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A quantum spin liquid (QSL) would be an exotic stage for superconductivity. A promising candidate for a doped QSL is the organic triangular-lattice system, kappa-(BEDT-TTF)4Hg2:89Br8, which hosts a non-Fermi liquid and magnetism of a QSL…

Superconductivity · Physics 2022-06-16 K. Wakamatsu , Y. Ueno , K. Miyagawa , H. Taniguchi , K. Kanoda

Quantum spin liquid is a nontrivial magnetic state of longstanding interest, in which spins are strongly correlated and entangled but do not order1, 2; further intriguing is its doped version, which possibly hosts strange metal and…

Strongly Correlated Electrons · Physics 2023-07-12 K. Wakamatsu , Y. Suzuki , T. Fujii , K. Miyagawa , H. Taniguchi , K. Kanoda

Quantum spin liquid (QSL) is an exotic quantum phase of matter whose ground state is quantum-mechanically entangled without any magnetic ordering. A central issue concerns emergent excitations that characterize QSLs, which are…

Strongly Correlated Electrons · Physics 2018-05-08 Y. Tokiwa , T. Yamashita , D. Terazawa , K. Kimura , Y. Kasahara , T. Onishi , Y. Kato , M. Halim , P. Gegenwart , T. Shibauchi , S. Nakatsuji , E. -G. Moon , Y. Matsuda

It has been more than 40 years since superconductivity was discovered in organic conductors, and the way scientists view organic superconductors has changed over time. At first, the fact that organic conductors exhibit superconductivity was…

Superconductivity · Physics 2023-07-20 Hiroshi Oike , Hiromi Taniguchi , Kazuya Miyagawa , Kazushi Kanoda

Broad interest in quantum spin liquid (QSL) phases was triggered by the notion that they can be viewed as insulating phases with preexisting electron-pairs, such that upon light doping they might automatically yield superconductivity. Yet…

Strongly Correlated Electrons · Physics 2021-08-23 Hong-Chen Jiang

Quantum spin liquids (QSLs) are fluid-like states of quantum spins where its long-range ordered state is destroyed by quantum fluctuations. The ground state of QSL and its exotic phenomena, which have been extensively discussed for decades,…

Strongly Correlated Electrons · Physics 2011-10-25 Minoru Yamashita , Takasada Shibauchi , Yuji Matsuda

Beyond the conventional electron pairing mediated by phonons, high-temperature superconductivity in cuprates is believed to stem from quantum spin liquid (QSL). The unconventional superconductivity by doping a spin liquid/Mott insulator, is…

A quantum spin liquid (QSL) is an exotic insulating phase with emergent gauge fields and fractionalized excitations. However, the unambiguous demonstration of the existence of a QSL in a "non-engineered" microscopic model (or in any…

Strongly Correlated Electrons · Physics 2025-10-01 Xun Cai , Zhaoyu Han , Zi-Xiang Li , Steven A. Kivelson , Hong Yao

The original proposal to achieve superconductivity by starting from a quantum spin-liquid (QSL) and doping it with charge carriers, as proposed by Anderson in 1987, has yet to be realized. Here we propose an alternative strategy: use a QSL…

Strongly Correlated Electrons · Physics 2017-11-21 Jian-Huang She , Choong H. Kim , Craig J. Fennie , Michael J. Lawler , Eun-Ah Kim

Quantum spin liquids are exotic Mott insulators that carry extraordinary spin excitations and thus, when doped, expected to afford novel metallic states coupled to the unconventional magnetic excitations. The organic triangular-lattice…

Strongly Correlated Electrons · Physics 2025-01-07 H. Oike , Y. Suzuki , H. Taniguchi , K. Miyagawa , K. Kanoda

The Kitaev model belongs to an unconventional class of two-dimensional spin systems characterized by anisotropic, bond-dependent interactions that give rise to Quantum Spin Liquid (QSL) states. These exotic phases, marked by the absence of…

Strongly Correlated Electrons · Physics 2026-01-29 A. R. Moura , L. V. Santos

Organic solids host various electronic phases. Especially, a milestone compound of organic solid, $\beta'$-$X$[Pd(dmit)$_2$]$_2$ with $X$=EtMe$_3$Sb shows quantum spin-liquid (QSL) properties suggesting a novel state of matter. However,…

Strongly Correlated Electrons · Physics 2022-04-29 Kota Ido , Kazuyoshi Yoshimi , Takahiro Misawa , Masatoshi Imada

Quantum materials exhibiting magnetic frustration are connected to diverse phenomena including high-Tc superconductivity, topological order and quantum spin liquids (QSLs). A QSL is a quantum phase (QP) related to a quantum-entangled…

Strongly Correlated Electrons · Physics 2021-08-03 Samuel Mañas-Valero , Benjamin Huddart , Tom Lancaster , Eugenio Coronado , Francis Pratt

A quantum spin liquid (QSL) is a state of matter in which magnetic spins interact strongly, but quantum fluctuations inhibit long-range magnetic order even at zero temperature. A QSL has been predicted to have a host of exotic properties,…

A central challenge for understanding unconventional superconductivity in most strongly correlated electronic materials is their complicated band structure and presence of competing orders. In contrast, quasi-two-dimensional organic spin…

The organic conductor $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_{3}$ seems to form a quantum spin liquid, although at low temperatures unusual properties are seen in the charge, spin and lattice degrees of freedom. Here we report results of X-band…

Strongly Correlated Electrons · Physics 2015-06-22 K. G. Padmalekha , M. Blankenhorn , T. Ivek , L. Bogani , J. A. Schlueter , M. Dressel

We introduce and analyze a variational wave function for quasi two-dimensional kappa-ET organic salts containing strong local and nonlocal correlation effects. We find an unconventional superconducting ground state for intermediate charge…

Strongly Correlated Electrons · Physics 2009-11-10 Jun Liu , Joerg Schmalian , Nandini Trivedi

To reveal the nature of elementary excitations in a quantum spin liquid (QSL), we measured low temperature thermal conductivity and specific heat of 1T-TaS$_2$, a QSL candidate material with frustrated triangular lattice of spin-1/2. The…

Strongly Correlated Electrons · Physics 2020-02-05 H. Murayama , Y. Sato , X. Z. Xing , T. Taniguchi , S. Kasahara , Y. Kasahara , M. Yoshida , Y. Iwasa , Y. Matsuda

The superconductor to insulator or metal transition in two dimensions (2D) provides a valuable platform for studying continuous quantum phase transitions (QPTs) and critical phenomena. Distinct theoretical models, including both fermionic…

Paired state of nonstandard quasiparticles is analyzed in detail in two model situations. Namely, we consider the Cooper-pair bound state and the condensed phase of an almost localized Fermi liquid (ALFL) composed of quasiparticles in a…

Strongly Correlated Electrons · Physics 2010-01-28 Jan Kaczmarczyk , Jozef Spalek
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