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Methanol is formed via surface reactions on icy dust grains. Methanol is also detected in the gas-phase at temperatures below its thermal desorption temperature and at levels higher than can be explained by pure gas-phase chemistry. The…

Solar and Stellar Astrophysics · Physics 2018-05-02 N. F. W. Ligterink , C. Walsh , R. G. Bhuin , S. Vissapragada , J. Terwisscha van Scheltinga , H. Linnartz

Porous heteroatom-doped carbons are desirable for catalytic reactions due to their tunable physicochemical properties, low cost and metal-free nature. Herein, we introduce a facile general bottom-up strategy, so-called "cooking carbon in a…

Chemical Physics · Physics 2019-01-16 Jiang Gong , Jinshui Zhang , Huijuan Lin , Jiayin Yuan

We report the discovery of a new class of molecular phases of solid nitrogen at high pressures and temperatures by Raman and infrared spectroscopy and powder x-ray diffraction. Unlike the molecular phases consisting of disk- and sphere-like…

We have studied the temperature dependence of the solubility of nitrogen in methane, ethane, and mixtures of methane and ethane using vapor-liquid equilibrium simulations of binary and ternary mixtures of nitrogen, methane and ethane for a…

Chemical Physics · Physics 2019-10-30 Pradeep Kumar , Vincent F. Chevrier

Solid and liquid sodium combustion with liquid water occurs through a thin gas layer where exothermic reactions happen with sodium and water vapors. It thus involves multiple interfaces separating liquid and gas in the presence of surface…

Computational Physics · Physics 2020-01-29 Damien Furfaro , Richard Saurel , Lucas David , François Beauchamp

We propose an approach that links density functional theory (DFT) and molecular dynamics (MD) simulation to study fluid behavior in nanopores in contact with bulk (macropores). It consists of two principal steps. First, the theoretical…

Computational Physics · Physics 2021-07-06 Mariia Vaganova , Irina Nesterova , Yuriy Kanygin , Andrey Kazennov , Aleksey Khlyupin

The fluid dynamics video shows the acoustophoretic handling of a metal sodium chunks and a water droplets before, during and after mixing. The violent exothermal reaction between solid and liquid introduces an additional phase (hydrogen…

Fluid Dynamics · Physics 2015-06-17 Daniele Foresti , Dimos Poulikakos

The US Department of Energy decided in 2000 to treat its sodium-bonded spent nuclear fuel, produced for experiments on breeder reactors, with an electrochemical process. The metallic waste produced is to be cast into ingots and the salt…

Diatomic nitrogen is an archetypal molecular system known for its exceptional stability and complex behavior at high pressures and temperatures, including rich solid polymorphism, formation of energetic states, and an insulator-to-metal…

Ultrafast synchrotron microtomography has been used to study in-situ and in real time the initial stages of silicate glass melt formation from crystalline granular raw materials. Significant and unexpected rearrangements of grains occur…

Nitrogen gas accidentally sealed in a sample container produces various spurious effects in elastic neutron scattering measurements. These effects are systematically investigated and the details of the spurious scattering are presented.

Diazo compounds are gathering interest for their potential in promoting greener synthesis routes. We investigate, at a lab-scale, the continuous synthesis of diazo acetonitrile (DAN) using a micro-structured flow reactor and a flow reaction…

Boron-doped multi-walled carbon nanotubes (MWNTs) were synthesized using a methanol solution of boric acid as a source material. Accurate measurements of the electrical resistivity of an individual boron-doped MWNT was performed with a…

The paper deals with analysis of a model of a multi-component fluid admitting chemical reactions. The flow is considered in the incompressible regime. The main result shows global existence of regular solutions under assumption of suitable…

Analysis of PDEs · Mathematics 2022-04-13 Piotr B. Mucha , Tomasz Piasecki

We have studied the pressure and temperature dependence of solubility of nitrogen in methane and ethane using vapor-liquid equilibrium simulations of binary mixtures of nitrogen in methane and ethane for a range of pressures between 1.5 atm…

Soft Condensed Matter · Physics 2020-02-18 Pradeep Kumar , Vincent F. Chevrier

Bulk nanobubbles (NBs) generated electrochemically by short voltage pulses of alternating polarity behave differently from those produced by regular methods. Only bubbles smaller than $200\;$nm are formed in the process and their…

Soft Condensed Matter · Physics 2021-02-08 Vitaly B. Svetovoy

Melanins are promising materials for organic bioelectronics devices like transistors, sensors and batteries. However, in general, melanin either natural or synthetic has low solubility in most solvents. In this study, the chemical…

Theoretical calculations of the conductivity of sodium nitrate in water are presented and compared with experimental measurements. The method of direct correlation force in the framework of the interionic theory is used for the calculation…

Soft Condensed Matter · Physics 2013-12-17 H. Krienke

Kinetic Monte-Carlo simulation is applied to study the partial oxidation of methane over a nickel catalyst. Based on the Langmuir-Hinshelwood mechanism, the kinetic behavior of this reaction is analyzed and the results are compared with…

Materials Science · Physics 2016-06-13 Sirawit Pruksawan , Boonyarach Kitiyanan , Robert M. Ziff

Methane is typically thought to be formed in the solid state on the surface of cold interstellar icy grain mantles via the successive atomic hydrogenation of a carbon atom. In the current work we investigate the potential role of molecular…

Astrophysics of Galaxies · Physics 2022-04-06 Thanja Lamberts , Gleb Fedoseev , Marc van Hemert , Danna Qasim , Ko-Ju Chuang , Julia C. Santos , Harold Linnartz