical networks at the molecular level is essential for studying complex cellular processes. In this paper, we provide a comprehensive description of biochemical networks by considering individual atoms and…

Molecular Networks · Quantitative Biology 2025-04-08 Hadjar Rahou , Hulda S. Haraldsdottir , Filippo Martinelli , Ines Thiele , Ronan M. T. Fleming

We consider collisional studies of linear polyatomic ions immersed in ultracold atomic gases and investigate the intermolecular interactions and chemical reactions of several molecular anions ($\mathrm{OH}^-$, $\mathrm{CN}^-$,…

Atomic Physics · Physics 2017-07-04 Michał Tomza

Metal-bearing species in diffuse or molecular clouds are often overlooked in astrochemical modeling except for the charge exchange process. However, catalytic cycles involving these metals can affect the abundance of other compounds. We…

Astrophysics of Galaxies · Physics 2025-08-20 Ankan Das , Milan Sil , Paola Caselli

Carbon chain molecules may be an important reservoir of reactive organics during star and planet formation. Carbon chains have been observed toward several low-mass young stellar objects (YSOs), but their typical abundances and chemical…

Astrophysics of Galaxies · Physics 2018-08-22 Charles J. Law , Karin I. Oberg , Jennifer B. Bergner , Dawn Graninger

Long-chain hydrocarbon anions CnH- (n=4, 6, 8) have recently been found to be abundant in a variety of interstellar clouds. In order to explain their large abundances in the denser (prestellar/protostellar) environments, new chemical models…

Astrophysics of Galaxies · Physics 2015-06-04 M. A. Cordiner , S. B Charnley

Neutron capture cross sections of unstable isotopes are important for neutron-induced nucleosynthesis as well as for technological applications. A combination of a radioactive beam facility, an ion storage ring and a high flux reactor would…

In the first part of this paper we give a short review of the hierarchy of stochastic models, related to physical chemistry. In the basement of this hierarchy there are two models --- stochastic chemical kinetics and the Kac model for…

Mathematical Physics · Physics 2011-12-26 V. A. Malyshev

We propose a new model for treating solid-phase photoprocesses in interstellar ice analogues. In this approach, photoionization and photoexcitation are included in more detail, and the production of electronically-excited (suprathermal)…

We theoretically characterize interactions, energetics, and chemical reaction paths in ionic two-body and three-body systems of alkali-metal and alkaline-earth-metal atoms in the context of modern experiments with cold hybrid ion-atom…

Atomic Physics · Physics 2021-02-16 Michał Śmiałkowski , Michał Tomza

HCN is a molecule central to interstellar chemistry, since it is the simplest molecule containing a carbon-nitrogen bond and its solid state chemistry is rich. The aim of this work was to study the NH3 + HCN -> NH4+CN- thermal reaction in…

Earth and Planetary Astrophysics · Physics 2015-06-11 J. A. Noble , P. Theule , F. Borget , G. Danger , M. Chomat , F. Duvernay , F. Mispelaer , T. Chiavassa

H3+ and the deuterated isotopomers are thought to play an important role in interstellar chemistry. The partition functions of H3+, D2H+ and D3+ are calculated to a temperature of 800 K by explicitly summing the ab initio determined…

Astrophysics · Physics 2009-11-10 Jayesh Ramanlal , Jonathan Tennyson
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