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As the bound state of two oppositely charged particles, excitons emerge from optically excited semiconductors as the electronic analogue of a hydrogen atom. In the two-dimensional (2D) case, realized either in quantum well systems or truly…

Optics · Physics 2022-05-13 Tobias Graß , Utso Bhattacharya , Julia Sell , Mohammad Hafezi

Time-resolved photoluminescence spectra after nonresonant excitation show a distinct 1s resonance, independent of the existence of bound excitons. A microscopic analysis identifies excitonic and electron-hole plasma contributions. For low…

Condensed Matter · Physics 2009-11-10 S. Chatterjee , C. Ell , S. Mosor , G. Khitrova , H. M. Gibbs , W. Hoyer , M. Kira , S. W. Koch , J. P. Prineas , H. Stolz

It is well-known that exciton effects are determinant to understand the optical absorption spectrum of low-dimensional materials. However, the role of excitons in nonlinear optical responses has been much less investigated at an…

Mesoscale and Nanoscale Physics · Physics 2024-06-21 J. J. Esteve-Paredes , M. A. García-Blázquez , A. J. Uría-Álvarez , M. Camarasa-Gómez , J. J. Palacios

Exciton binding energies of hundreds of meV and strong light absorption in the optical frequency range make transition metal dichalcogenides (TMDs) promising for novel optoelectronic nanodevices. In particular, atomically thin TMDs can be…

Mesoscale and Nanoscale Physics · Physics 2018-04-24 Simon Ovesen , Samuel Brem , Christopher Linderälv , Mikael Kuisma , Paul Erhart , Malte Selig , Ermin Malic

Excitonic insulators (EIs), arising in semiconductors when the electron-hole binding energy exceeds the band gap, are a solid-state prototype for bosonic phases of matter. Unlike the charged excitations that are frozen and unable to…

Mesoscale and Nanoscale Physics · Physics 2023-09-27 Phuong X. Nguyen , Liguo Ma , Raghav Chaturvedi , Kenji Watanabe , Takashi Taniguchi , Jie Shan , Kin Fai Mak

Innovations in imaging technology involves finding strategies and materials suitable for detection applications over the entire infrared range. Herein, we propose a new design concept based on the unique feature of an excitonic insulator,…

Materials Science · Physics 2022-07-27 Jing Liu , Yuanchang Li

Resolving the early-stage dynamics of exciton formation following non-resonant photoexcitation in time, energy, and momentum is quite challenging due to their inherently fast timescales and the proximity of the excitonic state to the bottom…

The effects of the electron-phonon interaction on optical excitations can be understood in terms of exciton-phonon coupling, and require a careful treatment in low-dimensional materials with strongly bound excitons or strong electron-hole…

Materials Science · Physics 2022-02-17 Gabriel Antonius , Steven G. Louie

In the 1960s, it was proposed that in small indirect band-gap materials, excitons can spontaneously form because the density of carriers is too low to screen the attractive Coulomb interaction between electrons and holes. The result is a…

Materials Science · Physics 2024-05-31 Zhi Li , Muhammad Nadeem , Zengji Yue , David Cortie , Michael Fuhrer , Xiaolin Wang

Excitons consist of electrons and holes held together by their attractive Coulomb interaction. Although excitons are neutral excitations, spatial fluctuations in their charge density couple with the ions of the crystal lattice. This…

Materials Science · Physics 2024-01-18 Zhenbang Dai , Chao Lian , Jon Lafuente-Bartolome , Feliciano Giustino

During a band-gap-tuned semimetal-to-semiconductor transition, Coulomb attraction between electrons and holes can cause spontaneously formed excitons near the zero-band-gap point, or the Lifshitz transition point. This has become an…

We investigate an interesting anisotropic van der Waals material, Ta$_{2}$NiSe$_{5}$, using optical spectroscopy. Ta$_{2}$NiSe$_{5}$ has been known as one of the few excitonic insulators proposed over 50 years ago. Ta$_{2}$NiSe$_{5}$ has…

Materials Science · Physics 2018-08-21 Yu-Seong Seo , Man Jin Eom , Jun Sung Kim , Chang-Jong Kang , Byung Il Min , Jungseek Hwang

The demonstration of Bose-Einstein condensation in atomic gases at micro-Kelvin temperatures is a striking landmark while its evidence for semiconductor excitons still is a long-awaited milestone. This situation was not foreseen because…

In heterostructures consisting of different transition-metal dichalcogenide monolayers, a staggered band alignment can occur, leading to rapid charge separation of optically generated electron-hole pairs into opposite monolayers. These…

The electro-optical properties of most semiconductors and insulators of technological interest are dominated by the presence of electron-hole quasiparticles called excitons. The manipulation of these hydrogen-like quasi-particles in…

Utilizing the unbiased time-dependent density-matrix renormalization group technique, we examine the photoemission spectra in the extended Falicov-Kimball model at zero and finite temperatures, particularly with regard to the excitonic…

Strongly Correlated Electrons · Physics 2021-03-31 Satoshi Ejima , Florian Lange , Holger Fehske

We present the phase diagram of free charges (electrons and holes), excitons, and biexcitons in highly excited CdSe nanoplatelets that predicts a crossover to a biexciton-dominated region at easily attainable low temperatures or high…

Mesoscale and Nanoscale Physics · Physics 2020-09-16 F. García Flórez , Laurens D. A. Siebbeles , H. T. C. Stoof

We report on small-cluster exact-diagonalization calculations which prove the formation of electron-hole pairs (excitons) as prerequisite for spontaneous interlayer phase coherence in bilayer systems described by the extended…

Strongly Correlated Electrons · Physics 2013-07-25 T. Kaneko , S. Ejima , H. Fehske , Y. Ohta

An odd number of gapless Dirac fermions is guaranteed to exist at a surface of a strong topological insulator. We show that in a thin-film geometry and under external bias, electron-hole pairs that reside in these surface states can…

Strongly Correlated Electrons · Physics 2009-10-15 B. Seradjeh , J. E. Moore , M. Franz

The development of a Turing instability to a spatially modulated state in a photoexcited electron-hole system is proposed as a novel signature of exciton Bose statistics. We show that such an instability, which is driven by kinetics of…

Mesoscale and Nanoscale Physics · Physics 2008-04-12 L. S. Levitov , B. D. Simons , L. V. Butov