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This work theoretically investigates high-order harmonic generation in rare gas atoms driven by two temporally delayed ultrashort laser pulses. Apart from their temporal delay, the two pulses are identical. Using a single-atom model of the…

Relativistic surface high harmonics have been considered a unique source for the generation of intense isolated attosecond pulses in the extreme ultra-violet (XUV) and X-ray spectral range. However, its experimental realization is still a…

The development of schemes for coherent nonlinear time-domain spectroscopy in the extreme-ultraviolet regime (XUV) has so far been impeded by experimental difficulties that arise at these short wavelengths. In this work we present a novel…

We demonstrate a novel technique for producing high-order harmonics with designer spectral combs in the extreme ultraviolet-soft X-ray range for resonance applications using spectrally controlled visible lasers. Our approach enables…

The emission of above-ionization-threshold harmonics results from the recombination of two electron wavepackets moving along a "short" and a "long" trajectory in the atomic continuum. Attosecond pulse train generation has so far been…

Optics · Physics 2015-05-19 J. E. Kruse , P. Tzallas , E. Skantzakis , D. Charalambidis

We generate high-order harmonics in gaseous medium with tunable photon energy using time domain interferometry of double pulses in a non-collinear generation geometry. The method is based on the fact that the generated harmonics inherit…

We present the experimental realization of spectrally tunable, ultrashort, quasi-monochromatic extreme ultraviolet (XUV) pulses generated at 100 kHz repetition rate in a user-oriented gas high harmonic generation (GHHG) beamline of the…

A scheme to infer the temporal coherence of EUV frequency combs generated from intra-cavity high-order harmonic generation is put forward. The excitation dynamics of highly charged Mg-like ions, interacting with EUV pulse trains featuring…

Atomic Physics · Physics 2020-09-02 Chunhai Lyu , Stefano M. Cavaletto , Christoph H. Keitel , Zoltán Harman

We present the design, implementation and alignment procedure for a two-stage time delay compensating monochromator. The setup spectrally filters the radiation of a high-order harmonic generation source providing wavelength-selected XUV…

Ionization with ultrashort pulses in the extreme ultraviolet (XUV) regime can be used to prepare an ion in a superposition of spin--orbit substates. In this work, we study the coherence properties of such a superposition, created by…

Laser pulses with a duration of one femtosecond or shorter can be generated both in the IR-VIS and in the extreme UV, but the deep UV is a spectral region where such extremely short pulses have not yet been demonstrated. Here, a method for…

Optics · Physics 2019-01-24 Jan Reislöhner , Christoph Leithold , Adrian N. Pfeiffer

We present observations of the emission of XUV continua in the 20-37 eV region by high harmonic generation (HHG) with $4$-$7\ \mathrm{fs}$ pulses focused onto a Kr gas jet. The underlying mechanism relies on coherent control of the relative…

High harmonic generation (HHG) enables coherent extreme-ultraviolet (XUV) radiation with ultra-short pulse duration in a table-top setup. This has already enabled a plethora of applications. Nearly all of these applications would benefit…

Optics · Physics 2021-06-07 R. Klas , A. Kirsche , M. Gebhardt , J. Buldt , H. Stark , S. Hädrich , J. Rothhardt , J. Limpert

High harmonic generation (HHG) in gaseous media provides a robust method for producing coherent extreme-ultraviolet (EUV) radiation and attosecond pulses. However, the spectral and temporal properties of these pulses -- such as bandwidth…

Characterizing and controlling electronic properties of quantum materials require direct measurements of non-equilibrium electronic band structures over large regions of momentum space. Here, we demonstrate an experimental apparatus for…

We theoretically investigate the generation of intense keV attosecond pulses in an orthogonally polarized multicycle midinfrared two-color laser field. It is demonstrated that multiple continuum-like humps, which have a spectral width of…

Optics · Physics 2017-11-22 Guicun Li , Yinghui Zheng , Zhinan Zeng , Ruxin Li

We report the observation of multiple ionization of Argon through multi-XUV-photon absorption induced by an unprecedentedly powerful laser driven high-harmonic-generation source. Comparing the measured intensity dependence of the yield of…

We investigated the high-order harmonic generation by interacting time-delayed, linearly polarized bi-chromatic laser pulses with the atomic target. The frequency ratio of secondary to primary fields ($\omega_2/\omega_1$), along with the…

Atomic Physics · Physics 2023-04-26 Rambabu Rajpoot , Amol R. Holkundkar

We observe a new regime of coherent XUV radiation generation in noble gases induced by femtosecond pulses at very high intensities. This XUV emission has both a reduced divergence and spectral width as compared to high-order harmonic…

We describe a setup to study ultrafast dynamics in gas-phase molecules using time-resolved photoelectron and photoion spectroscopy. The vacuum ultraviolet (VUV) probe pulses are generated via strong field high-order harmonic generation from…

Atomic and Molecular Clusters · Physics 2014-04-14 Markus Koch , Thomas J. A. Wolf , Jakob Grilj , Emily Sistrunk , Markus Gühr
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