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The magnetic structure of Ca$_2$MnReO$_6$ double perovskite is investigated by neutron powder diffraction and bulk magnetization, showing dominant non-collinear Mn magnetic moments [$4.35(7)$ $\mu_B$] that are orthogonally aligned with the…

Strongly Correlated Electrons · Physics 2018-03-01 A. S. Cavichini , M. T. Orlando , J. B. Depianti , J. L. Passamai , F. Damay , F. Porcher , E. Granado

This article contains a theoretical overview of the physical properties of antiferromagnetic Mott insulators in spatial dimensions greater than one. Many such materials have been experimentally studied in the past decade and a half, and we…

Strongly Correlated Electrons · Physics 2009-11-10 Subir Sachdev

The magnetic properties and structure of LixCoO2 for x between 0.5 and 1.0 are reported. Co4+ is found to be high-spin in LixCoO2 for x between 0.94 and 1.0 and low-spin for x between 0.50 and 0.78. Weak antiferromagnetic coupling is…

Strongly Correlated Electrons · Physics 2009-02-12 J. T. Hertz , Q. Huang , T. McQueen , T. Klimczuk , J. W. G. Bos , L. Viciu , R. J. Cava

Multiferroicity and magnetodielectric coupling in metal-organic-frameworks (MOFs) is rare and so far restricted mainly to formate-based systems with perovskite structure. In the course of this work we designed a tetragonal framework…

Materials Science · Physics 2017-10-31 Tathamay Basu , A. Jesche , B. Bredenkotter , M. Grzywa , D. Denysenko , D. Volkmer , A. Loidl , S. Krohns

The ordered tetragonal intermetallic Cr$_2$Al forms the same structure type as Mn$_2$Au, and the latter has been heavily investigated for its potential in antiferromagnetic spintronics due to its degenerate in-plane N\'{e}el vector. We…

Materials Science · Physics 2022-01-20 Chengxi Zhao , Kisung Kang , Joerg C. Neuefeind , Andre Schleife , Daniel P. Shoemaker

Motivated by the absence of cooperative Jahn-Teller effect and of magnetic ordering in LiNiO$_2$, a layered oxide with triangular planes, we study a general spin-orbital model on the triangular lattice. A mean-field approach reveals the…

Strongly Correlated Electrons · Physics 2009-11-10 F. Vernay , K. Penc , P. Fazekas , F. Mila

While both La$_{0.7}$Sr$_{0.3}$MnO$_3$ and La$_{0.7}$Sr$_{0.3}$CoO$_3$ are ferromagnets with metallic conductivity below $T_\mathrm{c}$ (360K and 220K, respectively), partial substitutions of Co by Mn in…

Materials Science · Physics 2007-05-23 D. N. H. Nam , L. V. Bau , N. V. Khiem , L. H. Son , N. X. Phuc

First principles calculations of the O surfaces of Co-ZnO show that substitutional Co ions develop large magnetic moments which long-range coupling depends on their mutual distance. The local spin polarization induced at the O atoms is…

Materials Science · Physics 2009-11-13 N. Sanchez , S. Gallego , M. C. Munoz

Using a combination of single-crystal neutron scattering and reverse Monte Carlo refinements, we study the magnetic structure of paramagnetic MnO at a temperature (160\,K) substantially below the Curie-Weiss temperature…

Resonant soft x-ray diffraction has been used to probe the temperature dependent orbital and magnetic structure of $\mathrm{LaSr_{2}Mn_{2}O_7}$. Previous crystallographic studies have shown that this material has almost no MnO$_{6}$ oxygen…

Strongly Correlated Electrons · Physics 2007-05-23 S. B. Wilkins , N. Stojic , T. A. W. Beale , N. Binggeli , P. Bencok , S. Stanescu , J. F. Mitchell , P. Abbamonte , P. D. Hatton , M. Altarelli

The effect of uniaxial strain on electronic structure and magnetism in LaMnO$_3$ is studied from a model Hamiltonian that illustrates the competition between the Jahn-Teller, super exchange, and double exchange interactions. We retain in…

Materials Science · Physics 2010-12-07 B. R. K. Nanda , S. Satpathy

Magnetic ordering of itinerant fermionic systems is at the forefront of condensed matter physics dating back to Stoner's instability. Spin-orbit coupling (SOC) which couples two essential ingredients of an itinerant fermionic system, namely…

Quantum Gases · Physics 2016-09-13 Shang-Shun Zhang , Jinwu Ye , Wu-Ming Liu

Motivated by studies of coexisting electron correlation and spin-orbit coupling effect in Na$_2$IrO$_3$ and a recent experiment of its 4d analogue Li$_2$RhO$_3$, we performed first-principles calculations of the rhodium oxide compound. The…

Strongly Correlated Electrons · Physics 2013-03-20 Chao Cao , Yongkang Luo , Zhuan Xu , Jianhui Dai

Two-dimensional magnetic materials provide an ideal platform to explore collective many-body excitations associated with spin fluctuations. In particular, it should be feasible to explore, manipulate and ultimately design magnonic…

Mesoscale and Nanoscale Physics · Physics 2023-04-27 Somesh Chandra Ganguli , Markus Aapro , Shawulienu Kezilebieke , Mohammad Amini , Jose L. Lado , Peter Liljeroth

Monolayer MnO$_2$ is one of the few predicted two-dimensional (2D) ferromagnets that has been experimentally synthesized and is commercially available. The Mermin-Wagner theorem states that magnetic order in a 2D material cannot persist…

Strongly Correlated Electrons · Physics 2022-03-28 Daniel Wines , Kayahan Saritas , Can Ataca

Using an effective Hamiltonian of mutiferroic BiFeO$_3$ (BFO) as a toy model, we explore the effect of the coefficient, C, characterizing the strength of the spin-current interaction, on physical properties. We observe that for larger C…

Materials Science · Physics 2013-12-17 Satadeep Bhattacharjee , Dovran Rahmedov , Dawei Wang , Laurent Bellaiche

We show that the off-diagonal exchange anisotropy drives Mott insulators with strong spin-orbit coupling to a classical spin liquid regime, characterized by an infinite number of ground states and Ising variables living on closed or open…

Strongly Correlated Electrons · Physics 2017-04-07 Ioannis Rousochatzakis , N. B. Perkins

We report a first-order phase transition at T_M=357 K in single crystal Ca_2RuO_4, an isomorph to the superconductor Sr_2RuO_4. The discontinuous decrease in electrical resistivity signals the near destruction of the Mott insulating phase…

Strongly Correlated Electrons · Physics 2009-10-31 C. S. Alexander , G. Cao , V. Dobrosavljevic , E. Lochner , S. McCall , J. E. Crow , R. P. Guertin

The standard view is that at low energies Mott insulators exhibit only magnetic properties while charge degrees of freedom are frozen out as the electrons become localized by a strong Coulomb repulsion. We demonstrate that this is in…

Strongly Correlated Electrons · Physics 2009-11-13 L. N. Bulaevskii , C. D. Batista , M. Mostovoy , D. Khomskii

Using ab initio calculations, we have investigated an insulating tetragonally distorted perovskite BaCrO$_3$ with a formal $3d^2$ configuration, the volume of which is apparently substantially enhanced by a strain due to SrTiO$_3$…

Strongly Correlated Electrons · Physics 2014-11-24 Hyo-Sun Jin , Kyo-Hoon Ahn , Myung-Chul Jung , K. -W. Lee