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We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…

Quantum Physics · Physics 2021-06-23 Zhedong Zhang , Tao Peng , Xiaoyu Nie , Girish S. Agarwal , Marlan O. Scully

We show that the quantum disentanglement eraser implemented on a two-photon system from parametric down-conversion is a general method to create hybrid photonic entanglement, namely the entanglement between different degrees of freedom of…

Quantum Physics · Physics 2015-05-13 Leonardo Neves , Gustavo Lima , Aldo Delgado , Carlos Saavedra

The electronic entanglement between two free atoms initially at rest is obtained including the effects of photon recoil, for the case when quantum dispersion can be neglected during the atomic excited-state lifetime. Different from previous…

Quantum Physics · Physics 2015-05-14 F. Lastra , S. Wallentowitz

Quantum information theory is a multidisciplinary field whose objective is to understand what happens when information is stored in the state of a quantum system. Quantum mechanics provides us with a new resource, called quantum…

Quantum Physics · Physics 2011-05-25 Nicolas Dutil

Quantum frequency up-conversion is a cutting-edge technique that leverages the interaction between photons and quantum systems to shift the frequency of single photons from a lower frequency to a higher frequency. If the photon before…

Quantum Physics · Physics 2024-04-02 Jiaxuan Wang , Alexei V. Sokolov , Girish S. Agarwal

We present a theoretical analysis of two-photon absorption of classical and squeezed light valid when one-photon absorption to an intermediate state is either resonant or far-detuned from resonance, and in both the low and high intensity…

Quantum Physics · Physics 2022-09-14 Christian Drago , John Sipe

The entanglement dynamics of two independent qubits each embedded in a structured environment under conditions of inhibition of spontaneous emission is analyzed, showing entanglement trapping. We demonstrate that entanglement trapping can…

Quantum Physics · Physics 2010-03-30 Bruno Bellomo , Rosario Lo Franco , Sabrina Maniscalco , Giuseppe Compagno

Enhancing quantum entanglement is important for many quantum information processing applications. In this paper, we consider a protocol for entanglement enhancing in a two-mode squeezed vacuum state (TMSVS), attained based on photon…

Quantum Physics · Physics 2022-06-07 Jiru Liu , Yusef Maleki , M. Suhail Zubairy

When a quantum particle traverses a rectangular potential created by a quantum field both photon exchange and entanglement between particle and field take place. We present analytic results for the transition amplitudes of any possible…

Quantum Physics · Physics 2015-06-11 Georg Sulyok , Katharina Durstberger-Rennhofer , Johann Summhammer

When a metastable state decays into radiation, there must be entanglement between the radiation and the decaying system, as well as between radiation collected at late and early times. We study the interplay between these two types of…

Quantum Physics · Physics 2026-04-13 Sergei Khlebnikov

We show a mechanism that projects a pair of neutral two-level atoms from an initially uncorrelated state to a maximally entangled state while they remain spacelike separated. The atoms begin both excited in a common electromagnetic vacuum,…

Quantum Physics · Physics 2009-11-13 Juan León , Carlos Sabín

We present a simple treatment for the phenomenon of parametric downconversion considering the coherent scattering of one pump photon into a photon pair by a nonlinear crystal. The energy and momentum entanglement of the quantum state of the…

Quantum Physics · Physics 2013-01-15 Pablo L. Saldanha , C. H. Monken

We report how the unique temporal and spectral features of pulsed entangled photons from a parametric downconversion source can be utilized for manipulating electronic excitations through the optimization of their spectral phase. A new…

Chemical Physics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

Most experimental demonstrations of entanglement require nonclassical states and correlated measurements of single-photon detection events. It is shown here that entanglement can produce a large decrease in the rate of two-photon absorption…

Quantum Physics · Physics 2009-11-11 J. D. Franson

The role of the timing and order of quantum measurements is not just a fundamental question of quantum mechanics, but also a puzzling one. Any part of a quantum system that has finished evolving, can be measured immediately or saved for…

Quantum Physics · Physics 2014-02-04 E. Megidish , A. Halevy , T. Shacham , T. Dvir , L. Dovrat , H. S. Eisenberg

We report on experimental evidences of the preservation of energy-time entanglement for extraordinary plasmonic light transmission through sub-wavelength metallic hole arrays, and for long range surface plasmon polaritons. Plasmons are…

Quantum Physics · Physics 2013-01-22 Sylvain Fasel , Nicolas Gisin , Hugo Zbinden , Daniel Erni , Esteban Moreno , Frank Robin

We describe a new experimental approach to probabilistic atom-photon (signal) entanglement. Two qubit states are encoded as orthogonal collective spin excitations of an unpolarized atomic ensemble. After a programmable delay, the atomic…

Multiparticle entangled states generated via interaction between narrow-band light and an ensemble of identical two-level atoms are considered. Depending on the initial photon statistics, correlation between atoms and photons can give rise…

Quantum Physics · Physics 2009-11-11 V. N. Gorbachev , A. I. Trubilko

We observe that a weak guided light field transmitted through an ensemble of atoms coupled to an optical nanofiber exhibits quadrature squeezing. From the measured squeezing spectrum we gain direct access to the phase and amplitude of the…

Quantum light spectroscopy, providing novel molecular information non-accessible by classical light, necessitates new computational tools when applied for complex molecular systems. We introduce two computational protocols for the molecular…

Chemical Physics · Physics 2021-09-14 Bing Gu , Daniel Keefer , Shaul Mukamel