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The local density of optical states governs an emitters lifetime and quantum yield through the Purcell effect. It can be modified by a surface plasmon electromagnetic field, but such a field has a spatial extension limited to a few hundreds…

Mesoscale and Nanoscale Physics · Physics 2019-06-04 H. Lourenço-Martins , M. Kociak , S. Meuret , F. Treussart , Yih Hong Lee , Xing Yi Ling , H. C. Chang , L. H. G. Tizei

Hybrid polymer-plasmonic nanostructures might combine high enhancement of localized fields from metal nanoparticles with light confinement and long-range transport in subwavelength dielectric structures. Here we report on the complex…

The radiation dynamics of optical emitters can be manipulated by properly designed material structures providing high local density of photonic states, a phenomenon often referred to as the Purcell effect. Plasmonic nanorod metamaterials…

We show that plasmonic solid-state nanopores with tunable hole diameter can be prepared via a photocatalytic effect resulting from the enhanced electromagnetic field inside a metallic ring prepared on top of a dielectric nanotube. Under…

Plasmonic nanopores combine nanofluidic confinement with electromagnetic field enhancement, enabling optical interrogation of single molecules in sub-wavelength volumes. Yet, direct optical readout within these metallic geometries has…

We investigate the feasibility of CMOS-compatible optical structures to develop novel integrated spectroscopy systems. We show that local field enhancement is achievable utilizing dimers of plasmonic nanospheres that can be assembled from…

We develop a novel approach to ultrafast optical modulation of quantum-mechanical phenomena at the interface of plasmonic metals. Focusing on efficient and versatile nanoparticle-on-mirror plasmonic nanocavities, we discuss indirect control…

Optics · Physics 2026-03-17 Artur Avdizhiyan , Ilya Razdolski , Anton Yu. Bykov

Silicon vacancy (V$_{Si}$) centers in 4H-silicon carbide have emerged as a strong candidate for quantum networking applications due to their robust electronic and optical properties including a long spin coherence lifetime and bright,…

Quantum Physics · Physics 2024-07-09 Jae-Pil So , Jialun Luo , Jaehong Choi , Brendan McCullian , Gregory D. Fuchs

We develop a quantum master equation (QME) approach to investigate the electroluminesence (EL) of molecules confined between metallic electrodes and coupled to quantum plasmonic modes. Within our general state-based framework, we describe…

Mesoscale and Nanoscale Physics · Physics 2018-03-06 Justin P. Bergfield , Joshua R. Hendrickson

Nanoparticle (NP) arrays of noble metals strongly absorb light in the visible to infrared wavelengths through resonant interactions between the incident electromagnetic field and the metal's free electron plasma. Such plasmonic interfaces…

Mesoscale and Nanoscale Physics · Physics 2013-09-06 Miriam Israelowitz , Jennifer Amey , Tao Cong , Radhakrishna Sureshkumar

We experimentally demonstrate a Purcell effect-based design technique for improved impedance matching, and thus enhanced radiation efficiency from a small microwave emitter. Using an iterative process centred on comparing the phase of the…

Applied Physics · Physics 2022-09-29 L. D. Stanfield , A. W. Powell , S. A. R. Horsley , J. R. Sambles , A. P. Hibbins

Today's cutting-edge optical spectroscopic exploratory tools, such as Raman or infrared spectroscopy, rely on methods of signal enhancement as a route for their development. These methods are indispensable for substance identification and…

Photo-induced charge transport in plasmonic metal nanostructures has garnered significant interest for applications in sensing and power conversion, yet the underlying mechanisms remain debated. Here, we report spatially correlated…

We investigate the dynamics of a plasmonic oscillation over a metal nanoparticle when it is strongly coupled to a quantum emitter (e.g. quantum dot, molecule). We simulate the density matrix evolution for a simple model; coupled…

Optics · Physics 2013-08-27 Mehmet Emre Tasgin

We report direct evidence of enhanced spontaneous emission in a photonic crystal (PhC) light-emitting diode. The device consists of p-i-n heterojunction embedded in a suspended membrane, comprising a layer of self-assembled quantum dots.…

Other Condensed Matter · Physics 2009-11-13 M. Francardi , L. Balet , A. Gerardino , N. Chauvin , D. Bitauld , L. H. Li , B. Alloing , A. Fiore

Purcell-enhanced emission from a coupled emitter-cavity system is a fundamental manifestation of cavity quantum electrodynamics. Starting from a theoretical description we derive a scheme for photon emission from an emitter coupled to a…

Quantum Physics · Physics 2020-08-26 Thomas D. Barrett , Thomas H. Doherty , Axel Kuhn

Color centers in diamond play a central role in the development of quantum photonic technologies, and their importance is only expected to grow in the near future. For many quantum applications, high collection efficiency from individual…

We study amplified spontaneous emission (ASE) from wavelength-scale composite bodies--complicated arrangements of active and passive media--demonstrating highly directional and tunable radiation patterns, depending strongly on pump…

Mesoscale and Nanoscale Physics · Physics 2016-03-29 Weiliang Jin , Chinmay Khandekar , Adi Pick , Athanasios G. Polimeridis , Alejandro W. Rodriguez

We present an analytical model for plasmonic enhancement of metal photoluminescence (MPL) in metal nanostructures with characteristic size below the diffraction limit. In such systems, the primary mechanism of MPL enhancement is excitation…

Mesoscale and Nanoscale Physics · Physics 2023-08-01 Tigran V. Shahbazyan

We investigate surface plasmon amplification in a silver nanoparticle coupled to an externally driven three-level gain medium, and show that quantum coherence significantly enhances the generation of surface plasmons. Surface plasmon…

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