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We report on the effects of electron collision and indirect ionization processes, occurring at photoexcitation and electron kinetic energies well below 30 eV on the photoemission spectra of liquid water. We show that the nascent…

We propose an imaging technique to follow core-hole wave-packet oscillations in the nitrogen molecule. In this scheme, an attosecond x-ray pulse core-ionizes the nitrogen molecule and a subsequent attosecond x-ray pulse probes the evolution…

Chemical Physics · Physics 2019-08-15 Ludger Inhester , Loren Greenman , Artem Rudenko , Daniel Rolles , Robin Santra

We present an experimental and theoretical study of core-level ionization of small hetero- and homo-nuclear molecules employing circularly polarized light and address molecular-frame photoelectron angular distributions in the light's…

In a recent paper [Phys. Rev. Lett. 125, 043201 (2020)] (Ref.1) Liao et al. propose a theory of the interferometric photoemission delay based on the concepts of the photoelectron phase and photoelectron effective mass. The present comment…

Materials Science · Physics 2021-04-26 E. E. Krasovskii , R. O. Kuzian

We investigate theoretically the relative time delay of photoelectrons originating from different atomic subshells of noble gases. This quantity was measured via attosecond streaking and studied theoretically by Schultze et al. [Science…

Atomic Physics · Physics 2015-06-22 Jonas Wätzel , Andrey Moskalenko , Yaroslav Pavlyukh , Jamal Berakdar

The coherent interaction with ultrashort light pulses is a powerful strategy for monitoring and controlling the dynamics of wave packets in all states of matter. As light presents an oscillation period of a few femtoseconds ($T=2.6$~fs in…

Using a Monte Carlo ray-tracing code in full general relativity, we calculate the transport of photons from a geodesic hot spot emitter through a corona of hot electrons surrounding a black hole. Each photon is followed until it is either…

Astrophysics · Physics 2007-05-23 Jeremy D. Schnittman

This paper concerns the theory of non-recollisional ionization or detachment of atoms or ions by intense few-cycle pulses. It is shown that in certain conditions of pulse duration, peak intensity and carrier-envelope phase, the ionization…

Atomic Physics · Physics 2014-09-04 C. C. Chirila , R. M. Potvliege

Quantum coherence plays a fundamental role in the study and control of ultrafast dynamics in matter. In the case of photoionization, entanglement of the photoelectron with the ion is a well known source of decoherence when only one of the…

We report the discovery of hard X-ray delays in the X-ray emission of the Seyfert 1 galaxy Mrk 110, based on a long XMM-Newton observation. Cross correlation between the X-ray light curves of different energy bands reveals an energy…

Astrophysics · Physics 2011-02-11 Surajit Dasgupta , A. R. Rao

We develop a model for predicting fine- and hyperfine intensities in the direct photoionization of molecules based on the separability of electron and nuclear spin states from vibrational-electronic states. Using spherical tensor algebra,…

Chemical Physics · Physics 2016-08-24 Matthias Germann , Stefan Willitsch

We describe numerically the ionization process induced by linearly and circularly polarized XUV attosecond laser pulses on an aligned atomic target, specifically, the excited state…

Atomic Physics · Physics 2021-05-26 Juan J. Omiste , Lars Bojer Madsen

We employ the R-matrix with time-dependence method to study attosecond angular streaking of F$^-$. Using this negative ion, free of long-range Coulomb interactions, we elucidate the role of short-range electron correlation effects in an…

Atomic Physics · Physics 2020-05-20 G. S. J. Armstrong , D. D. A. Clarke , J. Benda , A. C. Brown , H. W. van der Hart

Signatures of the Coulomb corrections in the photoelectron momentum distribution during laser-induced ionization of atoms or ions in tunneling and multiphoton regimes are investigated analytically in the case of an one-dimensional problem.…

After photon absorption, electrons from a dispersive band of a solid require a finite time in the photoemission process before being photoemitted as free particles, in line with recent attosecondresolved photoemission experiments. According…

Mesoscale and Nanoscale Physics · Physics 2017-02-15 Mauro Fanciulli , Henrieta Volfová , Stefan Muff , Jürgen Braun , Hubert Ebert , Jan Minár , Ulrich Heinzmann , J. Hugo Dil

We investigate the strong-field ionization of atomic hydrogen in a few-cycle elliptically polarized infrared pulse by solving the time-dependent Schr\"odinger equation. The dependence of the photoelectron momentum distribution on the pulse…

Atomic Physics · Physics 2022-11-30 Nicolas Douguet , Klaus Bartschat

The electron motion in atoms and molecules is at the heart of all phenomena in nature that occur outside the nucleus. Recently, ultrafast electron and X-ray imaging tools have been developed to image the ultrafast dynamics of matter in real…

Doubly charged molecular cations often carry signatures of electronic correlation and electron-nuclear entanglement present in the parent cation. Here, we produce ethylene dications using a combination of an extreme ultraviolet pump and…

Photoelectron spectroscopy in intense laser fields has proven to be a powerful tool for providing detailed insights into molecular structure. The ionizing molecular orbital, however, has not been reconstructed from the photoelectron…

Atomic Physics · Physics 2023-04-14 XuanYang Lai , RenPing Sun , ShaoGang Yu , YanLan Wang , Wei Quan , André Staudte , XiaoJun Liu

Study on ionization process of molecules in an intense infrared laser field is of paramount interest in strong-field physics and constitutes the foundation of imaging of molecular valence orbitals and attosecond science. We show measurement…

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