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Related papers: Exploring Coupled Cluster Green's function as a me…

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Coupled cluster Green's function (CCGF) approach has drawn much attention in recent years for targeting the molecular and material electronic structure problems from a many-body perspective in a systematically improvable way. Here, we will…

Chemical Physics · Physics 2021-11-01 Bo Peng , Nicholas P. Bauman , Sahil Gulania , Karol Kowalski

We study the single-band Hubbard model under the action of an external magnetic field using the cumulant Green's functions method (CGFM). The starting point of the method is to diagonalize a cluster containing N correlated sites (seed) and…

Strongly Correlated Electrons · Physics 2023-04-12 Renan Lira , Peter Riseborough , Jereson Silva-Valencia , Marcos Figueira

The self-energy method for quantum impurity models expresses the correlation part of the self-energy in terms of the ratio of two Green's functions and allows for a more accurate calculation of equilibrium spectral functions than is…

Strongly Correlated Electrons · Physics 2021-11-24 H. T. M. Nghiem , T. A. Costi

In this study, we have calculated single-electron energy spectra via the Green's function based on the coupled-cluster singles and doubles (GFCCSD) method for isolated atoms from H to Ne. In order to check the accuracy of the GFCCSD method,…

Materials Science · Physics 2018-07-26 Hirofumi Nishi , Taichi Kosugi , Yoritaka Furukawa , Yu-ichiro Matsushita

We investigate the ground-state properties of the Anderson single impurity model (finite Coulomb impurity repulsion) with the Coupled Cluster Method. We consider different CCM reference states and approximation schemes and make comparison…

Strongly Correlated Electrons · Physics 2009-06-26 Jin-Jun Liang , Clive Emary , Tobias Brandes

The vertex function ($\Gamma$) within the Green's function formalism encapsulates information about all higher-order electron-electron interaction beyond those mediated by density fluctuations. Herein, we present an efficient approach that…

Chemical Physics · Physics 2023-03-28 Guorong Weng , Rushil Mallarapu , Vojtech Vlcek

The cumulant expansion of the Green's function is a computationally efficient beyond-$GW$ approach renowned for its significant enhancement of satellite features in materials. In contrast to the ubiquitous $GW$ approximation of many-body…

Chemical Physics · Physics 2024-02-27 Pierre-François Loos , Antoine Marie , Abdallah Ammar

We demonstrate that the effective Hamiltonians obtained with the downfolding procedure based on double unitary coupled cluster (DUCC) ansatz can be used in the context of Greens function coupled cluster (GFCC) formalism to calculate…

Computational Physics · Physics 2020-12-02 Nicholas P Bauman , Bo Peng , Karol Kowalski

Real-time nonequilibrium Green functions (NEGF) have been very successful to simulate the dynamics of correlated many-particle systems far from equilibrium. However, NEGF simulations are computationally expensive since the effort scales…

Strongly Correlated Electrons · Physics 2023-12-27 Karsten Balzer , Niclas Schlünzen , Hannes Ohldag , Jan-Philip Joost , Michael Bonitz

Quantitative descriptions of strongly correlated materials pose a considerable challenge in condensed matter physics and chemistry. A promising approach to address this problem is quantum embedding methods. In particular, the dynamical…

Quantum Physics · Physics 2024-05-07 Rihito Sakurai , Wataru Mizukami , Hiroshi Shinaoka

We demonstrate in the present study that self-consistent calculations based on the self-energy functional theory (SFT) are possible for the electronic structure of realistic systems in the context of quantum chemistry. We describe the…

Materials Science · Physics 2018-06-14 Taichi Kosugi , Hirofumi Nishi , Yoritaka Furukawa , Yu-ichiro Matsushita

We demonstrate that coupled-cluster singles-and-doubles Green's function (GFCCSD) method is a powerful and prominent tool drawing the electronic band structures and the total energies, which many theoretical techniques struggle to…

Materials Science · Physics 2018-05-29 Yoritaka Furukawa , Taichi Kosugi , Hirofumi Nishi , Yu-ichiro Matsushita

We present an implementation of the self-energy embedding theory (SEET) for periodic systems and provide a fully self-consistent embedding solution for a simple realistic periodic problem - 1D crystalline hydrogen - that displays many of…

Chemical Physics · Physics 2019-10-01 Alexander A. Rusakov , Sergei Iskakov , Lan Nguyen Tran , Dominika Zgid

Deep clustering as an important branch of unsupervised representation learning focuses on embedding semantically similar samples into the identical feature space. This core demand inspires the exploration of contrastive learning and…

Computer Vision and Pattern Recognition · Computer Science 2024-04-16 Haifeng Xia , Hai Huang , Zhengming Ding

Quantum embedding theories provide a feasible route for obtaining quantitative descriptions of correlated materials. However, a critical challenge is solving an effective impurity model of correlated orbitals embedded in an electron bath.…

Strongly Correlated Electrons · Physics 2021-01-27 Hiroshi Shinaoka , Yuki Nagai

We develop a static quantum embedding scheme that utilizes different levels of approximations to coupled cluster (CC) theory for an active fragment region and its environment. To reduce the computational cost, we solve the local fragment…

Chemical Physics · Physics 2024-11-13 Avijit Shee , Fabian M. Faulstich , Birgitta Whaley , Lin Lin , Martin Head-Gordon

We present an efficient and accurate method for calculating electronic structure and related properties of random alloys with a proper treatment of local environment effects. The method is a generalization of the locally self-consistent…

Materials Science · Physics 2012-05-15 Oleg E. Peil , Andrei V. Ruban , Börje Johansson

We investigate transport properties of gate-all-around Si nanowires using non-equilibrium Green's function technique. By taking into account of the ionized impurity scattering we calculate Green's functions self-consistently and examine the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. H. OH , D. Ahn , Y. S. Yu , S. W. Hwang

Quantum embedding methods, such as dynamical mean-field theory (DMFT), provide a powerful framework for investigating strongly correlated materials. A central computational bottleneck in DMFT is in solving the Anderson impurity model (AIM),…

We present a Green's function formulation of the quantum defect embedding theory (QDET) where a double counting scheme is rigorously derived within the $G_0 W_0$ approximation. We then show the robustness of our methodology by applying the…

Quantum Physics · Physics 2022-06-07 Nan Sheng , Christian Vorwerk , Marco Govoni , Giulia Galli