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The first quantum technology, which harnesses uniquely quantum mechanical effects for its core operation, has arrived in the form of commercially available quantum key distribution systems that achieve enhanced security by encoding…

Quantum Physics · Physics 2010-03-23 Jeremy L. O'Brien , Akira Furusawa , Jelena Vučković

Excitation energy transfer between photosynthetic light-harvesting complexes is vital for highly efficient primary photosynthesis. Controlling this process is the key for advancing the emerging artificial photosynthetic systems. Here, we…

Optics · Physics 2025-02-17 Fan Wu , Tu C. Nguyen- Phan , Richard Cogdell , Tonu Pullerits

Despite several different measures of efficiency that are applicable to the photosynthetic systems, a precise degree of efficiency of these systems is not completely determined. Introducing an efficient model for the dynamics of…

Chemical Physics · Physics 2020-06-24 Fatemeh Ghasemi , Afshin Shafiee

We develop a method to simulate the excitonic dynamics of realistic photosynthetic light harvesting systems including non-Markovian coupling to phonon degrees of freedom, under excitation by N-photon Fock state pulses. This method combines…

Biological Physics · Physics 2023-06-27 Liwen Ko , Robert L. Cook , K. Birgitta Whaley

Giant strides in ultrashort laser pulse technology have enabled real-time observation of dynamical processes in complex molecular systems. Specifically, the discovery of oscillatory transients in the two-dimensional electronic spectra of…

Chemical Physics · Physics 2021-03-08 Akihito Ishizaki , Graham R. Fleming

Optical detection of nanoscale objects without relying on fluorescence is a current challenge due to their extremely weak interaction with light. Resonator-enhanced absorption microscopy is a novel tool to heavily boost the light-matter…

The photosensitivity of silicon is inherently very low in the visible electromagnetic spectrum, and it drops rapidly beyond 800 nm in near-infrared wavelengths. Herein, we have experimentally demonstrated a technique utilizing…

Photosynthesis is a plausible pathway for the sustenance of a substantial biosphere on an exoplanet. In fact, it is also anticipated to create distinctive biosignatures detectable by next-generation telescopes. In this work, we explore the…

Earth and Planetary Astrophysics · Physics 2023-06-08 Manasvi Lingam , Amedeo Balbi , Swadesh M. Mahajan

One of the main concerns in traditional Wireless Sensor Networks (WSNs) is energy efficiency. In this work, we analyze two techniques that can extend network lifetime. The first is Ambient \emph{Energy Harvesting} (EH), i.e., the capability…

Information Theory · Computer Science 2016-01-18 Alessandro Biason , Michele Zorzi

The spatial collection efficiency portrays the driving forces and loss mechanisms in photovoltaic and photoelectrochemical devices. It is defined as the fraction of photogenerated charge carriers created at a specific point within the…

The question of how quantum coherence facilitates energy transfer has been intensively debated in the scientific community. Since natural and artificial light-harvesting units operate under the stationary condition, we address this question…

Chemical Physics · Physics 2020-07-22 Pei-Yun Yang , Jianshu Cao

Most of our current understanding of mechanisms of photosynthesis comes from spectroscopy. However, classical definition of radio-antenna can be extended to optical regime to discuss the function of light-harvesting antennae. Further to our…

Biological Physics · Physics 2019-04-09 Julian Juhi-Lian Ting

Panchromatic absorbing materials are widely regarded as a key strategy for enhancing solar energy utilization and photocurrent generation. However, in artificial molecular systems, broadening the absorption spectrum is often accompanied by…

Chemical Physics · Physics 2026-01-01 Hsien-Hsin Chou

Single-photon detectors have achieved impressive performance, and have led to a number of new scientific discoveries and technological applications. Existing models of photodetectors are semiclassical in that the field-matter interaction is…

Optics · Physics 2018-03-28 Steve M. Young , Mohan Sarovar , François Léonard

A number of applications in basic science and technology would benefit from high fidelity photon number resolving photodetectors. While some recent experimental progress has been made in this direction, the requirements for true photon…

Quantum Physics · Physics 2020-05-21 Steve M. Young , Mohan Sarovar , François Léonard

Electronic 2D spectroscopy allows nontrivial quantum effects in chemistry and biology to be explored in unprecedented detail. Here, we apply recently developed fluorescence detected coherent 2D spectroscopy to study the light harvesting…

The photovoltaic reciprocity theory relates the electroluminescence spectrum of a solar cell under applied bias to the external photovoltaic quantum efficiency of the device as measured at short circuit conditions. Its derivation is based…

Mesoscale and Nanoscale Physics · Physics 2017-06-21 Urs Aeberhard , Uwe Rau

Loss is a critical roadblock to achieving photonic quantum-enhanced technologies. We explore a modular platform for implementing integrated photonics experiments and consider the effects of loss at different stages of these experiments,…

Conventional photocells suffer a fundamental efficiency threshold imposed by the principle of detailed balance, reflecting the fact that good absorbers must necessarily also be fast emitters. This limitation can be overcome by `parking' the…

Quantum Physics · Physics 2016-11-15 Amir Fruchtman , Rafael Gómez-Bombarelli , Brendon W. Lovett , Erik M. Gauger
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