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In the last few decades, ultrafast demagnetization elicited by ultrashort laser pulses has been the subject of a large body of work that aims to better understand and control this phenomenon. Although specific magnetic materials' properties…

We present a comprehensive experimental and numerical study of magnetization dynamics triggered in a thin metallic film by single-cycle terahertz pulses of $\sim20$ MV/m electric field amplitude and $\sim1$ ps duration. The experimental…

In past decades, ultrafast spin dynamics in magnetic systems have been associated with heat deposition from high energy laser pulses, limiting the selective access to spin order. Here we use a long wavelength terahertz pump optical probe…

Materials Science · Physics 2021-06-04 Hovan Lee , Cedric Weber , Manfred Fähnle , Mostafa Shalaby

We explore the impact of optical excitation using two interfering ultrashort optical pulses on ultrafast magnetization dynamics. Our investigation focuses on Pt/Co/Pt multilayers and TbCo alloy samples, employing a dual pump approach. We…

We theoretically investigate spin-dependent carrier dynamics due to the electron-phonon interaction after ultrafast optical excitation in ferromagnetic metals. We calculate the electron-phonon matrix elements including the spin-orbit…

Materials Science · Physics 2015-05-30 Sven Essert , Hans Christian Schneider

Irradiating a ferromagnetic material with an ultrashort laser pulse leads to demagnetization on a femtosecond timescale. We implement Elliott-Yafet type spin-flip scattering, mediated by electron-electron and electron-phonon collisions,…

Materials Science · Physics 2011-08-29 Benedikt Y. Mueller , T. Roth , M. Cinchetti , M. Aeschlimann , B. Rethfeld

We have performed a two-color time-resolved magneto-optical Kerr effect (MOKE) study of a ferromagnetic InMnAs/GaSb heterostructure. We observed ultrafast photo-induced changes in the MOKE signal induced by a large density of spin-polarized…

Materials Science · Physics 2007-05-23 J. Wang , G. A. Khodaparast , J. Kono , T. Slupinski , A. Oiwa , H. Munekata

Time-resolved magneto-optical Kerr spectroscopy of ferromagnetic InMnAs reveals two distinct {\em demagnetization} processes -- fast ($<1$ ps) and slow ($\sim$100 ps). Both components diminish with increasing temperature and are absent…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. Wang , C. Sun , J. Kono , A. Oiwa , H. Munekata , L. Cywinski , L. J. Sham

Ultrashort optical pulses are a cornerstone for manipulating electronic and magnetic states in materials on a femtosecond timescale. Conventional models assume that optical excitation primarily modifies the occupation of the electron energy…

Materials Science · Physics 2025-05-12 Sergii Parchenko , Peter M. Oppeneer , Andreas Scherz

The role of photon angular momentum in laser-induced demagnetization of Nickel thin films is investigated by means of pump-probe time-resolved magneto-optical Kerr effect in the polar geometry. The recorded data display a strong dependency…

Materials Science · Physics 2009-11-11 F. Dalla Longa , J. T. Kohlhepp , W. J. M. de Jonge , B. Koopmans

Ultrafast spin dynamics in ferromagnetic half-metallic compound Sr_2FeMoO_6 is investigated by pump-probe measurements of magneto-optical Kerr effect. Half-metallic nature of this material gives rise to anomalous thermal insulation between…

Strongly Correlated Electrons · Physics 2009-10-31 T. Kise , T. Ogasawara , M. Ashida , Y. Tomioka , Y. Tokura , M. Kuwata-Gonokami

We show that electric currents are induced in inversion asymmetric ferromagnets if the exchange splitting varies in time after excitation by laser pulses. We interpret this phenomenon as the magnetic variant of the inverse Edelstein effect.…

Materials Science · Physics 2017-04-04 Frank Freimuth , Stefan Blügel , Yuriy Mokrousov

Spin angular momentum transfer in magnetic bilayers offers the possibility of ultrafast and low-loss operation for next-generation spintronic devices. We report the field- and temperature- dependent measurements on the magnetization…

Materials Science · Physics 2023-01-03 X. Liu , P. Liu , H. C. Yuan , J. Y. Shi , H. L. Wang , S. H. Nie , F. Jin , Z. Zheng , X. Z. Yu , J. H. Zhao , H. B. Zhao , G. Lüpke

The magneto-optical Kerr effect (MOKE) in the extreme ultraviolet (EUV) regime has helped to elucidate some of the key processes that lead to the manipulation of magnetism on ultrafast timescales. However, as we show in this paper, the…

Ultrafast laser excitation of ferromagnetic metals gives rise to correlated, highly non-equilibrium dynamics of electrons, spins and lattice, which are, however, poorly described by the widely-used three-temperature model (3TM). Here, we…

Materials Science · Physics 2024-01-17 Markus Weißenhofer , Peter M. Oppeneer

Ultrafast magnetization dynamics in metallic heterostructures consists of a combination of local demagnetization in the ferromagnetic constituent and spin-dependent transport contributions within and in between the constituents. Separation…

We investigate the ultrafast magnetization dynamics of an interlayer-exchange-coupled Co/Mn/Co trilayer system after excitation with an ultrafast optical pump. We probe element- and time-resolved ferromagnetic order by X-ray magnetic…

Femtosecond magneto-optical pump-probe measurements of ultrafast demagnetization show an intriguing difference in the first 100 fs of the magneto-optical Kerr response depending on whether the polarization of the pump and probe beams are in…

Materials Science · Physics 2018-04-06 Ritwik Mondal , Marco Berritta , Peter M. Oppeneer

We develop a theory of the magnetization dynamics triggered by ultrafast optical excitation of ferromagnetic semiconductors. We describe the effects of the strong carrier spin relaxation on the nonlinear optical response by using the…

Strongly Correlated Electrons · Physics 2008-08-04 J. Chovan , E. G. Kavousanaki , I. E. Perakis

Recent investigations have advanced the understanding of how structure-property relationships in ferromagnetic metal alloys affect the magnetization dynamics on nanosecond time-scales. A similar understanding for magnetization dynamics on…

Materials Science · Physics 2021-07-27 Ramya Mohan , Victor H. Ortiz , Luat Vuong , Sinisa Coh , Richard B. Wilson
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