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Non-resonant second harmonic generation phase and amplitude measurements obtained from the silica:water interface at varying pH and 0.5 M ionic strength point to the existence of a nonlinear susceptibility term, which we call chi(3)X, that…

We perform molecular dynamics simulations of ionic liquids confined between graphene walls under a large variety of conditions (pure ionic liquids, mixtures with water and alcohols, mixtures with lithium salts and defective graphene walls).…

Ion specific outcomes at aqueous interfaces remain among the most enigmatic phenomena in interfacial chemistry. Here, charged fused silica/water interfaces have been probed by homodyne- and heterodyne-detected (HD) second harmonic…

Chemical Physics · Physics 2019-05-13 Mavis D. Boamah , Paul E. Ohno , Emilie Lozier , Jacqueline Van Ardenne , Franz M. Geiger

Second harmonic generation (SHG) spectroscopy has been applied to probe the fused silica/water interface at pH 7 and the uncharged 11bar02 sapphire/water interface at pH 5.2 in contact with aqueous solutions of NaCl, NaBr, NaI, KCl, RbCl,…

Materials Science · Physics 2018-03-28 Mavis D. Boamah , Paul E. Ohno , Franz M. Geiger , Kenneth B. Eisenthal

Surface X-ray scattering studies of electrochemical Stern layer are reported. The Stern layers formed at the interfaces of RuO2 (110) and (100) in 0.1 M CsF electrolyte are compared to the previously reported Stern layer on Pt(111) [Liu et…

We report new experimental results on the generation and dynamics of multiple double layers in front of a positively biased electrode immersed in a DP-machine plasma. Depending on the geometry or the dimensions of the electrode, this…

Recently the reversible heat production during the electric double layer (EDL) buildup in a sodium chloride solution was measured experimentally [Janssen et al., Phys. Rev. Lett. 119, 166002 (2017)] and matched with theoretical predictions…

Soft Condensed Matter · Physics 2022-01-24 Philipp Pelagejcev , Fabian Glatzel , Andreas Härtel

In moir\'e crystals resulting from the stacking of twisted two-dimensional (2D) layered materials, a subtle adjustment in the twist angle surprisingly gives rise to a wide range of correlated optical and electrical properties. Herein, we…

We investigate the hydrodynamic stability and the formation of patterns in a continuum model of epithelial layers, able to account for the interplay between mechanical activity, lateral adhesion and the $6-$fold orientational order…

Soft Condensed Matter · Physics 2025-02-19 Josep-Maria Armengol-Collado , Leonardo Puggioni , Livio N. Carenza , Luca Giomi

Morphological instability of the solid-liquid interface occuring in a crystal growing from an undercooled thin liquid being bounded on one side by a free surface and flowing down inclined plane is investigated by a linear stability analysis…

Materials Science · Physics 2009-11-10 K. Ueno

Previously, using an incompressible von K\'arm\'an-Howarth formalism, the behavior of cross-scale energy transfer in magnetic reconnection and turbulence was found to be essentially identical to each other, independent of an external…

We calculate the ion distributions around an interface in fluid mixtures of highly polar and less polar fluids (water and oil) for two and three ion species. We take into account the solvation and image interactions between ions and…

Soft Condensed Matter · Physics 2009-11-13 Akira Onuki

We consider the elastic scattering of electrons by hydrogen atoms in the presence of a two-color circularly polarized laser field in the domain of moderate intensities below $10^{13}$ W/cm$^2$ and high projectile energies. A hybrid approach…

Atomic Physics · Physics 2023-06-16 Gabriela Buica

We explore by means of modeling how absorptive-dispersive mixing between the second- and third-order terms modify the imaginary chi(2)total responses from air/water interfaces under conditions of varying charge densities and ionic strength.…

Other Condensed Matter · Physics 2018-07-04 Paul Ohno , Hong-fei Wang , James Skinner , Francesco Paesani , Franz M. Geiger

We study transition to phase synchronization in an ensemble of Stuart-Landau oscillators interacting on a star network. We observe that by introducing frequency weighted coupling and time scale variations in the dynamics of nodes, system…

Chaotic Dynamics · Physics 2022-09-14 Anjuman Ara Khatun , Ruby Varshney and , Haider Hasan Jafri

This work focuses on the evolution of structure and stress for an experimental system of 2D photoelastic particles that is subjected to multiple cycles of pure shear. Throughout this process, we determine the contact network and the contact…

Soft Condensed Matter · Physics 2009-06-16 J. Zhang , T. S. Majmudar , A. Tordesillas , R. P. Behringer

The structure of ionic adsorption layers is studied via a proper thermodynamic treatment of the electrostatic and non-electrostatic interactions between the surfactant ions as well as of the effect of thermodynamic non-locality. The…

Soft Condensed Matter · Physics 2014-10-28 R. Tsekov

Recent advances in experimental and computational techniques have allowed for an accurate description of the adsorption of ionic liquids on metallic electrodes. It is now well established that they adopt a multi-layered structure, and that…

Materials Science · Physics 2016-03-15 Benjamin Rotenberg , Mathieu Salanne

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

This paper is the first part of a two-fold study of mixing, i.e. the formation of layers and upwelling of buoyancy, in axially stratified Taylor--Couette flow, with fixed outer cylinder. Using linear analysis and direct numerical…

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