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We have investigated the exciton dynamics in transition metal dichalcogenide mono-layers using time-resolved photoluminescence experiments performed with optimized time-resolution. For MoSe2 monolayers, we measure $\tau_{rad}=1.8\pm0.2$ ps…

Materials Science · Physics 2016-05-18 C. Robert , D. Lagarde , F. Cadiz , G. Wang , B. Lassagne , T. Amand , A. Balocchi , P. Renucci , S. Tongay , B. Urbaszek , X. Marie

We revisit and extend the standard bosonic interpretation of interlayer excitons in the moir\'e potential of twisted heterostructures of transition-metal dichalcogenides. In our experiments, we probe a high quality MoSe$_2$/WSe$_2$ van der…

Integrating 2D materials into high-quality optical microcavities opens the door to fascinating many-particle phenomena including the formation of exciton-polaritons. These are hybrid quasi-particles inheriting properties of both the…

Mesoscale and Nanoscale Physics · Physics 2024-01-10 Beatriz Ferreira , Roberto Rosati , Jamie M. Fitzgerald , Ermin Malic

Monolayer transition metal dichalcogenides (TMDs) are characterized by relatively large carrier effective masses and suppressed screening of the Coulomb interaction, which substantially enhances the correlation effects in these structures.…

Strong Coulomb interactions in single-layer transition metal dichalcogenides (TMDs) result in the emergence of strongly bound excitons, trions and biexcitons. These excitonic complexes possess the valley degree of freedom, which can be…

Heterostructures of transition metal dichalcogenides (TMDs) offer unique opportunities in optoelectronics due to their strong light-matter interaction and the formation of dipolar interlayer excitons. Introducing a twist angle or lattice…

Optics · Physics 2025-09-16 Giuseppe Meneghini , Samuel Brem , Ermin Malic

The moir\'e pattern, which emerges due to a relative rotation between two monolayers of transition metal dichalcogenides, features a long lattice period for small twist angles. The resulting band structure modulation acts as an effective…

Excitons dominate the optics of atomically-thin transition metal dichalcogenides and 2D van der Waals heterostructures. Interlayer 2D excitons, with an electron and a hole residing in different layers, form rapidly in heterostructures…

Mesoscale and Nanoscale Physics · Physics 2021-04-20 M. G. Burdanova , M. Liu , M. Staniforth , Y. Zheng , R. Xiang , S. Chiashi , A. Anisimov , E. I. Kauppinen , S. Maruyama , J. Lloyd-Hughes

We present a unified description of the excitonic properties of four monolayer transition-metal dichalcogenides (TMDC's) using an equation of motion method for deriving the Bethe-Salpeter equation in momentum space. Our method is able to…

Mesoscale and Nanoscale Physics · Physics 2017-08-08 A. J. Chaves , R. M. Ribeiro , T. Frederico , N. M. R. Peres

Reduced dielectric screening in two-dimensional materials enables bound excitons, which modifies their optical absorption and optoelectronic response even at room temperature. Here, we demonstrate the existence of excitons in the bandgap of…

Mesoscale and Nanoscale Physics · Physics 2022-07-12 Pushpendra Yadav , Bramhachari Khamari , Bahadur Singh , K. V. Adarsh , Amit Agarwal

We present here a formalism based on time-dependent density-functional theory (TDDFT) to describe characteristics of both intra- and inter-valley excitons in semiconductors, the latter of which had remained a challenge. Through the usage of…

Materials Science · Physics 2023-05-10 Jia Shi , Volodymyr Turkowski , Duy Le , Talat S. Rahman

When doped with a high density of mobile charge carriers, monolayer transition-metal dichalcogenide (TMD) semiconductors can host new types of composite many-particle exciton states that do not exist in conventional semiconductors. Such…

Mesoscale and Nanoscale Physics · Physics 2024-11-22 J. Choi , J. Li , D. Van Tuan , H. Dery , S. A. Crooker

We present a first-principles investigation of the electronic and optical properties of hybrid organic-inorganic interfaces consisting of MoS$_2$ monolayer and the $\pi$-conjugate molecules pyrene and pyridine. For both hybrid systems, the…

Materials Science · Physics 2021-12-16 Ignacio Gonzalez Oliva , Fabio Caruso , Pasquale Pavone , Claudia Draxl

Monolayer transition-metal dichalcogenides (TMDs) provide a platform for realizing Wigner crystals and enable their detection via exciton spectroscopy. We develop a microscopic theoretical model for excitons interacting with the localized…

Strongly Correlated Electrons · Physics 2025-12-22 Haydn S. Adlong , Eugen Dizer , Richard Schmidt , Atac Imamoglu , Arthur Christianen

Moir\'e heterostructures are rapidly emerging as a tunable platform to study correlated electronic phenomena. Discovery of exotic quantum phases in moir\'e systems requires novel probes of charge and spin order. Unlike detection schemes…

Mesoscale and Nanoscale Physics · Physics 2021-11-19 Weijie Li , Luka M. Devenica , Jin Zhang , Yang Zhang , Xin Lu , Kenji Watanabe , Takashi Taniguchi , Angel Rubio , Ajit Srivastava

The optical properties of atomically thin transition metal dichalcogenide (TMDC) semiconductors are shaped by the emergence of correlated many-body complexes due to strong Coulomb interaction. Exceptional electron-hole exchange predestines…

Monolayer transition metal dichalcogenides host a variety of optically excited quasiparticles species that stem from two-dimensional confinement combined with relatively large carrier effective masses and reduced dielectric screening. The…

Transitions metal dichalcogenides (TMDs) are direct semiconductors in the atomic monolayer (ML) limit with fascinating optical and spin-valley properties. The strong optical absorption of up to 20 % for a single ML is governed by excitons,…

Mesoscale and Nanoscale Physics · Physics 2018-09-26 B. Han , C. Robert , E. Courtade , M. Manca , S. Shree , T. Amand , P. Renucci , T. Taniguchi , K. Watanabe , X. Marie , L. E. Golub , M. M. Glazov , B. Urbaszek

Atomically thin layered two dimensional (2D) material has provided a rich library for both fundamental research and device applications. One of the special advantages is that, bandgap engineering and controlled material response can be…

Mesoscale and Nanoscale Physics · Physics 2019-12-02 Yuanda Liu , Hanlin Fang , Abdullah Rasmita , Yu Zhou , Juntao Li , Ting Yu , Qihua Xiong , Nikolay Zheludev , Jin Liu , Weibo Gao

Transition metal dichalcogenide heterobilayers offer attractive opportunities to realize lattices of interacting bosons with several degrees of freedom. Such heterobilayers can feature moir\'e patterns that modulate their electronic band…

Mesoscale and Nanoscale Physics · Physics 2021-08-16 Mauro Brotons-Gisbert , Hyeonjun Baek , Aidan Campbell , Kenji Watanabe , Takashi Taniguchi , Brian D. Gerardot