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In this paper, we present a theoretical study of the nonlinear optical response of the newly discovered conjugated polymer poly(diphenyl)polyacetylene (PDPA). In particular, we compute the third-order nonlinear susceptibility corresponding…

Mesoscale and Nanoscale Physics · Physics 2010-01-14 Alok Shukla

Platinum diselenide (PtSe2) is a promising two-dimensional (2D) material for the terahertz (THz) range as, unlike other transition metal dichalcogenides (TMDs), its bandgap can be uniquely tuned from a semiconductor in the near-infrared to…

Light-matter interactions in two-dimensional (2D) materials have gained significant interest due to their distinctive optical and electronic properties. Recently, silicates have emerged as a promising new class of 2D materials, but their…

We investigate the nonlinear optical properties of BiOBr nanoflakes, a novel two-dimensional (2D) layered material from the Bismuth oxyhalide family. We measure the nonlinear absorption and Kerr nonlinearity of BiOBr nanoflakes at both 800…

Following a recently manifested guide of how to team up infrared transparency and high electrical conductivity within semimetal materials [C. Cui $et$ $al.$ Prog. Mater. Sci. 2023, 136, 101112], we evaluate an applicability of the calcium…

This study demonstrates that two-dimensional (2D) Bi2Te3 exhibits strong light-matter interaction, enabling a broadband Kerr nonlinear optical response. This characteristic is advantageous for nonreciprocal light propagation in passive…

We investigate the third harmonic response of platinum ditelluride (PtTe$_2$), a Dirac semimetal belonging to the transition metal dichalcogenides class. Due to its topological properties, this material has drawn a lot of attention,…

Recently, two-dimensional materials and in particular transition metal dichalcogenides (TMDs) were extensively studied because of their strong light-matter interaction and the remarkable optoelectronic response of their field-effect…

Although diamond photonics has driven considerable interest and useful applications, as shown in frequency generation devices and single photon emitters, fundamental studies on the third-order optical nonlinearities of diamond are still…

The existence of large nonlinear optical coefficients is one of the preconditions for using nonlinear optical materials in nonlinear optical devices. For a crystal, such large coefficients can be achieved by matching photon energies with…

Materials Science · Physics 2018-12-27 J. L. Cheng , J. E. Sipe , S. W. Wu , Chunlei Guo

Optical Kerr nonlinearity (n2) in n-type indium tin oxide (ITO) films coated on glass substrates has been measured using Z-scans with 200-fs laser pulses at wavelengths ranging from 720 to 780 nm. The magnitudes of the measured nonlinearity…

Materials Science · Physics 2009-11-11 Hendry Izaac Elim , Wei Ji , Furong Zhu

We report on the successful synthesis of highly conductive PdCoO2 ultrathin films on Al2O3 (0001) by pulsed laser deposition. The thin films grow along the c-axis of the layered delafossite structure of PdCoO2, corresponding to the…

Strongly Correlated Electrons · Physics 2018-04-24 T. Harada , K. Fujiwara , A. Tsukazaki

Two-dimensional (2D) noble-metal dichalcogenides have emerged as a new platform for the realization of versatile flat optics with a considerable degree of miniaturization. However, light field manipulation at the atomic scale is widely…

In this paper, we study the third-order nonlinear optical response due to transitions between excitonic levels in two-dimensional transition metal dichalcogeniedes. To accomplish this, we use methods not applied to the description of…

Mesoscale and Nanoscale Physics · Physics 2021-06-14 J. C. G. Henriques , Høgni C. Kamban , Thomas G. Pedersen , N. M. R. Peres

Single-layer semiconducting transition-metal dichalcogenides, lacking point inversion symmetry, provide an efficient platform for valleytronics, where the electronic, magnetic, valley and lattice degrees of freedom can be selectively…

Mesoscale and Nanoscale Physics · Physics 2024-11-19 Emmanuele Cappelluti , Habib Rostami , Federico Cilento

We present a detailed investigation on thickness-dependent third-order (\c{hi}^(3)) nonlinear optical properties of RF-sputtered WSe2 thin-films using ultrashort pulses centered at different excitation wavelengths. The single-beam Z-scan…

Thin films of noble-metal-based transition metal dichalcogenides, such as PtSe$_2$, have attracted increasing attention due to their interesting layer-number dependent properties and application potential. While it is difficult to cleave…

High-power optical pulses experience self-focusing when propagating in a gaseous medium due to the manifestation of the cubic (Kerr-like) nonlinearity. The magnitude of this effect depends on the Kerr nonlinearity coefficient n2, which in…

Optics · Physics 2025-08-22 Yury E. Geints , Victor O. Kompanets , Sergey V. Chekalin

Two-dimensional (2D) materials have become a fertile playground for the exploration and manipulation of novel collective electronic states. Recent experiments have unveiled a variety of robust 2D orders in highly-crystalline materials…

Using an enhanced optically heterodyned optical Kerr effect method and a theoretical description of the interactions between an optical beam, a single layer of graphene, and its substrate, we provide experimental answers to questions raised…

Optics · Physics 2017-12-20 Evdokia Dremetsika , Pascal Kockaert