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We investigate angular emission distributions of the 1s-photoelectrons of N$_2$ ionized by linearly polarized synchrotron radiation at $h \nu=40$ keV. As expected, nondipole contributions cause a very strong forward-backward asymmetry in…

We present analytical expressions of momentum-resolved core-level photoemission time delay in a molecular frame of a heteronuclear diatomic molecule upon photoionization by a linearly polarized soft x-rays attosecond pulse. For this…

Chemical Physics · Physics 2022-05-31 Y. Tamura , K. Yamazaki , K. Ueda , K. Hatada

We have measured the molecular frame angular distributions of photoelectrons emitted from the Carbon K shell of fixed-in-space CO molecules for the case of simultaneous excitation of the remaining molecular ion. Normal and conjugate shake…

The polarization of soft and tender X-rays serves as a widely utilized probe for investigating diverse physical properties, such as magnetic order in materials. However, experimental methods for determining the polarization of tender X-rays…

Materials Science · Physics 2026-03-26 Yoshiyuki Ohtsubo , Hiroaki Kimura

The proton analyzing power in carbon has been measured for energies of 82 to 217 MeV and proton scattering angles of 5 to 41 degrees. The measurements were carried out using polarized protons from the elastic scattering H(pol. e, pol. p)…

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

Atomic Physics · Physics 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

We present the angular distribution of electrons knocked out from an atom in a fast charge particle collision at small momentum transfer. It is determined not only by dipole but also by quadrupole transitions, the contribution of which can…

Atomic Physics · Physics 2015-06-03 M. Ya. Amusia , L. V. Chernysheva , E. Z. Liverts

We explore photo-electron spectra (PES) and photo-electron angular distributions (PAD) of C$_{60}$ with time-dependent density functional theory (TDDFT) in real time. To simulate experiments in gas phase, we consider isotropic ensembles of…

Atomic and Molecular Clusters · Physics 2014-12-12 C. -Z. Gao , P. Wopperer , P. M. Dinh , E. Suraud , P. -G. Reinhard

Methods for experimental reconstruction of molecular frame (MF) photoionization dynamics, and related properties - specifically MF photoelectron angular distributions (PADs) and continuum density matrices - are outlined and discussed.…

Chemical Physics · Physics 2024-06-06 Paul Hockett , Varun Makhija

Differential cross sections for Compton scattering from the proton have been measured at scattering angles of $55^\circ$, $90^\circ$, and $125^\circ$ in the laboratory frame using quasimonoenergetic linearly (circularly) polarized photon…

The spectrum and the circular polarization of radiation from longitudinally polarized high-energy electrons in oriented single crystal are considered using the method which permits inseparable consideration of both the coherent and the…

High Energy Physics - Phenomenology · Physics 2008-11-26 V. N. Baier , V. M. Katkov

Emitting dipole orientation (EDO) is an important issue of emitting materials in organic light-emitting diodes (OLEDs) for an increase of outcoupling efficiency of light. The origin of preferred orientation of emitting dipole of spherically…

Materials Science · Physics 2018-02-07 Chang-Ki Moon , Kwon-Hyeon Kim , Jang-Joo Kim

We study ionization dynamics of aligned diatomic molecules N$_2$ in strong elliptical laser fields experimentally and theoretically. The alignment dependence of photoelectron momentum distributions (PMDs) of N$_2$ measured in experiments is…

Recent experiments [D. Pengel, S. Kerbstadt, L. Englert, T. Bayer, and M. Wollenhaupt, \href{https://journals.aps.org/pra/abstract/10.1103/PhysRevA.96.043426}{{\PRA} {\bf 96} 043426 (2017)}] have measured the photoelectron momentum…

Atomic Physics · Physics 2019-12-18 G. S. J. Armstrong , D. D. A. Clarke , J. Benda , J. Wragg , A. C. Brown , H. W. van der Hart

We present here the results of calculations of photoelectrons' angular anisotropy and spin-polarization parameters for a number of semi-filled shell atoms. We consider ionization of outer or in some cases next to the outer electrons in a…

Atomic Physics · Physics 2007-05-23 M. Ya. Amusia , L. V. Chernysheva

Based on the quantum electrodynamics, we present a generic formalism of the polarization for beamed monochromatic photons scattered by electrons in any spectral distribution. The formulae reduce to the components of the Fano matrix when…

High Energy Astrophysical Phenomena · Physics 2014-11-07 Zhe Chang , Yunguo Jiang , Hai-Nan Lin

We present a time-dependent density-functional method able to describe the photoelectron spectrum of atoms and molecules when excited by laser pulses. This computationally feasible scheme is based on a geometrical partitioning that…

Atomic Physics · Physics 2012-06-28 U. De Giovannini , D. Varsano , M. A. L. Marques , H. Appel , E. K. U. Gross , A. Rubio

We report fully differential photoelectron spectra from an {\it ab-inito} coupled channels treatment of CO$_2$. Photoionization by laser pulses centered at 400 nm and 800 nm wavelength are considered, with arbitrary molecular alignment and…

Atomic Physics · Physics 2017-09-05 Vinay Pramod Majety , Armin Scrinzi

We have probed the fragmentation dynamics in a bent triatomic molecule, water, a non-planar molecule, methanol, and a planar ring-structured molecule, benzene, using 100 fs duration pulses of linearly and circularly polarized, infrared,…

Atomic Physics · Physics 2009-11-10 F A Rajgara , M Krishnamurthy , D Mathur

We consider deflection of polarizable molecules by inhomogeneous optical fields, and analyze the role of molecular orientation and rotation in the scattering process. It is shown that molecular rotation induces spectacular rainbow-like…

Atomic Physics · Physics 2015-05-14 E. Gershnabel , I. Sh. Averbukh