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Related papers: Heat Transport in Herbertsmithite: Can a Quantum S…

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Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental…

Based on experimental data and our theoretical analysis, we provide a strategy for unambiguous establishing of gapless quantum spin liquid state (QSL) in herbertsmithite and other materials. To clarify the nature of QSL, we recommend…

The spin-1/2 kagom\'{e} Heisenberg antiferromagnet is generally accepted as one of the most promising two-dimensional models to realize a quantum spin liquid state. Previous experimental efforts were almost exclusively on only one…

Strongly Correlated Electrons · Physics 2022-12-28 Xiaochen Hong , Mahdi Behnami , Long Yuan , Boqiang Li , Wolfram Brenig , Bernd Büchner , Yuesheng Li , Christian Hess

The kagome Heisenberg antiferromagnet formed by frustrated spins arranged in a lattice of corner-sharing triangles is a prime candidate for hosting a quantum spin liquid (QSL) ground state consisting of entangled spin singlets. But the…

Strongly Correlated Electrons · Physics 2022-03-09 Jiaming Wang , Weishi Yuan , Philip M. Singer , Rebecca W. Smaha , Wei He , Jiajia Wen , Young S. Lee , Takashi Imai

Quantum spin liquid (QSL) is a novel state of matter with exotic excitations and was theoretically predicted to be realized most possibly in an S=1/2 kagome antiferromagnet. Experimentally searching for the candidate materials is a big…

Strongly Correlated Electrons · Physics 2014-09-15 Yuesheng Li , Bingying Pan , Shiyan Li , Wei Tong , Langsheng Ling , Zhaorong Yang , Junfeng Wang , Zhongjun Chen , Zhonghua Wu , Qingming Zhang

The metal-organic-framework (MOF) compound Cu$_3$(HOTP)$_2$, a.k.a. Cu$_3$(HHTP)$_2$, is a small-gap semiconductor containing a kagome lattice of antiferromagnetically coupled $S$=1/2 Cu$^\mathrm{II}$ spins with intra-layer nearest-neighbor…

Strongly Correlated Electrons · Physics 2024-11-28 F. L. Pratt , D. Lopez-Alcala , V. Garcia-Lopez , M. Clemente-Leon , J. J. Baldovi , E. Coronado

Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in lattices that act to frustrate the…

Strongly Correlated Electrons · Physics 2016-12-05 M. R. Norman

A quantum spin liquid (QSL) is a state of matter in which magnetic spins interact strongly, but quantum fluctuations inhibit long-range magnetic order even at zero temperature. A QSL has been predicted to have a host of exotic properties,…

Quantum spin liquids (QSLs) are fluid-like states of quantum spins where its long-range ordered state is destroyed by quantum fluctuations. The ground state of QSL and its exotic phenomena, which have been extensively discussed for decades,…

Strongly Correlated Electrons · Physics 2011-10-25 Minoru Yamashita , Takasada Shibauchi , Yuji Matsuda

Quantum spin liquids (QSL) are novel phases of matter which remain quantum disordered even at the lowest temperature. They are characterized by emergent gauge fields and fractionalized quasiparticles. Here we show that the sub-Kelvin…

Recently Han et al. have provided an analysis of the observed behavior of $\rm ZnCu_{3}(OH)_6Cl_2$ Herbertsmithite based on a separation of the contributions to its thermodynamic properties due to impurities from those due to the kagome…

Strongly Correlated Electrons · Physics 2016-09-20 V. R. Shaginyan , M. Ya. Amusia , J. W. Clark , G. S. Japaridze , A. Z. Msezane , K. G. Popov

Geometric frustration of magnetic ions can lead to a quantum spin liquid ground state where long range magnetic order is avoided despite strong exchange interactions. The physical realization of quantum spin liquids comprises a major…

Strongly Correlated Electrons · Physics 2023-06-07 Alex Hallett , Catalina Avarvarei , John W. Harter

One main theme in current condensed matter physics is the search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature without static order. However, there is no…

Strongly Correlated Electrons · Physics 2023-01-10 Chengpeng Tu , Dongzhe Dai , Xu Zhang , Chengcheng Zhao , Xiaobo Jin , Bin Gao , Tong Chen , Pengcheng Dai , Shiyan Li

The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet…

Strongly Correlated Electrons · Physics 2016-03-02 M. Gomilsek , M. Klanjsek , M. Pregelj , F. C. Coomer , H. Luetkens , O. Zaharko , T. Fennell , Y. Li , Q. M. Zhang , A. Zorko

A quantum spin liquid (QSL) is an exotic quantum state of matter characterized by fluctuating spins which may exhibit long-range entanglement. Among the possible host candidates for a QSL ground state, the $S$=1/2 kagome lattice…

Herbertsmithite, ZnCu3(OH)6Cl2, is the prototype candidate for a spin liquid behavior on a geometrically perfect kagome lattice. Its discovery and the absence of any evidence for spin-freezing down to the lowest probed temperature to-date…

Strongly Correlated Electrons · Physics 2015-05-28 P. Mendels , F. Bert

Spin liquids are exotic phases of quantum matter challenging Landau's paradigm of symmetry-breaking phase transitions. Despite strong exchange interactions, spins do not order or freeze down to zero temperature. While well-established for…

Strongly Correlated Electrons · Physics 2020-04-22 P. Khuntia , M. Velazquez , Q. Barthélemy , F. Bert , E. Kermarrec , A. Legros , B. Bernu , L. Messio , A. Zorko , P. Mendels

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

Despite tremendous investigations, a quantum spin liquid state realized in spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, a quantum spin liquid candidate on the perfect kagome…

Strongly Correlated Electrons · Physics 2021-06-15 H. Murayama , T. Tominaga , T. Asaba , A. de Oliveira Silva , Y. Sato , H. Suzuki , Y. Ukai , S. Suetsugu , Y. Kasahara , R. Okuma , I. Kimchi , Y. Matsuda

Quantum spin liquids represent exotic states of spin systems characterized by long-range entanglement and emergent fractionalized quasiparticles. It is generally believed that disorder is hostile to quantum spin liquids. In our study, we…

Strongly Correlated Electrons · Physics 2024-08-30 Aini Xu , Qinxin Shen , Bo Liu , Zhenyuan Zeng , Lankun Han , Liqin Yan , Jun Luo , Jie Yang , Rui Zhou , Shiliang Li
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