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We report Raman-scattering results of YbRu$_2$Ge$_2$ single crystals to explore the phononic and crystal-field (CF) excitations. This heavy-fermion metal is suggested to enter a ferroquadrupolar (FQ) phase below T$_0$=10 K. The tetragonal…

Strongly Correlated Electrons · Physics 2019-06-06 Mai Ye , E. W. Rosenberg , I. R. Fisher , G. Blumberg

Inelastic neutron scattering studies in single crystals of TbInO3 and TbIn0.95Mn0.05O3 with nearly-triangular antiferromagnetic lattice are reported. At low energies, a broad and apparently gapless continuum of magnetic excitations, located…

Strongly Correlated Electrons · Physics 2019-07-10 M. G. Kim , B. Winn , S. Chi , A. T. Savici , J. A. Rodriguez-Rivera , W. C. Chen , X. Xu , Y. Li , J. W. Kim , S. -W. Cheong , V. Kiryukhin

Pr$_2$Zr$_2$O$_7$ is a pyrochlore quantum spin-ice candidate. Using Raman scattering spectroscopy we probe crystal electric field excitations of Pr$^{3+}$, and demonstrate the importance of their interactions with the lattice. We identify a…

Strongly Correlated Electrons · Physics 2021-09-03 Yuanyuan Xu , Huiyuan Man , Nan Tang , Santu Baidya , Hongbin Zhang , Satoru Nakatsuji , David Vanderbilt , Natalia Drichko

We apply moderate-high-energy inelastic neutron scattering (INS) measurements to investigate Yb$^{3+}$ crystalline electric field (CEF) levels in the triangular spin-liquid candidate YbMgGaO$_4$. Three CEF excitations from the ground-state…

We study ground state properties and particle excitation spectra across a commensurate charge density wave transition in a system of strongly interacting fermions, using series expansion methods and mean-field theory. We consider a…

Strongly Correlated Electrons · Physics 2015-06-22 Trithep Devakul , Rajiv R. P. Singh

The strong coupling between spin, lattice and electronic degrees of freedom in magnetic materials can produce interesting phenomena, including multiferroic and magnetodielectric (MD) behavior, and exotic coupled excitations, such as…

Strongly Correlated Electrons · Physics 2019-05-08 A. Sethi , J. E. Slimak , T. Kolodiazhnyi , S. L. Cooper

One- and multi-phonon excitations of the single crystalline LaCoO3 were studied using Raman spectroscopy in the temperature region of 5 K - 300 K. First-order Raman spectra show a larger number of phonon modes than allowed for the…

Strongly Correlated Electrons · Physics 2022-05-31 V. Gnezdilov , K. -Y. Choi , Yu. Pashkevich , P. Lemmens , S. Shiryaev , G. Bychkov , S. Barilo , V. Fomin , A. V. Yeremenko

The phonon and crystal field excitations in several rare earth titanate pyrochlores are investigated. Magnetic measurements on single crystals of Gd2Ti2O7, Tb2Ti2O7, Dy2Ti2O7 and Ho2Ti2O7 are used for characterization, while Raman…

Lattice and spin excitations have been studied by Raman scattering in hexagonal YbMnO3 single crystals. The temperature dependences of the phonon modes show that the E2 mode at 256 cm-1 related to the displacement of Mn and O ions in a-b…

Strongly Correlated Electrons · Physics 2012-11-12 J. Liu , C. Toulouse , P. Rovillain , M. Cazayous , Y. Gallais , M. -A. Measson , S. W. Cheong , N. Lee , A. Sacuto

We present a comprehensive study of polar and magnetic excitations in BiFeO3 ceramics and a thin film epitaxially grown on an orthorhombic (110) TbScO3 substrate. Infrared reflectivity spectroscopy was performed at temperatures from 5 to…

Materials Science · Physics 2015-05-22 S. Skiadopoulou , V. Goian , C. Kadlec , F. Kadlec , X. F. Bai , I. C. Infante , B. Dkhil , C. Adamo , D. G. Schlom , S. Kamba

The low-dimensional s=1/2 compound (NO)[Cu(NO3)3] has recently been suggested to follow the Nersesyan-Tsvelik model of coupled spin chains. Such a system shows unbound spinon excitations and a resonating valence bond ground state due spin…

Strongly Correlated Electrons · Physics 2022-06-08 V. Gnezdilov , P. Lemmens , Yu. G. Pashkevich , D. Wulferding , I. V. Morozov , O. S. Volkova , A. Vasiliev

In this paper, we study the spin excitation properties of the frustrated triangular-lattice antiferromagnet Yb(BaBO$_3$)$_3$ with nuclear magnetic resonance. From the spectral analysis, neither magnetic ordering nor spin freezing is…

Strongly Correlated Electrons · Physics 2020-08-03 K. Y. Zeng , Long Ma , Y. X. Gao , Z. M. Tian , L. S. Ling , Li Pi

We report time-of-flight neutron scattering measurements of the magnetic spectrum of Tb3+ in Tb2Ti2O7. The data, which extend up to 120 meV and have calibrated intensity, enable us to consolidate and extend previous studies of the…

Strongly Correlated Electrons · Physics 2015-09-04 A. J. Princep , H. C. Walker , D. T. Adroja , D. Prabhakaran , A. T. Boothroyd

We present the low-temperature magnetic properties of two Yb$^{3+}$-based triangular lattice compounds NaSrYb(BO$_3$)$_2$ and K$_3$YbSi$_2$O$_7$ via thermodynamic measurements followed by crystal electric field (CEF) calculations.…

Materials Science · Physics 2025-01-27 S. Guchhait , R. Kolay , A. Magar , R. Nath

Raman scattering experiments on stoichiometric, Mott-insulating LaTiO$_3$ over a wide range of excitation energies reveal a broad electronic continuum which is featureless in the paramagnetic state, but develops a gap of $\sim 800$…

Strongly Correlated Electrons · Physics 2015-10-28 C. Ulrich , G. Khaliullin , M. Guennou , H. Roth , T. Lorenz , B. Keimer

We study ground-state properties and the low-lying excitations of Heisenberg spin ladders composed of two ferrimagnetic chains with alternating site spins $(S_1>S_2)$ by using the bosonic Dyson-Maleev formalism and Lanczos numerical…

Strongly Correlated Electrons · Physics 2009-10-31 N. B. Ivanov , J. Richter

We employ tensor network renormalization to explore the dynamical spectra of the easy-axis triangular-lattice antiferromagnet (TLAF) in a magnetic field. Our analysis identifies two distinct low-energy magnon excitations: a gapless…

Strongly Correlated Electrons · Physics 2024-04-23 Runze Chi , Jiahang Hu , Hai-Jun Liao , T. Xiang

The spin liquid state of the antiferromagnetic Heisenberg model on a triangular lattice is studied within the self-consistent Green's function method. It is shown that the spin excitation spectra is gapless, and ground-state energy per site…

Strongly Correlated Electrons · Physics 2009-10-31 Zhan-hai Dong , Shiping Feng

The entanglement of electronic spin and orbital degrees of freedom is often the precursor to emergent behaviors in condensed matter systems. With considerable spin-orbit coupling strength, the cobalt atom on a honeycomb lattice offers a…

Here we present a neutron scattering-based study of magnetic excitations and magnetic order in NaYbO$_2$ under the application of an external magnetic field. The crystal electric field-split $J = 7/2$ multiplet structure is determined,…

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