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We propose and demonstrate a method for measuring the joint spectrum of photon pairs via Fourier spectroscopy. The biphoton spectral intensity is computed from a two-dimensional interferogram of coincidence counts. The method has been…

Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…

We present a technique to completely characterise the spectral-temporal wave function of a broadband photon pair using spectral-shearing interferometry. Our method is fully self-referencing and is generalisable across a wide range of…

Quantum Physics · Physics 2018-09-12 Alex O. C. Davis , Valerian Thiel , Brian J. Smith

The development of new quantum light sources requires robust and convenient methods of characterizing their joint spectral properties. Measuring the joint spectral intensity between a photon pair ignores any correlations in spectral phase…

Quantum Physics · Physics 2020-12-02 Bryn A. Bell , Gil Triginer Garces , Ian A. Walmsley

Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…

Quantum Physics · Physics 2022-11-23 Yuanyuan Chen , Roberto de J. León-Montiel , Lixiang Chen

Interferometers provide a highly sensitive means to investigate and exploit the coherence properties of light in metrology applications. However, interferometers come in various forms and exploit different properties of the optical states…

We demonstrate experimentally the tunable control of the joint spectrum, i.e. waveform and degree of frequency correlations, of paired photons generated in spontaneous parametric downconversion. This control is mediated by the spatial shape…

Quantum metrology overcomes standard precision limits by exploiting collective quantum superpositions of physical systems used for sensing, with the prominent example of non-classical multiphoton states improving interferometric techniques.…

In this work we present a simple method to reconstruct the complex spectral wavefunction of a biphoton, and hence gain complete information about the spectral and temporal properties of a photon pair. The technique, which relies on quantum…

The frequency comb of a multimode interferometer offers exceptional scalability potential for field-encoded quantum information. However, the staple field detection method, homodyne detection, cannot access quantum information in the whole…

Quantum Physics · Physics 2026-03-11 Bakhao Dioum , Virginia D'Auria , Alessandro Zavatta , Olivier Pfister , Giuseppe Patera

Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…

We describe a detector that measures the mutual coherence of two optical fields directly using quantum interference, free from photon noise of the individual irradiances. Our approach utilizes Raman transition in an atomic system where the…

Quantum Physics · Physics 2008-12-16 Jungsang Kim , David J. Brady

Joint spectral measurements are a powerful tool for characterising biphoton spectral correlation, which is crucial for quantum information and communication technologies. In these applications, highly pure biphoton states are essential in…

The ability to characterize the complete quantum state of light is essential for both fundamental and applied science. For single photons the quantum state is provided by the mode that it occupies. The spectral temporal mode structure of…

Quantum interferometry based on induced-coherence phenomena has demonstrated the possibility of undetected-photon measurements. Perturbation in the optical path of probe photons can be detected by interference signals generated by quantum…

Quantum Physics · Physics 2023-09-14 Eun Mi Kim , Sun Kyung Lee , Sang Min Lee , Myeong Soo Kang , Hee Su Park

The authors demonstrate a form of two-photon-counting interferometry by measuring the coincidence counts between single-photon-counting detectors at an output port of a Mach-Zehnder Interferometer (MZI) following injection of broad-band…

Fourier transform spectroscopy with classical interferometry corresponds to the measurement of a single-photon intensity spectrum from the viewpoint of the particle nature of light. In contrast, the Fourier transform of two-photon quantum…

Quantum Physics · Physics 2021-11-04 Hiroya Seki , Kensuke Miyajima , Ryosuke Shimizu

We present an optical method to measure radio-frequency electro-optic phase modulation profiles by employing spectrum-to-time mapping realized by highly chirped optical pulses. We directly characterize temporal phase modulation profiles of…

Instrumentation and Detectors · Physics 2017-11-23 Michał Jachura , Jan Szczepanek , Wojciech Wasilewski , Michal Karpinski

Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…

Chemical Physics · Physics 2026-04-21 Yuta Fujihashi , Ozora Iso , Ryosuke Shimizu , Akihito Ishizaki

As first demonstrated by Hanbury Brown and Twiss, it is possible to observe interference between independent light sources by measuring correlations in their intensities rather than their amplitudes. In this work, we apply this concept of…

Quantum Physics · Physics 2023-07-07 G. S. Thekkadath , D. England , F. Bouchard , Y. Zhang , M. S. Kim , B. Sussman
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