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We describe a two-color pump-probe scanning magneto-optical Kerr effect (MOKE) microscope which we have developed to investigate electron spin phenomena in semiconductors at cryogenic temperatures with picosecond time and micrometer spatial…

Instrumentation and Detectors · Physics 2015-06-17 T. Henn , T. Kiessling , W. Ossau , L. W. Molenkamp , K. Biermann , P. V. Santos

The possibility of spatially resolving the optical properties of atomically thin materials is especially appealing as they can be modulated at the micro- and nanoscale by reducing their thickness, changing the doping level or applying a…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 Andres Castellanos-Gomez , Jorge Quereda , Herko P. van der Meulen , Nicolás Agraït , Gabino Rubio-Bollinger

Monolayer transition metal dichalcogenides (TMD) have immense potential for future spintronic and valleytronic applications due to their two-dimensional nature and long spin/valley lifetimes. We investigate the origin of these long-lived…

How atoms and electrons in a molecule move during a chemical reaction and how rapidly energy is transferred to or from the surroundings can be studied with flashes of laser light. However, despite prolonged efforts to develop various…

Chemical Physics · Physics 2022-01-05 JunWoo Kim , Jonggu Jeon , Tai Hyun Yoon , Minhaeng Cho

Imaging with ultrashort exposure times is generally achieved with a crossed-beam geometry. In the usual arrangement, an off-axis gating pulse induces birefringence in a medium exhibiting a strong Kerr response (commonly carbon disulfide)…

We present an ultrasensitive technique for probing transient optical changes in atomically thin molybdenum disulfide (MoS$_2$) layers integrated onto silicon nitride (Si$_3$N$_4$) ring resonators. The MoS$_2$ is illuminated by a femtosecond…

Spectral analysis is one of the most powerful technologies for studying and understanding matter. As the devices for spectral analysis, spectrometers are widely used in material detection, isotope analysis, trace gas detection, and the…

Mid-infrared (mid-IR) spectroscopy offers unparalleled sensitivity for the detection of trace gases, solids and liquids, which is based on the existence of strong telltale vibrational bands in this part of the spectrum. It was shown more…

Optics · Physics 2016-08-29 Viktor O. Smolski , Honglei Yang , Jia Xu , Konstantin L. Vodopyanov

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…

Atomically thin two-dimensional (2D) transition metal dichalcogenides (TMDs), such as MoS$_2$, are promising candidates for nanoscale photonics because of strong-light matter interactions. However, Fermi level pinning due to metal-induced…

Mesoscale and Nanoscale Physics · Physics 2023-03-07 Hon-Loen Sinn , Aravindh Kumar , Eric Pop , Akm Newaz

We present a widefield two-dimensional electronic spectroscopy microscope (2DESM) that integrates multidimensional coherent spectroscopy with optical imaging, enabling femtosecond temporal and micrometer spatial resolution. The broadband…

Within the curl-curl type vector equation describing a monochromatic light wave in a focusing Kerr medium, the transverse structure of extremely narrow, linearly polarized self-focused optical beams is found numerically with a high…

Optics · Physics 2026-02-10 Victor P. Ruban

Achieving spatiotemporal control of light at subwavelength and subcycle scales is an important milestone in the development of new photonic materials and technologies. Ultrafast spatiotemporal light modulation currently relies on electronic…

Optics · Physics 2025-11-07 Claudio U. Hail , Lior Michaeli , Harry A. Atwater

The Kerr soliton frequency comb is a revolutionary compact ruler of coherent light that allows applications, from precision metrology to quantum information technology. The universal, reliable, and low-cost soliton microcomb source is key…

Fourier-transform spectroscopy is an indispensable tool for analyzing chemical samples in scientific research as well as chemical and pharmaceutical industries. Recently, its measurement speed, sensitivity, and precision have been shown to…

Optics · Physics 2025-05-06 Takuro Ideguchi , Tasuku Nakamura , Yohei Kobayashi , Keisuke Goda

Dual-comb interferometry utilizes two optical frequency combs to map the optical field's spectrum to a radio-frequency signal without using moving parts, allowing improved speed and accuracy. However, the method is compounded by the…

Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

In analogy with optical near-field scanning methods, we use tapered dielectric waveguides as probes for a millimeter wave vector network analyzer. By scanning thin samples between two such probes we are able to map the spatially varying…

Soft Condensed Matter · Physics 2009-11-13 Nathan S. Greeney , John A. Scales

The two-dimensional sub-cycle-time to electron momentum mapping provided by orthogonal two-color laser fields is applied to photoelectron spectroscopy. Using neon as the example we gain experimental access to the dynamics of emitted…

Transition metal dichalcogenide MoS2 is a two-dimensional material, attracting much attention for next-generation applications thanks to rich functionalities stemmed from the crystal structure. Many experimental and theoretical works have…

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