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A major impediment towards realizing technologies based on the emerging principles of antiferromagnetic spintronics is the shortage of suitable materials. In this paper, we propose a design of polar|nonpolar heterostructures of perovskite…

Materials Science · Physics 2020-12-23 Jayita Chakraborty , Nirmal Ganguli

We investigate the effect of oxygen vacancies and hydrogen dopants at the surface and inside slabs of LaAlO3, SrTiO3, and LaAlO3/SrTiO3 heterostructures on the electronic properties by means of electronic structure calculations as based on…

Strongly Correlated Electrons · Physics 2019-05-03 I. I. Piyanzina , V. Eyert , Yu. V. Lysogorskiy , D. A. Tayurskii , T. Kopp

The discovery of conducting two-dimensional electron gas (2DEG) and magnetism at the interface between insulating nonmagnetic oxides, as exemplified by the polar LaAlO3 and nonpolar SrTiO3 has raised prospects for attaining interfacial…

Materials Science · Physics 2014-10-15 Liping Yu , Alex Zunger

We perform first-principles density functional calculations to elucidate structural, electronic and magnetic properties at the interface of \ce{(0001)Cr2O3-(111)Pt} bilayers. This investigation is motivated by the fact that, despite the…

Materials Science · Physics 2024-05-09 Marlies Reher , Nicola A. Spaldin , Sophie F. Weber

The emerging interest in two-dimensional electron gases (2DEGs), formed at interfaces between two insulating oxide perovskites poses crucial fundamental question in view of future electronic devices. In the framework of density-functional…

Materials Science · Physics 2022-03-09 Le Fang , Wahib Aggoune , Wei Ren , Claudia Draxl

Interfacial polarization-charge accumulation at the heterointerface-is a well-established tool in semiconductors, but its influence in metals remains unexplored. Here, we demonstrate that interfacial polarization can robustly modulate…

Amorphous insulating oxides play a significant role in the contemporary electronic industry. Understanding the band alignment of heterogeneous interfaces containing amorphous structures helps to better control the carrier transport property…

Materials Science · Physics 2017-05-17 Jianqiu Huang , Fei Lin , Celine Hin

At the interface between complex insulating oxides, novel phases with interesting properties may occur, such as the metallic state reported in the LaAlO3/SrTiO3 system. While this state has been predicted and reported to be confined at the…

Black TiO2 nanoparticles with a crystalline-core and amorphous-shell structure exhibit superior optoelectronic properties in comparison with pristine TiO2. The fundamental mechanisms underlying these enhancements, however, remain unclear,…

Lattice structure can dictate electronic and magnetic properties of a material. Especially, reconstruction at a surface or heterointerface can create properties that are fundamentally different from those of the corresponding bulk material.…

Materials Science · Physics 2021-06-21 Prahald Siwakoti , Zhen Wang , Mohammad Saghayezhian , David Howe , Zeeshan Ali , Yimei Zhu , Jiandi Zhang

The predictions of the polar catastrophe scenario to explain the occurrence of a metallic interface in heterostructures of the solid solution(LaAlO$_3$)$_{x}$(SrTiO$_3$)$_{1-x}$ (LASTO:x) grown on (001) SrTiO$_3$ were investigated as a…

The two-dimensional electron gas (2DEG) found in KTaO3-based interfaces has garnered attention due to its remarkable electronic properties. In this study, we investigated the conducting system embedded at the Si3N4/Al//KTO(110)…

Photonic modes exhibiting a polarization winding akin to a vortex possess an integer topological charge. Lasing with topological charge 1 or 2 can be realized in periodic lattices of up to six-fold rotational symmetry. Higher order charges…

We studied strain-induced polarization and resulting conductivity in the nonpolar/nonpolar CaZrO3/SrTiO3 (CZO/STO) heterostructure (HS) system by means of first-principles electronic structure calculations. By modeling four types of CZO/STO…

Materials Science · Physics 2019-12-18 Safdar Nazir , Jianli Cheng , Kesong Yang

We use density functional theory plus dynamical mean-field theory to demonstrate the emergence of a metallic layer at the interface between the two Mott insulators LaTiO$_3$ and LaVO$_3$. The metallic layer is due to charge transfer across…

Strongly Correlated Electrons · Physics 2019-09-11 Sophie Beck , Claude Ederer

The interface between magnetic materials and topological insulators can drive the formation of exotic phases of matter and enable functionality through manipulation of the strong spin polarized transport. Here, we report that the…

Quantum confinement at complex oxide interfaces establishes an intricate hierarchy of the strongly correlated $d$-orbitals which is widely recognized as a source of emergent physics. The most prominent example is the (001)…

Strongly Correlated Electrons · Physics 2019-05-15 A. M. R. V. L. Monteiro , M. Vivek , D. J. Groenendijk , P. Bruneel , I. Leermakers , U. Zeitler , M. Gabay , A. D. Caviglia

The collective behavior of correlated electrons in the VO$_2-$interface layer of LaVO$_3$/SrTiO$_3$ heterostructure is studied within a quarter-filled $t_{2g}$-orbital Hubbard model on a square lattice. We argue that the ground state is…

Strongly Correlated Electrons · Physics 2008-11-21 G. Jackeli , G. Khaliullin

We studied LaAlO3/SrTiO3 interfaces for varying LaAlO3 thickness by core-level photoemission spectroscopy. In Ti 2p spectra for conducting "n-type" interfaces, Ti3+ signals appeared, which were absent for insulating "p-type" interfaces. The…

Materials Science · Physics 2015-05-28 M. Takizawa , S. Tsuda , T. Susaki , H. Y. Hwang , A. Fujimori

The heterointerface between topological insulators and magnetic materials provides a crucial platform for investigating exotic electronic and magnetic phases, with implications for both fundamental studies and potential applications. A key…

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