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We compare the photoluminescence spectra of the low-temperature Mott insulator \etcl (T_{MIT}=40 K) with spectra of metallic \kappa-(BEDT-TTF)_2Cu[N(CN)_2]Br, which is superconducting below T_c=11.8 K, in the temperature range between 300…

Strongly Correlated Electrons · Physics 2013-09-17 N. Drichko , R. Hackl , J. A. Schlueter

Recent studies of organic molecular solids are highlighted by their complex phase diagram and light-induced phenomena, such as Mott insulator, spin liquid phase, and superconductivity. However, a discrepancy between experimental observation…

Strongly Correlated Electrons · Physics 2024-12-25 Dongbin Shin , Fabijan Pavošević , Nicolas Tancogne-Dejean , Michele Buzzi , Emil Viñas Boström , Angel Rubio

Superconductivity in organic conductors is often tuned by the application of chemical or external pressure. With this type of tuning, orbital overlaps and electronic bandwidths are manipulated, whilst the properties of the molecular…

The polarized optical reflectance spectra of the quasi two dimensional organic correlated electron system $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]$Y$, $Y =$ Br and Cl are measured in the infrared region. The former shows the…

Superconductivity · Physics 2007-05-23 T. Sasaki , I. Ito , N. Yoneyama , N. Kobayashi , N. Hanasaki , H. Tajima , T. Ito , Y. Iwasa

The magnetic susceptibility of the organic superconductors $\kappa$-(h8 or d8-ET)$_{2}$$X$, $X =$ Cu(NCS)$_{2}$ and Cu[N(CN)$_{2}$]Br has been studied. A metallic phase below $T^{*} =$ 37 $\sim$ 38 K for $X =$ Cu[N(CN)$_{2}$]Br and 46…

Superconductivity · Physics 2009-11-07 T. Sasaki , N. Yoneyama , A. Matsuyama , N. Kobayashi

We have studied the interlayer resistivity of the prototypical quasi-two-dimensional organic superconductor $\kappa$-(BEDT-TTF)$_2$Cu(NCS)$_2$ as a function of temperature, current and magnetic field, within the superconducting state. We…

Infrared reflection measurements of the half-filled two-dimensional organic conductors $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_{2}$]Br$_{x}$Cl$_{1-x}$ were performed as a function of temperature ($5 {\rm K}<T<300$ K) and Br-substitution ($x=0%$,…

A few organic conductors show a diversity of exciting properties like Mott insulating behaviour, spin liquid, antiferromagnetism, bad metal or unconventional superconductivity controlled by small changes in temperature, pressure or chemical…

Strongly Correlated Electrons · Physics 2014-02-05 Johannes Ferber , Kateryna Foyevtsova , Harald O. Jeschke , Roser Valenti

Partial suppression of superconductivity by fast cooling has been observed in the organic superconductor $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br by two means: a marked sample size effect on the magnetic susceptibility and direct imaging of…

Superconductivity · Physics 2007-05-23 N. Yoneyama , T. Sasaki , N. Kobayashi , Y. Ikemoto , H. Kimura

The interplane optical spectrum of the organic superconductor kappa-(BEDT-TTF)2Cu[N(CN)2]Br was investigated in the frequency range from 40 to 40,000 cm-1. The optical conductivity was obtained by Kramers-Kronig analysis of the reflectance.…

Superconductivity · Physics 2009-11-07 J. J. McGuire , T. Room , A. Pronin , T. Timusk , J. A. Schlueter , M. E. Kelly , A. M. Kini

We investigate superconductivity emerging in the photodoped Mott insulating Hubbard model using steady-state dynamical mean-field theory implemented on the real-frequency axis. By employing high-order strong-coupling impurity solvers, we…

Strongly Correlated Electrons · Physics 2026-02-20 Lei Geng , Aaram J. Kim , Philipp Werner

The fascinating electronic properties of the family of layered organic molecular crystals kappa-(BEDT-TTF)2X where X is an anion (e.g., X=I3, Cu[N(CN)2]Br, Cu(SCN)2) are reviewed. These materials are particularly interesting because of…

Strongly Correlated Electrons · Physics 2007-05-23 Ross H. McKenzie

Fluctuation spectroscopy is used to investigate the organic bandwidth-controlled Mott system $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Cl. We find evidence for percolative-type superconductivity in the spatially inhomogeneous coexistence region…

Strongly Correlated Electrons · Physics 2008-11-04 Jens Mueller , Jens Brandenburg , John A. Schlueter

We present an ab initio analysis for the ground-state properties of a correlated organic compound $\kappa$-(BEDT-TTF)2Cu(NCS)2. First, we derive an effective two-dimensional low-energy model from first principles, having short-ranged…

Strongly Correlated Electrons · Physics 2012-03-09 Hiroshi Shinaoka , Takahiro Misawa , Kazuma Nakamura , Masatoshi Imada

The magnetic field-induced superconductor-insulator-metal transition (SIMT) in partially deuterated $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br, which is just on the Mott boundary, has been observed using the infrared magneto-optical imaging…

The phase diagram of the layered organic superconductor $\kappa$-(ET)$_{2}$Cu[N(CN)$_{2}$]Cl has been accurately measured from a combination of $^{1}$H NMR and AC susceptibility techniques under helium gas pressure. The domains of stability…

Strongly Correlated Electrons · Physics 2009-10-31 S. Lefebvre , P. Wzietek , S. Brown , C. Bourbonnais , D. Jerome , C. Meziere , M. Fourmigue , P. Batail

We investigated the effect of magnetic field on the highly correlated metal near the Mott transition in the quasi-two-dimensional layered organic conductor, $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl, by the resistance measurements under…

Strongly Correlated Electrons · Physics 2009-11-10 F. Kagawa , T. Itou , K. Miyagawa , K. Kanoda

The first study of thermal conductivity, $\kappa$, in a quasi-two-dimensional organic superconductor of the $\kappa$-(BEDT-TTF)$_2$X family reveals features analogous to those already observed in the cuprates. The onset of superconductivity…

Superconductivity · Physics 2009-10-31 S. Belin , K. Behnia , A. Deluzet

We report the in-plane microwave surface impedance of a high quality single crystal of \kappa-(BEDT-TTF)2Cu[N(CN)2]Br. In the superconducting state, we find three independent signatures of d-wave pairing: i) a strong, linear temperature…

We study the superconducting transition temperature and the electronic properties of the metallic phase of $\kappa$-type (BEDT-TTF)$_2$X which shows unconventional properties in experiments, on the basis of the third order perturbation…

Superconductivity · Physics 2009-10-31 T. Jujo , S. Koikegami , K. Yamada
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