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We perform accurate calculations of the dependence of transition frequencies in two valence electron atoms and ions on a variation of the fine structure constant, alpha. The relativistic Hartree-Fock method is used with many-body…

Atomic Physics · Physics 2009-02-05 E. J. Angstmann , V. A. Dzuba , V. V. Flambaum

We investigate the existence of holomorphic Hartree-Fock solutions using a revised SCF algorithm. We use this algorithm to study the Hartree-Fock solutions for H$_{2}$ and H$_{4}^{2+}$ and report the emergence of holomorphic solutions at…

Chemical Physics · Physics 2015-11-20 Hugh G. A. Burton , Alex J. W. Thom

Octupole vibrations are studied in some doubly magic nuclei using the time-dependent Hartree-Fock (TDHF) theory with a Skyrme energy density functional. Through the use of the linear response theory, the energies and transition amplitudes…

Nuclear Theory · Physics 2016-09-07 C. Simenel , J. Buete , K. Vo-Phuoc

The Hartree-Fock equation which is the Euler-Lagrange equation corresponding to the Hartree-Fock energy functional is used in many-electron problems. Since the Hartree-Fock equation is a system of nonlinear eigenvalue problems, the study of…

Analysis of PDEs · Mathematics 2023-06-23 Sohei Ashida

By the use of integer and noninteger n-Slater Type Orbitals in combined Hartree-Fock-Roothaan method, self consistent field calculations of orbital and lowest states energies have been performed for the isoelectronic series of open shell…

Chemical Physics · Physics 2012-10-10 I. I. Guseinov , M. Erturk , E. Sahin

The Hartree-Fock based diagonalization is a computational method for the investigation of the low-energy properties of correlated electrons in disordered solids. The method is related to the quantum-chemical configuration interaction…

Disordered Systems and Neural Networks · Physics 2007-05-23 Michael Schreiber , Thomas Vojta

Time-dependent Hartree-Fock theory is used to describe density oscillations of symmetry-unrestricted two-dimensional nanostructures. In the small amplitude limit the results reproduce those obtained within a perturbative approach such as…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Antonio Puente , Llorenç Serra , Vidar Gudmundsson

We introduce the Deep Post-Hartree-Fock (DeePHF) method, a machine learning based scheme for constructing accurate and transferable models for the ground-state energy of electronic structure problems. DeePHF predicts the energy difference…

Chemical Physics · Physics 2020-08-11 Yixiao Chen , Linfeng Zhang , Han Wang , Weinan E

We describe the new version 2.00d of the code HFBTHO that solves the nuclear Skyrme Hartree-Fock (HF) or Skyrme Hartree-Fock-Bogolyubov (HFB) problem by using the cylindrical transformed deformed harmonic-oscillator basis. In the new…

Nuclear Theory · Physics 2013-03-19 M. V. Stoitsov , N. Schunck , M. Kortelainen , N. Michel , H. Nam , E. Olsen , J. Sarich , S. Wild

The evaluation of exact (Hartree--Fock, HF) exchange operator is a crucial ingredient for the accurate description of electronic structure in periodic systems through ab initio and hybrid density functional approaches. An efficient…

Chemical Physics · Physics 2020-10-28 Xiao Wang , Cannada A. Lewis , Edward F. Valeev

The two-basis method to solve the HFB for deformed nuclei in coordinate space is examined concerning the precision of the density tail. Small cutoff energies are shown to give rise to ripples in the tail, whose wave length corresponds to…

Nuclear Theory · Physics 2007-05-23 Naoki Tajima

Hartree-Fock calculations with the SKX Skyrme interaction are carried out to obtain alpha-decay Q values for deformed nuclei above $^{208}$Pb assuming axial symmetry. The results for even-even nuclei are compared with experiment and with…

Nuclear Theory · Physics 2008-11-26 S. Typel , B. A. Brown

For neutral and positively charged atoms and molecules, we prove the existence of infinitely many Hartree-Fock critical points below the first energy threshold (that is, the lowest energy of the same system with one electron removed). This…

Mathematical Physics · Physics 2017-11-22 Mathieu Lewin

We present the first of a two-part Mathematica notebook collection that implements a symbolic approach for the application of the density matrix expansion (DME) to the Hartree-Fock (HF) energy from a chiral effective field theory (EFT)…

Computational Physics · Physics 2010-04-22 B. Gebremariam , S. K. Bogner , T. Duguet

Analytical Hartree-Fock gradients with respect to the cell parameter have been implemented in the electronic structure code CRYSTAL, for the case of three-dimensional periodicity. The code is based on Gaussian type orbitals, and the…

Materials Science · Physics 2007-05-23 K. Doll , R. Dovesi , R. Orlando

We consider here variational solutions in the Hartree-Fock approximation upon breaking time reversal and axial symmetries. When decomposed on axial harmonic oscillator functions, the corresponding single particle triaxial eigenstates as…

Nuclear Theory · Physics 2009-10-31 D. Samsoen , P. Quentin , J. Bartel

The Fock exchange operator plays a central role in modern quantum chemistry. The large computational cost associated with the Fock exchange operator hinders Hartree-Fock calculations and Kohn-Sham density functional theory calculations with…

Computational Physics · Physics 2020-05-22 Lin Lin

By introducing a density-dependent contact term, M3Y-type interactions applicable to the Hartree-Fock calculations are developed. In order to view basic characters of the interactions, we carry out calculations on the uniform nuclear matter…

Nuclear Theory · Physics 2009-11-10 H. Nakada

In this paper we study the problem of uniqueness of solutions to the Hartree and Hartree-Fock equations of atoms. We show, for example, that the Hartree-Fock ground state of a closed shell atom is unique provided the atomic number $Z$ is…

Mathematical Physics · Physics 2015-05-20 M. Griesemer , F. Hantsch

This work presents exchange potentials for specific orbitals calculated by inverting Hartree-Fock wavefunctions. This was achieved by using a Depurated Inversion Method. The basic idea of the method relies upon the substitution of…

Atomic and Molecular Clusters · Physics 2016-10-21 A. M. P. Mendez , D. M. Mitnik , J. E. Miraglia
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