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The effects of pressure on a quantum spin liquid are investigated in an organic Mott insulator $\kappa$-(ET)$_2$Ag$_2$(CN)$_3$ with a spin-1/2 triangular lattice. The application of negative chemical pressure to…

Pyrochlore magnets have proven to provide an excellent arena for the realization of a variety of many-body phenomena such as classical and quantum order-by-disorder, as well as spin liquid phases described by emergent gauge field theories.…

Strongly Correlated Electrons · Physics 2025-02-21 Niccolò Francini , Lukas Janssen , Daniel Lozano-Gómez

Exchange interaction tends to favor collinear or coplanar magnetic orders in rotationally invariant spin systems. Indeed, such magnetic structures are usually selected by thermal or quantum fluctuations in highly frustrated magnets. Here we…

Strongly Correlated Electrons · Physics 2010-11-25 Gia-Wei Chern

$^{1}$H NMR and static susceptibility measurements have been performed in an organic Mott insulator with nearly isotropic triangular lattice, $\kappa$-(BEDT-TTF)$_{2}$Cu$_{2}$(CN)$_{3}$, which is a model system of frustrated quantum spins.…

Strongly Correlated Electrons · Physics 2009-11-10 Y. Shimizu , K. Miyagawa , K. Kanoda , M. Maesato , G. Saito

Recently, a number of experiments indicate the possible presence of spin liquid phases in quantum magnets with spin-1/2 and spin-1 moments sitting on triangular-lattice-based structures in Ba3CuSb2O9 and Ba3NiSb2O9 respectively. In relation…

Strongly Correlated Electrons · Physics 2013-06-04 Kyusung Hwang , Tyler Dodds , Subhro Bhattacharjee , Yong Baek Kim

The interplay between spin frustration and charge fluctuation gives rise to an exotic quantum state in the intermediate-interaction regime of the half-filled triangular-lattice Hubbard model, while the nature of the state is under debate.…

Strongly Correlated Electrons · Physics 2022-10-05 Bin-Bin Chen , Ziyu Chen , Shou-Shu Gong , D. N. Sheng , Wei Li , Andreas Weichselbaum

Quantum spin liquids attract great interest due to their exceptional magnetic properties characterized by the absence of long-range order down to low temperatures despite the strong magnetic interaction. Commonly, these compounds are…

Strongly Correlated Electrons · Physics 2018-05-01 Martin Dressel , Andrej Pustogow

The dimer Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ exhibits unusual electrodynamic properties. Numerical investigations of the electronic ground state and the molecular and lattice vibrations reveal the importance of the…

Strongly Correlated Electrons · Physics 2016-02-02 M. Dressel , P. Lazic , A. Pustogow , E. Zhukova , B. Gorshunov , J. A. Schlueter , O. Milat , B. Gumhalter , S. Tomic

Using synchrotron X-rays and neutron diffraction we disentangle spin-lattice order in highly frustrated ZnCr$_2$O$_4$ where magnetic chromium ions occupy the vertices of regular tetrahedra. Upon cooling below 12.5 K the quandary of…

Strongly Correlated Electrons · Physics 2009-05-14 S. Ji , S. -H. Lee , C. Broholm , T. Y. Koo , W. Ratcliff , S-W. Cheong , P. Zschack

We have discovered a novel candidate for a spin liquid state in a ruthenium oxide composed of dimers of $S = $ 3/2 spins of Ru$^{5+}$,Ba$_3$ZnRu$_2$O$_9$. This compound lacks a long range order down to 37 mK, which is a temperature…

Spirals and helices are common motifs of long-range order in magnetic solids, and they may also be organized into more complex emergent structures such as magnetic skyrmions and vortices. A new type of spiral state, the spiral spin-liquid,…

We study the quantum phase transition between the $Z_2$ spin liquid and valence bond solid (VBS) orders on a triangular lattice. With a fully isotropic triangular lattice, the transition from a columnar or resonating-plaquette VBS order can…

Strongly Correlated Electrons · Physics 2015-06-16 Kevin Slagle , Cenke Xu

For certain crystalline systems, most notably the organic compound EtMe3Sb[Pd(dmit)2]2, experimental evidence has accumulated of an insulating state with a high density of gapless neutral excitations that produce Fermi-liquid-like power…

Strongly Correlated Electrons · Physics 2013-04-09 Maissam Barkeshli , Hong Yao , Steven A. Kivelson

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

Strongly Correlated Electrons · Physics 2019-07-02 A. Zorko , M. Pregelj , M. Klanjšek , M. Gomilšek , Z. Jagličić , J. S. Lord , J. A. T. Verezhak , T. Shang , W. Sun , J. -X. Mi

Recent experiments on the organic compound \kappa-(ET)_2Cu_2(CN)_3 have provided a promising example of a two dimensional spin liquid state. This phase is described by a two-dimensional spinon Fermi sea coupled to a U(1) gauge field. We…

Strongly Correlated Electrons · Physics 2009-11-13 Victor Galitski , Yong Baek Kim

In this paper we present a study of magnetic order of quantum Heisenberg spins on pyrochlore type lattices: a lattice of corner sharing tetrahedra. We use the Cluster Variation Approximation with the tetrahedron as basic cluster. We find…

Strongly Correlated Electrons · Physics 2007-05-23 Wiebe Geertsma

We propose a variant of the antiferromagnetic XY model on the triangular lattice to study the interplay between the chiral and nematic orders in addition to the magnetic order. The model has a significant bi-quadratic interaction of the…

Strongly Correlated Electrons · Physics 2009-11-13 Jin-Hong Park , Shigeki Onoda , Naoto Nagaosa , Jung Hoon Han

The collective behavior of interacting magnetic moments can be strongly influenced by the topology of the underlying lattice. In geometrically frustrated spin systems, interesting chiral correlations may develop that are related to the spin…

Strongly Correlated Electrons · Physics 2007-05-23 D. Grohol , K. Matan , J. H. Cho , S. -H. Lee , J. W. Lynn , D. G. Nocera , Y. S. Lee

Utilizing infrared vibrational spectroscopy we have investigated dimerized two-dimensional organic salts in order to search for possible charge redistribution that might cause electronic dipoles and ferroelectricity: the quantum spin liquid…

Strongly Correlated Electrons · Physics 2012-12-19 Katrin Sedlmeier , Sebastian Elsasser , Rebecca Beyer , Dan Wu , Tomislav Ivek , Silvia Tomic , John A. Schlueter , Martin Dressel

Geometrical frustration, quantum entanglement and disorder may prevent long-range order of localized spins with strong exchange interactions, resulting in a novel state of matter. $\kappa$-(BEDT-TTF)$_2$-Cu$_2$(CN)$_3$ is considered the…