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High pressure chemistry is known to inspire the creation of unexpected new classes of compounds with exceptional properties. Here we report the synthesis at ~90 GPa of novel beryllium polynitrides, monoclinic and triclinic BeN4. The…

Most recently, Bykov and coworkers reported the successful synthesis of layered structure of BeN4. Followed by the experimental report, Bafekry and coworkers published their first-principles results on the stability, electronic, optical and…

Materials Science · Physics 2021-09-03 Bohayra Mortazavi , Masoud Shahrokhi , Fazel Shojaei

The newly synthesized BeN4 monolayer has introduced a novel group of 2D materials called nitrogen-rich 2D materials. In the present study, the anisotropic mechanical and thermal properties of three members of this group, BeN4, MgN4, and…

Materials Science · Physics 2024-02-08 K. Ghorbani , P. Mirchi , S. Arabha , Ali Rajabpour , Sebastian Volz

Two-dimensional (2D) carbon nitride materials play an important role in energy-harvesting, energy-storage and environmental applications. Recently, a new carbon nitride, 2D polyaniline (C3N) was proposed [PNAS 113 (2016) 7414-7419]. Based…

Materials Science · Physics 2016-12-13 Linyang Li , Xiangru Kong , Ortwin Leenaerts , Xin Chen , Biplab Sanyal , François M. Peeters

Carbon nitride two-dimensional (2D) materials are among the most attractive class of nanomaterials, with wide range of application prospects. As a continuous progress, most recently, two novel carbon nitride 2D lattices of C3N5 and C3N4…

Chemical vapor deposition has been most recently employed to fabricate centimeter-scale high-quality single-layer MoSi2N4 (Science; 2020;369; 670). Motivated by this exciting experimental advance, herein we conduct extensive…

In the latest experimental advances, Ni-, Co- and Cu-HAB MOFs were synthesized in 2D forms, with high electrical conductivities and capacitances as well. Motivated by these experimental advances, we employed first-principles simulations to…

Computational Physics · Physics 2018-11-05 Bohayra Mortazavi , Masoud Shahrokhi , Meysam Makaremi , Gianaurelio Cuniberti , Timon Rabczuk

In this work, three novel porous carbon-nitride nanosheets with C7N6, C9N4 and C10N3 stoichiometries are predicted. First-principles simulations were accordingly employed to evaluate stability and explore the mechanical, electronic and…

Computational Physics · Physics 2019-08-19 Bohayra Mortazavi , Masoud Shahrokhi , Alexander V Shapeev , Timon Rabczuk , Xiaoying Zhuang

Motivated by the recent successful formation of the MoSi2N4 monolayer [Hong et al., Sci. 369, 670 (2020)], the structural, electronic and magnetic properties of MoSi2N4 nanoribbons (NRs) is investigated for the first time . The band…

Two-dimensional (2D) magnetic materials have attracted tremendous research interest because of the promising application in the next-generation microelectronic devices. Here, by the first-principles calculations, we propose a…

Materials Science · Physics 2024-06-19 Ming Yan , Z. Y. Xie , Miao Gao

Due to the flexibility of C and N atoms in forming different types of bonds, the prediction of new two-dimensional (2D) carbon nitrides is a hot topic in the field of carbon-based materials. Using first-principles calculations, we propose…

Materials Science · Physics 2024-01-09 Linyang Li , Jialei Li , Yawei Yu , Yuxuan Song , Jia Li , Xiaobiao Liu , François M. Peeters , Xin Chen , Guodong Liu

High pressure synthesis of rhenium nitride pernitride ReN$_2$ with crystal structure unusual for transition metal dinitrides and high values of hardness and bulk modulus attracted significant attention to this system. We investigate the…

Recently, a new type of two-dimensional layered material, i.e. C3N, has been fabricated by polymerization of 2,3-diaminophenazine and used to fabricate a field-effect transistor device with an on/off current ratio reaching 5.5E10 (Adv.…

Materials Science · Physics 2017-03-28 Haidi Wang , Hong Wu , Jinlong Yang

The existence of a new two dimensional CN2 structure was predicted using ab-initio molecular dynamics (AIMD) and density-functional theory calculations. It consists tetragonal and hexagonal rings with C-N and N-N bonds arranged in a…

Materials Science · Physics 2021-01-29 Qun Wei , Ying Yang , Alexander Gavrilov , Xihong Peng

Three two-dimensional phosphorus nitride (PN) monolayer sheets (named as $\alpha$-, $\beta$-, and $\gamma$-PN, respectively) with fantastic structures and properties are predicted based on first-principles calculations. The $\alpha$-PN and…

Materials Science · Physics 2015-10-02 ShuangYing Ma , Chaoyu He , L. Z. Sun , Haiping Lin , Youyong Li , K. W. Zhang

Structural, electronic, ferroelectric, and optical properties of two-dimensional (2D) BiN monolayer material with phosphorene-like structure are studied in terms of the density functional theory and modern Berry phase ferroelectric method.…

Materials Science · Physics 2017-11-28 Peng Chen , Xue-Jing Zhang , Bang-Gui Liu

Recently, Bafekry et al. [Appl. Phys. Lett. 119, 142102 (2021)] reported their density functional theory (DFT) results on the elastic constants of a novel C6N7 monolayer. They predicted a very soft elastic modulus of 36.29 GPa for the C6N7…

Materials Science · Physics 2022-04-25 Bohayra Mortazavi , Fazel Shojaei , and Masoud Shahrokhi

The seminal experimental discovery of the remarkably stable MoSi$_2$N$_4$ monolayer has led to a handful of predicted magnetic two-dimensional (2D) materials in the MA$_2$Z$_4$ family (M = transition metals, A = Si, Ge, and Z = N, P, As).…

Materials Science · Physics 2022-06-30 Dibyendu Dey , Avijeet Ray , Liping Yu

Two-dimensional (2D) multiferroic materials with controllable magnetism have promising prospects in miniaturized quantum device applications, such as high-density data storage and spintronic devices. Here, using first-principles…

Materials Science · Physics 2021-12-22 Shaowen Xu , Fanhao Jia , Xuli Cheng , Wei Ren

Experimental realization of single-layer MoSi2N4 is among the latest groundbreaking advances in the field of two-dimensional (2D) materials. Inspired by this accomplishment, herein we conduct first-principles calculations to explore the…

Materials Science · Physics 2021-08-31 Bohayra Mortazavi , Fazel Shojaei , Brahmanandam Javvaji , Timon Rabczuk , Xiaoying Zhuang
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