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Signal Amplification By Reversible Exchange (SABRE) and the heteronuclear variant, X-SABRE, increase the sensitivity of magnetic resonance techniques using order derived from reversible binding of para-hydrogen. One current limitations of…

Chemical Physics · Physics 2022-08-31 Shannon L Eriksson , Mathew W Mammen , Clark W Eriksson , Jacob R Lindale , Warren S Warren

Signal amplification by reversible exchange (SABRE) is a nuclear spin hyperpolarization technique in which the transient interaction of parahydrogen (pH2) and a target substrate with an iridium complex leads to polarization transfer to the…

Hyperpolarisation using Signal Amplification By Reversible Exchange (SABRE) is a convenient method for high repeatability studies. The core of this technique is polarisation transfer to the target substrate during an on-going chemical…

Signal Amplification By Reversible Exchange (SABRE) creates hyperpolarization (large spin magnetization) using a transition metal catalyst and parahydrogen, addressing the sensitivity limitations of magnetic resonance. SABRE and its…

Chemical Physics · Physics 2021-07-13 Shannon L. Eriksson , Jacob R. Lindale , Xiaoqing Li , Warren S. Warren

Hyperpolarization approaches in magnetic resonance overcome the sensitivity limitations imposed by thermal magnetization and play an important role in a very wide range of modern applications. One of the newer strategies, variants of what…

Chemical Physics · Physics 2025-11-10 Loren L. Smith , Warren S. Warren

SABRE (Signal Amplification By Reversible Exchange) has become a widely used method for hyper-polarizing nuclear spins, thereby enhancing their Nuclear Magnetic Resonance (NMR) signals by orders of magnitude. In SABRE experiments,…

Chemical Physics · Physics 2020-12-02 Stephan Knecht , Danila A. Barskiy , Gerd Buntkowsky , Konstantin L. Ivanov

A theoretical approach is proposed for quantitative modeling of SABRE (Signal Amplification By Reversible Exchange) experiments performed at a high magnetic field of an NMR spectrometer. SABRE is a method, which exploits the spin order of…

Chemical Physics · Physics 2019-05-01 Stephan Knecht , Konstantin L. Ivanov

The inherently low signal-to-noise ratio of NMR and MRI is now being addressed by hyperpolarization methods. For example, iridium-based catalysts that reversibly bind both parahydrogen and ligands in solution can hyperpolarize protons…

SABRE (Signal Amplification by Reversible Exchange) methods provide a simple, fast, and cost-effective method to hyperpolarize a wide variety of molecules in solution, and have been demonstrated with protons and, more recently, with…

Chemical Physics · Physics 2022-02-14 Xiaoqing Li , Jacob R. Lindale , Shannon L. Eriksson , Warren S. Warren

SABRE (Signal Amplification By Reversible Exchange) is a technique for enhancement of NMR (Nuclear Magnetic Resonance) signals, which utilizes parahydrogen (pH2, the H2 molecule in its nuclear spin state) as a source of non-thermal spin…

Hyperpolarization methods in magnetic resonance overcome sensitivity limitations, especially for low-{\gamma} nuclei such as 13C and 15N. Signal Amplification By Reversible Exchange (SABRE) and extended SABRE (X-SABRE) are efficient and…

Chemical Physics · Physics 2022-04-06 Jacob R. Lindale , Shannon L. Eriksson , Warren S. Warren

Development of the methods to exploit nuclear hyperpolarization and search for molecules whose nuclear spins can be efficiently hyperpolarized is an active area in nuclear magnetic resonance. Of particular interest are those molecules that…

The sensitivity of NMR and MRI can be boosted via hyperpolarization of nuclear spins. However, current methods are costly, polarization is relatively low, or applicability is limited. Here, we report a new hyperpolarization method combining…

Spin-polarized solid targets have underpinned many recent key advances in nuclear and particle physics, yet traditional methods to produce them face significant limitations due to the high cost and demanding cryogenic and magnetic field…

It is well known that the association of parahydrogen (pH2) with an unsaturated molecule or a transient metalorganic complex can enhance the intensity of NMR signals; the effect is known as parahydrogen-induced polarization (PHIP). During…

Chemical Physics · Physics 2024-09-26 Andrey N. Pravdivtsev , Danila A. Barskiy , Jan-Bernd Hövener , Igor V. Koptyug

We describe a new method for pulsed spin order transfer (SOT) of parahydrogen induced polarization (PHIP) that enables close to 100 % polarization in incompletely 2H-labeled molecules by exciting only the desired protons in a…

Nuclear spin hyperpolarization enables real-time observation of metabolism and intermolecular interactions in vivo. 1-13C-Pyruvate is the leading hyperpolarized tracer currently under evaluation in several clinical trials as a promising…

We describe a new approach to precision NMR with hyperpolarized gases designed to mitigate NMR frequency shifts due to the alkali spin exchange field. The electronic spin polarization of optically pumped alkali atoms is square-wave…

Atomic Physics · Physics 2015-12-23 Anna Korver , Daniel Thrasher , Mike Bulatowicz , Thad Walker

The potential of exchange spring bilayers and graded media is reviewed. An analytical model for the optimization of graded media gives an optimal value of the magnetic polarization of Js = 0.8 T. The optimum design allows for thermally…

Materials Science · Physics 2011-11-02 D. Suess , J. Lee , J. Fidler , T. Schrefl

Four-wave parametric amplification can be extended to the TW/cm$^2$ regime using femtosecond pump pulses to amplify nearly octave spanning pulses with gain $> 20$~mm$^{-1}$, which we call Kerr instability amplification. Cross-polarized wave…

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