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Due to its fast and high resolution characteristics, dual-comb spectroscopy has attracted an increasing amount of interest since its first demonstration. In the terahertz frequency range where abundant absorption lines (finger prints) of…

Broadband dual-comb spectroscopy (DCS) based on portable mode-locked fiber frequency combs is a powerful tool for in situ, calibration free, multi-species spectroscopy. While the acquisition of a single spectrum with mode-locked DCS…

Optics · Physics 2021-02-03 Nazanin Hoghooghi , Ryan K. Cole , Gregory B. Rieker

Dual-comb spectroscopy (DCS) utilizes a pair of broadband mutually coherent laser frequency combs to enable high-resolution, high-accuracy spectroscopic measurements with atomic-clock-level frequency referencing, and rapid, multiplexed…

Optics · Physics 2025-10-01 D. Konnov , A. Muraviev , K. L. Vodopyanov

Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of…

Open-path dual-comb spectroscopy (DCS) significantly enhances our understanding of regional trace gases. However, due to technical challenges, cost considerations, and eye-safety regulations, its sensing range and flexibility remain…

Optical two-dimensional coherent spectroscopy (2DCS) has become a powerful tool for studying energy level structure, dynamics, and coupling in many systems including atomic ensembles. Various types of two-dimensional (2D) spectra, including…

Atomic Physics · Physics 2022-05-25 Jieli Yan , Stephen Revesz , Danfu Liang , Hebin Li

Chiral molecules show differences in their chemical and optical properties due to different spatial arrangements of the atoms in the two enantiomers. A common way to optically differentiate them is to detect the disparity in the absorption…

Double-quantum two-dimensional coherent spectroscopy (MDCS) is a powerful optical method that is used to study optical properties of atomic and complex molecular systems and semiconductor materials. Double-quantum 2D spectra and…

Optics · Physics 2020-10-21 Bachana Lomsadze , Steven T. Cundiff

The detection of light of thermal origin is the principal means by which humanity has learned about our world and the cosmos. In optical astronomy, in particular, direct detection of thermal photons and the resolution of their spectra have…

Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…

With the advent of laser frequency combs, coherent light sources that offer equally-spaced sharp lines over a broad spectral bandwidth have become available. One decade after revolutionizing optical frequency metrology, frequency combs hold…

On-chip spectroscopy that could realize real-time fingerprinting with label-free and high-throughput detection of trace molecules is one of the 'holy grails" of sensing. Such miniaturized spectrometers would greatly enable applications in…

The sensitivity of molecular fingerprinting is dramatically improved when placing the absorbing sample in a high-finesse optical cavity, thanks to the large increase of the effective path-length. As demonstrated recently, when the…

Dual-comb spectroscopy utilizes two sets of comb lines with slightly different comb-tooth-spacings, and optical spectral information is acquired by measuring the radio-frequency beat notes between the sets of comb lines. It holds the…

Optics · Physics 2016-09-13 Xin Zhao , Guoqing Hu , Bofeng Zhao , Cui Li , Yingling Pan , Ya Liu , Takeshi Yasui , Zheng Zheng

Measurements of ultrahigh-fidelity absorption spectra can help validate quantum theory, engineer ultracold chemistry, and remotely sense atmospheres. Recent achievements in cavity-enhanced spectroscopy using either frequency-based…

Optics · Physics 2020-01-24 A. Cygan , A. J. Fleisher , R. Ciuryło , K. A. Gillis , J. T. Hodges , D. Lisak

Hyperspectral imaging provides spatially resolved spectral information. Utilising dual frequency combs as active illumination sources, hyperspectral imaging with ultra-high spectral resolution can be implemented in a scan-free manner when a…

We present a new type of dual optical frequency comb source capable of scaling applications to high measurement speeds while combining high average power, ultra-low noise operation, and a compact setup. Our approach is based on a…

Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…

Optics · Physics 2015-05-18 I. Coddington , W. C. Swann , N. R. Newbury

Dual-comb spectroscopy (DCS) is useful for gas spectroscopy due to high potential of optical frequency comb (OFC). However, fast Fourier transform (FFT) calculation of a huge amount of temporal data spends significantly longer time than the…

Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent…