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Excitons dominate the optoelectronic response of many materials. Depending on the time scale and host material, excitons can exhibit free diffusion, phonon-limited diffusion, or polaronic diffusion, and exciton transport often limits the…

Mesoscale and Nanoscale Physics · Physics 2026-01-28 Joshua J. P. Thompson , Wojciech J. Jankowski , Robert-Jan Slager , Bartomeu Monserrat

Van der Waals heterostructures constitute a platform for investigating intriguing many-body quantum phenomena. In particular, transition-metal dichalcogenide (TMD) hetero-bilayers host long-lived interlayer excitons which exhibit permanent…

Mesoscale and Nanoscale Physics · Physics 2022-09-14 Daniel Erkensten , Samuel Brem , Raül Perea-Causin , Ermin Malic

The rapidly increasing use of sensors throughout different research disciplines and the demand for more efficient devices with less power consumption depends critically on the emergence of new sensor materials and novel sensor concepts.…

Materials Science · Physics 2016-12-12 Maja Feierabend , Gunnar Berghäuser , Andreas Knorr , Ermin Malic

The optically dark states play an important role in the electronic and optical properties of monolayers (MLs) of semiconducting transition metal dichalcogenides. The effect of temperature on the in-plane-field activation of the neutral and…

We experimentally demonstrate hot exciton transport in h-BN encapsulated WSe2 monolayers via spatially and temporally resolved photoluminescence measurements at room temperature. We show that the nonlinear evolution of the mean squared…

Mesoscale and Nanoscale Physics · Physics 2019-12-11 Darwin F. Cordovilla Leon , Zidong Li , Sung Woon Jang , Parag B. Deotare

The time evolution from coherent states to squeezed states of high density excitons is studied theoretically based on the boson formalism and within the Random Phase Approximation. Both the mutual interaction between excitons and the…

Condensed Matter · Physics 2007-05-23 Nguyen Hong Quang

Many of the fundamental optical and electronic properties of atomically thin transition metal dichalcogenides are dominated by strong Coulomb interactions between electrons and holes, forming tightly bound atom-like excitons. Here, we…

Two-dimensional transition metal dichalcogenides (TMDs) provide an attractive platform for studying strain dependent exciton transport at room temperature due to large exciton binding energy and strong bandgap sensitivity to mechanical…

Mesoscale and Nanoscale Physics · Physics 2022-03-23 Kanak Datta , Zhengyang Lyu , Zidong Li , Takashi Taniguchi , Kenji Watanabe , Parag B. Deotare

The dynamics of excitons in a one-dimensional ensemble with partial spatial order are studied. During optical excitation, cold Rydberg atoms spontaneously organize into regular spatial arrangements due to their mutual interactions. This…

Atomic Physics · Physics 2013-11-01 S. Bettelli , D. Maxwell , T. Fernholz , C. S. Adams , I. Lesanovsky , C. Ates

Excitons, quasi particles composed of an electron and a hole, play an important role in optical responses in low-dimensional nanostructures. In this work, we have investigated exciton diffusion in a monolayer MoSe2 encapsulated between…

Mesoscale and Nanoscale Physics · Physics 2020-09-30 T. Hotta , S. Higuchi , A. Ueda , K. Shinokita , Y. Miyauchi , K. Matsuda , K. Ueno , T. Taniguchi , K. Watanabe , R. Kitaura

The equilibrium and non-equilibrium optical properties of single-layer transition metal dichalcogenides (TMDs) are determined by strongly bound excitons. Exciton relaxation dynamics in TMDs have been extensively studied by time-domain…

We study exciton radiative decay in a two-dimensional material, taking into account large thermal population in the non-radiative states, from which excitons are scattered into the radiative states by acoustic phonons. We find an analytical…

Mesoscale and Nanoscale Physics · Physics 2016-11-23 A. O. Slobodeniuk , D. M. Basko

Transition-metal dichalcogenides (TMDs) host tightly bound quasi-particles called excitons. Based on spin and momentum selection rules, these excitons can be either optically bright or dark. In tungsten-based TMDs, momentum-forbidden dark…

Semiconductor nanocrystals could replace conventional bulk materials completely in displays and light-emitting diodes. Exciton transport dominates over charge carrier transport for materials with high exciton binding energies and long…

Excitons in two-dimensional semiconductors provide a novel platform for fundamental studies of many-body interactions. In particular, dipolar interactions between spatially indirect excitons may give rise to strongly correlated phases of…

Mesoscale and Nanoscale Physics · Physics 2022-09-14 Rafał Ołdziejewski , Alessio Chiocchetta , Johannes Knörzer , Richard Schmidt

The optical properties of transition metal dichalcogenide monolayers such as the two-dimensional semiconductors MoS$_2$ and WSe$_2$ are dominated by excitons, Coulomb bound electron-hole pairs. The light emission yield depends on whether…

Materials Science · Physics 2016-03-23 J. P. Echeverry , B. Urbaszek , T. Amand , X. Marie , I. C. Gerber

The intricate interplay between optically dark and bright excitons governs the light-matter interaction in transition metal dichalcogenide monolayers. We have performed a detailed investigation of the "spin-forbidden" dark excitons in WSe2…

Atomically-thin transition metal dichalcogenide crystals (TMDCs) hold great promise for future semiconductor optoelectronics due to their unique electronic and optical properties. In particular, electron-hole pairs (excitons) in TMDCs are…

Mesoscale and Nanoscale Physics · Physics 2021-10-04 M. Wurdack , E. Estrecho , S. Todd , T. Yun , M. Pieczarka , S. K. Earl , J. A. Davis , C. Schneider , A. G. Truscott , E. A. Ostrovskaya

We have investigated the exciton dynamics in transition metal dichalcogenide mono-layers using time-resolved photoluminescence experiments performed with optimized time-resolution. For MoSe2 monolayers, we measure $\tau_{rad}=1.8\pm0.2$ ps…

Materials Science · Physics 2016-05-18 C. Robert , D. Lagarde , F. Cadiz , G. Wang , B. Lassagne , T. Amand , A. Balocchi , P. Renucci , S. Tongay , B. Urbaszek , X. Marie

Nanomaterials exhibit unique optical phenomena, in particular excitonic quantum processes occurring at room temperature. The low dimensionality, however, imposes strict requirements for conventional optical excitation, and an approach for…

Mesoscale and Nanoscale Physics · Physics 2023-12-15 N. Fang , D. Yamashita , S. Fujii , M. Maruyama , Y. Gao , Y. R. Chang , C. F. Fong , K. Otsuka , K. Nagashio , S. Okada , Y. K. Kato