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Accurate modeling of diffusive transport of nanoparticles across nanopores is a particularly challenging problem. The reason is that for such narrow pores the large surface-to-volume ratio amplifies the relevance of the nanoscopic details…

Mesoscale and Nanoscale Physics · Physics 2022-11-15 Andreas Baer , Paolo Malgaretti , Malte Kaspereit , Jens Harting , Ana-Suncana Smith

The interfaces between organic molecules and metal surfaces with layered antiferromagnetic order have gained increasing interests in the field of antiferromagnetic spintronics. The C60 layered AFM spinterfaces have been studied for C60…

Computational Physics · Physics 2016-10-27 Yangfan Shao , Rui Pang , Hui Pan , Xingqiang Shi

We investigate the static and dynamic behaviors of a Br adlayer electrochemically deposited onto single-crystal Ag(100) using an off-lattice model of the adlayer. Unlike previous studies using a lattice-gas model, the off-lattice model…

Materials Science · Physics 2015-06-24 S. J. Mitchell , Sanwu Wang , P. A. Rikvold

We use different semi-empirical dispersion correction schemes to assess the role of long-range van der Waals interactions in the adsorption of the prototypical molecular switch azobenzene (C6H5-N2-C6H5) at the coinage metal surfaces…

Materials Science · Physics 2011-06-20 Erik McNellis , Jorg Meyer , Karsten Reuter

Chemical interactions between two surfaces in contact play a crucial role in determining the mechanical and tribological behavior of solid interfaces. These interactions can be quantified via adhesion energy, that is a measure of the…

An analytical framework is proposed to describe the elasticity, viscosity and fragility of metallic glasses in relation to their atomic-level structure and the effective interatomic interaction. The bottom-up approach starts with forming an…

Soft Condensed Matter · Physics 2016-08-15 Alexandra E. Lagogianni , Johannes Krausser , Zach Evenson , Konrad Samwer , A Zaccone

We present a novel potential model for calculating the interaction between a molecule and a single graphene sheet. The dispersion/repulsion, induction, dipole-quadrupole, quadrupole-quadrupole interactions between a fluid molecule and a…

Mesoscale and Nanoscale Physics · Physics 2012-09-20 Xiongce Zhao

An extended theoretical study of interface potentials in adsorbed colloid-polymer mixtures is performed. To describe the colloid-polymer mixture near a hard wall, a simple Cahn-Nakanishi-Fisher free-energy functional is used. The bulk phase…

Soft Condensed Matter · Physics 2015-06-19 Jesper Koning , Yves Vandecan , Joseph Indekeu

The Casimir-Polder interaction of an atom with a metallic wall is investigated in the framework of the Lifshitz theory. It is demonstrated that in some temperature (separation) region the Casimir-Polder entropy takes negative values and…

Quantum Physics · Physics 2009-11-13 V. B. Bezerra , G. L. Klimchitskaya , V. M. Mostepanenko , C. Romero

Based on a microscopic density functional theory we calculate the internal structure of the three-phase contact line between liquid, vapor, and a confining wall as well as the morphology of liquid wetting films on a substrate exhibiting a…

Soft Condensed Matter · Physics 2009-10-31 C. Bauer , S. Dietrich

In this paper we use ab initio density functional theory (DFT) to calculate the electronic properties of C_50Cl_10. In comparison with the unstable C_50 which has a small t_lu(LUMO) - h_u(HOMO) energy gap and a high total free energy…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Steven W. D. Bailey , Colin J. Lambert

We consider the impingement of a droplet onto a wall with high impact speed. To model this process we favour a diffuse-interface concept. Precisely, we suggest a compressible Navier--Stokes--Allen--Cahn model. Basic properties of the model…

Fluid Dynamics · Physics 2019-09-30 Lukas Ostrowski , Christian Rohde

We studied the interaction between a single hydrogen atom and a single graphene using classical molecular dynamics simulation with modified Brenner REBO potential. Three interactions, which are adsorption, reflection, penetration, were…

Materials Science · Physics 2007-10-16 Atsushi Ito , Arimichi Takayama , Hiroaki Nakamura

This chapter begins with pure aluminium and a discussion of the form of the crystal structure and different unit cells that can be used to describe the crystal structure. Measurements of the face-centred cubic lattice parameter and thermal…

Materials Science · Physics 2020-02-06 Philip N. H. Nakashima

We report an investigation of the suitability of quantum embedding for modeling the effects of the environment on the X-ray photoelectron spectra of hydrogen chloride and the chloride ions adsorbed on ice surfaces, as well as of chloride…

Chemical Physics · Physics 2023-05-10 Richard Asamoah Opoku , Céline Toubin , André Severo Pereira Gomes

We present a theoretical study of wetting phenomena and interactions between liquid-vapor interfaces based on the density functional theory. The focus is mostly on the impact of long-range van der Waals interactions both within the fluid…

Chemical Physics · Physics 2011-11-10 Arik Yochelis , Len M. Pismen

The kinetics of sorption and subsequent desorption of argon gas by a C60 powder has been investigated in the temperature interval 58-290 K. The temperature dependence of the coefficients of Ar diffusion in fullerite has been obtained using…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 A. V. Dolbin , V. B. Esel'son , V. G. Gavrilko , V. G. Manzhelii , N. A. Vinnikov , R. M. Basnukaeva

We develop several configuration interaction approaches for characterizing the electronic structure of an adsorbate on a metal surface (at least in model form). When one can separate adsorbate from substrate, these methods can achieve a…

Chemical Physics · Physics 2020-02-26 Zuxin Jin , Wenjie Dou , Joseph E. Subotnik

Monte Carlo computer simulations with an embedded-atom potential are applied to study coherent gamma/gamma' interfaces in the Ni-Al system. The (100) interface free energy has been extracted from the power spectrum of equilibrium shape…

Materials Science · Physics 2019-06-11 Y. Mishin

We use an atom-atom potential between carbon atoms to obtain an interaction potential between nanotubes (assumed rigid), thereby calculating the cohesive energy of a bunch of nanotubes in hexagonal two dimensional packing. The model…

Materials Science · Physics 2007-05-23 V. K. Jindal , Shuchi Gupta , K. Dharamvir