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Related papers: Many-body theory of positron binding in polyatomic…

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Electron-positron interactions have been utilized in various fields of science. Here we develop time-dependent multi-component density functional theory to study the coupled electron-positron dynamics from first principles. We prove that…

Chemical Physics · Physics 2018-10-03 Yasumitsu Suzuki , Satoshi Hagiwara , Kazuyuki Watanabe

Computational studies have shown that one or more positrons can stabilize two repelling atomic anions through the formation of two-center positronic bonds. In the present work, we study the energetic stability of a system containing two…

A particular difficulty in studying many-body interactions in a solid is the absence of an experimental technique that can directly probe their key characteristics. We show that 2D Fourier spectroscopy provides an efficient tool for the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Mikhail Erementchouk , Michael N. Leuenberger , L. J. Sham

Some recent results concerning nonlinear optics in semiconductor microcavities are reviewed from the point of view of the many-body physics of an interacting photon gas. Analogies with systems of cold atoms at thermal equilibrium are drawn,…

Statistical Mechanics · Physics 2009-11-11 Iacopo Carusotto , Michiel Wouters , Cristiano Ciuti

The many-body system comprising a He nucleus, three electrons, and a positron has been studied using the exact diagonalization technique. The purpose has been to clarify to which extent the system can be considered as a distinguishable…

Atomic and Molecular Clusters · Physics 2013-05-31 A. Zubiaga , F. Tuomisto , M. J. Puska

The method of many-body Green's functions is developed for arbitrary systems of electrons and nuclei starting from the full (beyond Born-Oppenheimer) Hamiltonian of Coulomb interactions and kinetic energies. The theory presented here…

Other Condensed Matter · Physics 2020-06-23 Ville J. Härkönen , Robert van Leeuwen , E. K. U. Gross

A method is proposed for detecting positron-atom bound states by observing enhanced positron annihilation due to electronic Feshbach resonances at electron-volt energies. The method is applicable to a range of open-shell transition metal…

Atomic Physics · Physics 2010-12-10 V. A. Dzuba , V. V. Flambaum , G. F. Gribakin

Measurements of energy-resolved positron-molecule annihilation show the existence of positron binding and vibrational Feshbach resonances. The existing theory describes this phenomenon successfully for the case of infrared-active…

Atomic Physics · Physics 2017-09-25 M. R. Natisin , J. R. Danielson , G. F. Gribakin , A. R. Swann , C. M. Surko

A large collaboration carefully benchmarks 20 first principles many-body electronic structure methods on a test set of 7 transition metal atoms, and their ions and monoxides. Good agreement is attained between the 3 systematically converged…

In this work we define single-particle potentials for a positron and a positronium atom interacting with light atoms (H, He, Li and Be) by inverting a single-particle Schr\"odinger equation. For this purpose, we use accurate energies and…

Atomic and Molecular Clusters · Physics 2014-05-21 A. Zubiaga , F. Tuomisto , M. Puska

Mijnarends et al. [J. Phys. Condens. Matter {\bf 10}, 10383 (1998)] contested the best existing calculations of positron annihilation rates in jellium and crystal lattices, pointing in this way at deficiencies of existing theories of…

Soft Condensed Matter · Physics 2007-05-23 H. Stachowiak , E. Boronski

Angular resolved photoelectron spectra of metal clusters have been experimentally measured for the first time only recently. These measurements have been performed systematically for sodium clusters in a broad range of cluster sizes. This…

Atomic and Molecular Clusters · Physics 2009-05-04 Andrey V. Solov'yov , Roman G. Polozkov , Vadim K. Ivanov

Polymorphs in molecular crystals are often very close in energy, yet they may possess markedly different physical and chemical properties. The understanding and prediction of polymorphism is of paramount importance for a variety of…

The Many-Body Expansion (MBE) is a useful tool to simulate condensed phase chemical systems, often avoiding the steep computational cost of usual electronic structure methods. However, it often requires higher than 2-body terms to achieve…

Chemical Physics · Physics 2019-11-21 Srimukh Prasad Veccham , Joonho Lee , Martin Head-Gordon

The positronium molecule (Ps$_2$) has not been experimentally observed yet because its tiny (4.5 eV) binding energy cannot be detected when the molecule annihilates by emitting two photons with energy of 0.51 MeV each. It is shown in this…

Atomic Physics · Physics 2009-10-31 J. Usukura , K. Varga , Y. Suzuki

A many-body Green's function approach to the microscopic theory of surface-enhanced Raman scattering is presented. Interaction effects between a general molecular system and a spatially anisotropic metal particle supporting plasmon…

Quantum Physics · Physics 2008-10-18 David J. Masiello , George C. Schatz

Recent experimental progress in the field of cavity quantum electrodynamics allows to study the regime of strong interaction between quantized light and complex matter systems. Due to the coherent coupling between photons and matter-degrees…

Quantum Physics · Physics 2021-02-24 Florian Buchholz

Molecular polaritons are hybrid states of photonic and molecular character that form when molecules strongly interact with light. Strong coupling tunes energy levels and importantly, can modify molecular properties (e.g. photoreaction…

Chemical Physics · Physics 2023-02-14 Francesca Fassioli , Kyu Hyung Park , Sarah E. Bard , Gregory D. Scholes

In this paper we report first-principles calculations on the ground-state electronic structure of two infinite one-dimensional systems: (a) a chain of carbon atoms and (b) a chain of alternating boron and nitrogen atoms. Meanfield results…

Condensed Matter · Physics 2010-01-14 Ayjamal Abdurahman , Alok Shukla , Michael Dolg

An effective theory of the excited states of positronium is derived and some of its consequences are explored. At large physical separation, the binding of the electron and positron is assumed to be described completely by QED, whereas all…

High Energy Physics - Phenomenology · Physics 2022-06-07 David M. Jacobs