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We perform molecular-dynamics simulations of a molecular system in supercooled states for different values of inertia parameters to provide evidence that the long-time dynamics depends only on the equilibrium structure. This observation is…

Soft Condensed Matter · Physics 2009-11-10 S. -H. Chong , F. Sciortino

Dynamic heterogeneity in glass-formers has been related to their static structure using the concept of dynamic propensity. We re-examine this relationship by analyzing dynamical fluctuations in two atomistic glass-formers and two…

Statistical Mechanics · Physics 2009-08-25 Ludovic Berthier , Robert L. Jack

The original Maxwell visco-elastic constitutive model cannot predict the correct mechanical properties for most fluids. In this work, the model is generalized with respect to wave-vector and extended with a correction function. This new…

Soft Condensed Matter · Physics 2024-01-25 Jesper Schmidt Hansen

We present a coarse-graining strategy for reducing the number of particle species in mixtures to achieve a simpler system with higher diffusion while preserving the total particle number and characteristic dynamic features. As a system of…

Soft Condensed Matter · Physics 2020-09-16 Thomas Heinemann , YounJoon Jung

Glass formation is one of the most interesting phenomena in the condensed matter field. Considerable effort has gone into understanding and predicting the glass formability. However, the previous prediction requires the glass first made…

Materials Science · Physics 2019-02-12 R. Dai , R. Ashcraft , A. K. Gangopadhyay , K. F. Kelton

We examine the structural and dynamic properties of confined binary hard-sphere mixtures designed to mimic realizable colloidal thin films. Using computer simulations, governed by either Newtonian or overdamped Langevin dynamics, together…

Soft Condensed Matter · Physics 2015-05-01 Jonathan A. Bollinger , Avni Jain , James Carmer , Thomas M. Truskett

We consider the Kob-Andersen model, a cooperative lattice gas with kinetic constraints which has been widely analyzed in the physics literature in connection with the study of the liquid/glass transition. We consider the model in a finite…

Probability · Mathematics 2020-09-02 Fabio Martinelli , Assaf Shapira , Cristina Toninelli

It is demonstrated that properly reduced transport coefficients (self-diffusion, shear viscosity, and thermal conductivity) of Lennard-Jones fluids along isotherms exhibit quasi-universal scaling on the density divided by its value at the…

Soft Condensed Matter · Physics 2021-09-30 S. A. Khrapak , A. G. Khrapak

The swap Monte Carlo algorithm allows the preparation of highly stable glassy configurations for a number of glass-formers, but is inefficient for some models, such as the much studied binary Kob-Andersen (KA) mixture. We have recently…

Statistical Mechanics · Physics 2020-10-07 Anshul D. S. Parmar , Benjamin Guiselin , Ludovic Berthier

Glass-forming liquids are broadly classified as being fragile or strong, depending on the deviation from Arrhenius behavior of their relaxation times. A fragile to strong crossover is observed or inferred in liquids like water and silica,…

Soft Condensed Matter · Physics 2022-04-12 Pallai Das , Srikanth Sastry

We present a numerical simulation study of a simple monatomic Lennard-Jones liquid under shear flow, as a function of both temperature and shear rate. By investigating different observables we find that i) It exists a line in the…

Soft Condensed Matter · Physics 2009-11-07 L. Angelani , G. Ruocco , F. Sciortino , P. Tartaglia , F. Zamponi

We solved the mode-coupling equations for the Kob-Andersen binary mixture using the structure factors calculated from Brownian dynamics simulations of the same system. We found, as was previously observed, that the mode-coupling…

Soft Condensed Matter · Physics 2009-11-11 Elijah Flenner , Grzegorz Szamel

We infer both microscopic and macroscopic behaviors of a three-dimensional chaotic fluid flow using reservoir computing. In our procedure of the inference, we assume no prior knowledge of a physical process of a fluid flow except that its…

Computational Physics · Physics 2018-09-12 Kengo Nakai , Yoshitaka Saiki

The dynamical correlations of a model consisting of particles constrained on the line and interacting with a nearest--neighbour Lennard--Jones potential are computed by molecular--dynamics simulations. A drastic qualitative change of the…

Statistical Mechanics · Physics 2009-11-11 Stefano Lepri , Paolo Sandri , Antonio Politi

Molecular dynamics simulations of a Lennard-Jones binary mixture confined in a disordered array of soft spheres are presented. The single particle dynamical behavior of the glass former is examined upon supercooling. Predictions of mode…

Statistical Mechanics · Physics 2009-11-07 P. Gallo , R. Pellarin , M. Rovere

We present computer simulation results on the dynamic propensity [as defined by Widmer- Cooper, Harrowell, and Fynewever, Phys. Rev. Lett. 93, 135701 (2004)] in a Kob-Andersen binary Lennard-Jones liquid system consisting of 8788 particles.…

Materials Science · Physics 2011-05-26 M. Shajahan G. Razul , Gurpreet S. Matharoo , Peter H. Poole

Predicting the local dynamics of supercooled liquids based purely on local structure is a key challenge in our quest for understanding glassy materials. Recent years have seen an explosion of methods for making such a prediction, often via…

Soft Condensed Matter · Physics 2021-08-25 Emanuele Boattini , Frank Smallenburg , Laura Filion

According to excess-entropy scaling, dynamic properties of liquids like viscosity and diffusion coefficient are determined by the entropy. This link between dynamics and thermodynamics is increasingly studied and of interest also for…

Soft Condensed Matter · Physics 2024-08-13 Ian M. Douglass , Jeppe C. Dyre , Lorenzo Costigliola

We study the simplest model of dynamic heterogeneities in glass forming liquids: one-spin facilitated kinetic Ising model introduced by Fredrickson and Andersen [G.H. Fredrickson and H.C. Andersen, Phys. Rev. Lett. 53, 1244 (1984); J. Chem.…

Statistical Mechanics · Physics 2009-11-10 Grzegorz Szamel

The nonequilibrium dynamics of a binary Lennard-Jones mixture in a simple shear flow is investigated by means of molecular dynamics simulations. The range of temperature investigated covers both the liquid, supercooled and glassy states,…

Soft Condensed Matter · Physics 2009-11-07 Ludovic Berthier , Jean-Louis Barrat