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A first principles approach for spin and angle resolved resonant photoemission is developed within multiple scattering theory and applied to a Cr(110) surface at the 2$p$-3$d$ resonance. The resonant photocurrent from this non ferromagnetic…

Strongly Correlated Electrons · Physics 2015-06-15 F. Da Pieve , P. Krüger

We elucidate light-induced orbital and spin current through nonlinear response theory, which generalizes the well-known bulk photovoltaic effect in centrosymmetric broken materials from charge to the spin and orbital degrees of freedom. We…

Materials Science · Physics 2021-08-30 Xingchi Mu , Jian Zhou

Photo-excited quantum materials can be driven into thermally inaccessible metastable states that exhibit structural, charge, spin, topological and superconducting orders. Metastable states typically emerge on timescales set by the intrinsic…

Strongly Correlated Electrons · Physics 2025-07-24 Xinwei Li , Iliya Esin , Youngjoon Han , Yincheng Liu , Hengdi Zhao , Honglie Ning , Cora Barrett , Jun-Yi Shan , Kyle Seyler , Gang Cao , Gil Refael , David Hsieh

We study the microscopic origins of photocurrent generation in the topological insulator Bi$_2$Se$_3$ via time- and angle-resolved photoemission spectroscopy. We image the unoccupied band structure as it evolves following a circularly…

Due to the lack of a net magnetic moment, antiferromagnets possess a unique robustness to external magnetic fields and are thus predicted to play an important role in future magnetic technologies. However, this robustness also makes them…

The interplay between crystal symmetry and its optical responses is at the heart of tremendous recent advances in light-matter interactions and applications. Nonlinear optical processes that produce electric currents, for example bulk…

Materials Science · Physics 2021-10-27 Yongliang Shi , Jian Zhou

A linearly polarized light normally incident on a semiconductor quantum well with spin-orbit coupling may generate pure spin current via direct interband optical transition. An electric photocurrent can be extracted from the pure spin…

Mesoscale and Nanoscale Physics · Physics 2011-04-04 Hai-Zhou Lu , Bin Zhou , Fu-Chun Zhang , Shun-Qing Shen

The phenomena of crystal size changes and structural phase transitions induced by light irradiation have garnered significant interest due to their potential for tuning and controlling a wide range of material properties through highly…

Materials Science · Physics 2023-10-11 Ruixiang Fei , Li Yang

The currently accepted magnetic ground state of Sr2IrO4 (the -++- state) preserves inversion symmetry. This is at odds, though, with recent experiments that indicate a magnetoelectric ground state, leading to the speculation that orbital…

Strongly Correlated Electrons · Physics 2016-08-30 S. Di Matteo , M. R. Norman

Photocurrent measurements provide a powerful means of studying the spatially resolved optoelectronic and electrical properties of a material or device. Generally speaking there are two classes of mechanism for photocurrent generation: those…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 Helin Cao , Grant Aivazian , Zaiyao Fei , Jason Ross , David H. Cobden , Xiaodong Xu

In the circular photogalvanic effect, circularly polarized light can produce a direct electron photocurrent in metals and the direction of the current depends on the polarization. We suggest that an analogous nonlinear effect exists for…

Mesoscale and Nanoscale Physics · Physics 2018-10-16 Igor Proskurin , Alexander S. Ovchinnikov , Jun-ichiro Kishine , Robert L. Stamps

A new class of photocurrents is predicted to occur in both type-I and type-II Weyl semimetals. Unlike the previously studied photocurrents in chiral materials, the proposed current requires neither circularly polarized light, nor an absence…

Mesoscale and Nanoscale Physics · Physics 2020-10-21 Sahal Kaushik , Dmitri E. Kharzeev , Evan John Philip

Layered 5$d$ transition iridium oxides, Sr$_2$(Ir,Rh)O$_4$, are described as unconventional Mott insulators with strong spin-orbit coupling. The undoped compound, Sr$_2$IrO$_4$, is a nearly ideal two-dimensional pseudospin-$1/2$ Heisenberg…

Strongly Correlated Electrons · Physics 2017-05-02 Jaehong Jeong , Yvan Sidis , Alex Louat , Véronique Brouet , Philippe Bourges

We theoretically predict the emergence of 120-degree spin order as a nonequilibrium steady state in the photodriven Kondo-lattice model on a triangular lattice. In the system away from the half filling with ferromagnetic ground state, the…

Strongly Correlated Electrons · Physics 2022-05-04 Takashi Inoue , Masahito Mochizuki

To add to the rapidly progressing field of ultrafast photocurrent, we propose a universal method to generate photocurrent in normal and topological materials using a pair of multicycle linearly polarized laser pulses. The interplay of the…

Mesoscale and Nanoscale Physics · Physics 2024-03-20 Amar Bharti , Gopal Dixit

Transport properties of a quantum dot coupled to a photon cavity are investigated using a quantum master equation in the steady-state regime. In the off-resonance regime, when the photon energy is smaller than the energy spacing between the…

Mesoscale and Nanoscale Physics · Physics 2019-10-29 Nzar Rauf Abdullah , Chi-Shung Tang , Andrei Manolescu , Vidar Gudmundsson

Photoinduced hidden phases are often observed in materials with intertwined orders. Understanding the formation of these non-thermal phases is challenging and requires a resolution of the cooperative interplay between different orders on…

Strongly Correlated Electrons · Physics 2018-11-06 Jiajun Li , Hugo U. R. Strand , Philipp Werner , Martin Eckstein

Photovoltaic effect, e.g., solar cells, converts light into DC electric current. This phenomenon takes place in various setups such as in noncentrosymmetric crystals and semiconductor pn junctions. Recently, we proposed a theory for…

Strongly Correlated Electrons · Physics 2020-10-23 Masahiro Sato , Hiroaki Ishizuka

Nonlinear optical responses are often used as a probe for studying electronic properties of materials. For topological materials, studies so far focused on the photogalvanic electric current, which requires breaking inversion symmetry. In…

Materials Science · Physics 2022-03-21 Margarita Davydova , Maksym Serbyn , Hiroaki Ishizuka

An anapole state that breaks inversion and time reversal symmetries with preserving translation symmetry of underlying lattice has aroused great interest as a new quantum state, but only a few candidate materials have been reported.…

Strongly Correlated Electrons · Physics 2021-02-10 H. Murayama , K. Ishida , R. Kurihara , T. Ono , Y. Sato , Y. Kasahara , H. Watanabe , Y. Yanase , G. Cao , Y. Mizukami , T. Shibauchi , Y. Matsuda , S. Kasahara